1. |
- Arnold, C. L., et al.
(author)
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The ELI-ALPS secondary sources : A getaway to scientific excellence
- 2013
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In: 2013 Conference on Lasers and Electro-Optics, CLEO 2013. - 9781557529725 ; 2013
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Conference paper (peer-reviewed)abstract
- The essence of ELI-ALPS, the laser driven secondary sources ranging from X-ray and X-UV to THz with duration as short as tens of attoseconds, are designed to be available for users from 2016.
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2. |
- Kolliopoulos, G., et al.
(author)
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Single-shot autocorrelator for extreme-ultraviolet radiation
- 2014
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In: Journal of the Optical Society of America. B, Optical physics. - : Optical Society of America. - 0740-3224 .- 1520-8540. ; 31:5, s. 926-938
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Journal article (peer-reviewed)abstract
- A novel single-shot second-order autocorrelation scheme for extreme-ultraviolet radiation (XUV) is proposed. It is based on an ion-imaging technique, which provides spatial information of ionization products in the focal volume of the XUV beam. Using simple analytical and detailed numerical modeling, an evaluation toward selecting an optimum configuration has been performed. The implementation of the concept to characterize attosecond pulses is discussed, and the proposed setups are assessed.
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3. |
- Kolliopoulos, G., et al.
(author)
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Revealing quantum path details in high-field physics
- 2014
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In: Physical Review A. Atomic, Molecular, and Optical Physics. - : American Physical Society. - 1050-2947 .- 1094-1622. ; 90:1
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Journal article (peer-reviewed)abstract
- The fundamental mechanism underlying harmonic emission in the strong-field regime is governed by tunnel ionization of the atom, followed by the motion of the electron wave packet in the continuum, and finally by its recollision with the atomic core. Due to the quantum nature of the process, the properties of the electron wave packet strongly correlate with those of the emitted radiation. Here, by spatially resolving the interference pattern generated by overlapping the harmonic radiation emitted by different interfering electron quantum paths, we have succeeded in unravelling the intricacies associated with the recollision process. This has been achieved by mapping the spatial extreme-ultraviolet (EUV)-intensity distribution onto a spatial ion distribution, produced in the EUV focal area through the linear and nonlinear processes of atoms. By in situ manipulation of the intensity-dependent motion of the electron wave packets, we have been able to directly measure the difference between the harmonic emission times and electron path lengths resulting from different electron trajectories. Due to the high degree of accuracy that the present approach provides, we have been able to demonstrate the quantum nature of the recollision process. This is done by quantitatively correlating the photoemission time and the electron quantum path-length differences, taking into account the energy-momentum transfer from the driving laser field into the system. This information paves the way for electron-photon correlation studies at the attosecond time scale, while it puts the recollision process from the semiclassical prospective into a full quantum-mechanical context.
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4. |
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5. |
- Makos, I, et al.
(author)
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Α 10-gigawatt attosecond source for non-linear XUV optics and XUV-pump-XUV-probe studies
- 2020
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In: Scientific Reports. - : Springer Science and Business Media LLC. - 2045-2322. ; 10:1
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Journal article (peer-reviewed)abstract
- The quantum mechanical motion of electrons and nuclei in systems spatially confined to the molecular dimensions occurs on the sub-femtosecond to the femtosecond timescales respectively. Consequently, the study of ultrafast electronic and, in specific cases, nuclear dynamics requires the availability of light pulses with attosecond (asec) duration and of sufficient intensity to induce two-photon processes, essential for probing the intrinsic system dynamics. The majority of atoms, molecules and solids absorb in the extreme-ultraviolet (XUV) spectral region, in which the synthesis of the required attosecond pulses is feasible. Therefore, the XUV spectral region optimally serves the study of such ultrafast phenomena. Here, we present a detailed review of the first 10-GW class XUV attosecond source based on laser driven high harmonic generation in rare gases. The pulse energy of this source largely exceeds other laser driven attosecond sources and is comparable to the pulse energy of femtosecond Free-Electron-Laser (FEL) XUV sources. The measured pulse duration in the attosecond pulse train is 650 ± 80 asec. The uniqueness of the combined high intensity and short pulse duration of the source is evidenced in non-linear XUV-optics experiments. It further advances the implementation of XUV-pump-XUV-probe experiments and enables the investigation of strong field effects in the XUV spectral region.
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6. |
- Bergues, B., et al.
(author)
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Nonlinear interaction of 100-eV attosecond XUV-pulses with core electrons in Xenon
- 2018
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In: Optics InfoBase Conference Papers. - : Optica Publishing Group. - 9781557528209
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Conference paper (peer-reviewed)abstract
- We demonstrate multiphoton ionization of inner-shell electrons in Xenon with 100-eV attosecond pulses. This was achieved with a novel XUV source based on high-harmonic generation in the gas phase driven with multi-TW few-cycle laser pulses.
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7. |
- Bergues, B., et al.
(author)
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Tabletop nonlinear optics in the 100-eV spectral region
- 2018
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In: Optica. - : Optical Society of America. - 2334-2536. ; 5:3, s. 237-242
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Journal article (peer-reviewed)abstract
- Nonlinear light-matter interactions in the extreme ultraviolet (XUV) are a prerequisite to perform XUV-pump/XUV-probe spectroscopy of core electrons. Such interactions are now routinely investigated at free-electron laser (FEL) facilities. Yet, electron dynamics are often too fast to be captured with the femtosecond resolution of state-of-the-art FELs. Attosecond pulses from laser-driven XUV-sources offer the necessary temporal resolution. However, intense attosecond pulses supporting nonlinear processes have only been available for photon energy below 50 eV, precluding XUV-pump/XUV-probe investigation of typical inner-shell processes. Here, we surpass this limitation by demonstrating two-photon absorption from inner electronic shells of xenon at photon energies around 93 eV and 115 eV. This advance opens the door for attosecond real-time observation of nonlinear electron dynamics deep inside atoms.
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8. |
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9. |
- Rivas, D. E., et al.
(author)
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Next Generation Driver for Attosecond and Laser-plasma Physics
- 2017
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In: Scientific Reports. - : Nature Publishing Group. - 2045-2322. ; 7
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Journal article (peer-reviewed)abstract
- The observation and manipulation of electron dynamics in matter call for attosecond light pulses, routinely available from high-order harmonic generation driven by few-femtosecond lasers. However, the energy limitation of these lasers supports only weak sources and correspondingly linear attosecond studies. Here we report on an optical parametric synthesizer designed for nonlinear attosecond optics and relativistic laser-plasma physics. This synthesizer uniquely combines ultra-relativistic focused intensities of about 10(20)W/cm(2) with a pulse duration of sub-two carrier-wave cycles. The coherent combination of two sequentially amplified and complementary spectral ranges yields sub-5-fs pulses with multi-TW peak power. The application of this source allows the generation of a broad spectral continuum at 100-eV photon energy in gases as well as high-order harmonics in relativistic plasmas. Unprecedented spatio-temporal confinement of light now permits the investigation of electric-field-driven electron phenomena in the relativistic regime and ultimately the rise of next-generation intense isolated attosecond sources.
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10. |
- Tsatrafyllis, N., et al.
(author)
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The ion microscope as a tool for imaging the ion distribution produced by linear and non-linear processes at the focus of an XUV beam
- 2017
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In: 2017 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC). - : IEEE. - 9781509067367
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Conference paper (peer-reviewed)abstract
- Summary form only given. We demonstrate a tool for quantitative measurements in the linear and non-linear extreme ultraviolet (XUV) spectral region measuring spatially resolved atomic ionization products at the focus of an XUV beam [1, 2]. The ionizing radiation is a comb of the 11th-15th harmonics of a Ti:Sapphire femtosecond laser beam produced in a Xenon gas jet. The spatial ion distribution at the focus of the harmonics is recorded using an ion microscope detector [2, 3]. Spatially resolved single- and two-photon ionization products of Argon and Helium are observed. From such ion distributions single- and two-photon generalized cross sections have be extracted by a self-calibrating method. This is the first observation of spatially resolved two-XUV-photon ionization at the focus of the XUV radiation which constitutes an important step towards future single-shot temporal characterization of attosecond (asec) pulses [4].
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