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  • Park, Youjin, et al. (author)
  • Sub-30 nm 2D Perovskites Patterns via Block Copolymer Guided Self-Assembly for Color Conversion Optical Polarizer
  • 2023
  • In: Small. - : WILEY-V C H VERLAG GMBH. - 1613-6810 .- 1613-6829.
  • Journal article (peer-reviewed)abstract
    • Despite the remarkable advances made in the development of 2D perovskites suitable for various high-performance devices, the development of sub-30 nm nanopatterns of 2D perovskites with anisotropic photoelectronic properties remains challenging. Herein, a simple but robust route for fabricating sub-30 nm 1D nanopatterns of 2D perovskites over a large area is presented. This method is based on nanoimprinting a thin precursor film of a 2D perovskite with a topographically pre-patterned hard poly(dimethylsiloxane) mold replicated from a block copolymer nanopattern consisting of guided self-assembled monolayered in-plane cylinders. 1D nanopatterns of various 2D perovskites (A & PRIME;(2)MA(n)(-1)Pb(n)X(3)(n)(+1),A & PRIME; = BA, PEA, X = Br, I) are developed; their enhanced photoluminescence (PL) quantum yields are approximately four times greater than those of the corresponding control flat films. Anisotropic photocurrent is observed because 2D perovskite nanocrystals are embedded in a topological 1D nanopattern. Furthermore, this 1D metal-coated nanopattern of a 2D perovskite is employed as a color conversion optical polarizer, in which polarized PL is developed. This is due to its capability of polarization of an incident light arising from the sub-30 nm line pattern, as well as the PL of the confined 2D perovskite nanocrystals in the pattern.
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Type of publication
journal article (1)
Type of content
peer-reviewed (1)
Author/Editor
Kim, Jiwon (1)
Kim, Sohee (1)
Park, Taehyun (1)
Park, Cheolmin (1)
Park, Youjin (1)
Han, Hyowon (1)
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Lee, Hyeokjung (1)
Jang, Jihye (1)
Kim, Gwanho (1)
Park, Yemin (1)
Lee, Jiyeon (1)
Kim, Dongjun (1)
Jung, Yeon Sik (1)
Jeong, Beomjin (1)
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University
Linköping University (1)
Language
English (1)
Research subject (UKÄ/SCB)
Natural sciences (1)
Year

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