1. |
- Karis, O., et al.
(author)
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Observation of short- and long-range hybridization of a buried Cu monolayer in Ni
- 2000
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In: Physical Review B Condensed Matter. - 0163-1829 .- 1095-3795. ; 62:24, s. R16239-R16242
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Journal article (peer-reviewed)abstract
- The electronic structure of a Cu monolayer buried in Ni fcc(100) is studied by means of x-ray emission and absorption spectroscopies in combination with first principles calculations. The local character of the x-ray probes allows us to investigate changes in the chemical interaction for these ultrathin film systems. In comparison to bulk Cu, the occupied d states of a buried Cu monolayer, as mapped in the x-ray emission spectrum, remain mostly unaltered. The absorption spectrum on the other hand shows that the empty states of the buried Cu monolayer are modified, and instead resemble the unoccupied electronic density of bulk Ni. These findings agree well with our first principle electronic structure calculations and the results are interpreted in terms of short- and long-range hybridization.
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2. |
- Karis, O, et al.
(author)
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Probing surface states of Cu/Ni thin films using x-ray absorption spectroscopy
- 2001
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In: Physical Review B. Condensed Matter and Materials Physics. - 1098-0121 .- 1550-235X. ; 63:11
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Journal article (peer-reviewed)abstract
- Surface and interface properties of Cu thin films (1–4 monolayers) deposited on Ni(100) have been extracted by means of x-ray absorption spectroscopy and analyzed in combination with ab initio density-functional calculations. An unoccupied Cu surface state is identified in an x-ray absorption spectra and studied as a function of film thickness. Experimental data is supported by calculations of the layer-resolved density of states and the results from this combined theoretical-experimental effort show that the surface state is almost entirely located on the atomic layer closest to the vacuum. Our results also indicate strong hybridization between unoccupied states at the Cu/Ni interface boundary.
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3. |
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4. |
- Wassdahl, N., et al.
(author)
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Soft x-ray emission studies of adsorbates
- 1992
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In: Physical Review Letters. - 0031-9007. ; 69:5, s. 812-815
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Journal article (peer-reviewed)abstract
- Soft x-ray emission spectroscopy is for the first time applied to surfaces and adsorbates. Surface sensitivity is achieved by employing synchrotron radiation in grazing incidence for the excitation. We present O K emission from adsorbed atomic oxygen on Ni(100) and Cu(100) and molecular CO on Ni(100). The observed spectral features correspond to the occupied 2p partial density of states of the adsorbates.
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5. |
- Denecke, R., et al.
(author)
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Beamline 1511 at MAX II, capabilities and performance
- 1999
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In: Journal of Electron Spectroscopy and Related Phenomena. - 0368-2048. ; 101-103, s. 971-977
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Journal article (peer-reviewed)abstract
- The new undulator beamline 1511 at MAX-lab, now under commissioning, has been optimized for X-ray emission and photoelectron spectroscopies. Using an SX-700 high flux monochromator the accessible photon energy range is from 90 eV to about 1500 eV. The performance of the undulator agrees very well with the specifications, as shown by measurements using a photodiode. The energy resolution of the monochromator has been checked using absorption measurements in a gas cell. It was found to meet the expectations and exceeds a resolving power of 10 000 at 244 eV. The photon flux as a function of energy has been recorded as well and gives a maximum flux of 3×1013 photons/s/100 mA/0.1% BW. Beamlines 1511 and 1411 will be the first synchrotron beamlines making use of a so-called beam waist phenomenon, known from laser physics. We show results of ray-tracing calculations to determine the ultimate spot size on the sample location. The endstations to be used at this new beamline and their capabilities will be discussed as an example of the future use of this facility.
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6. |
- Denecke, R, et al.
(author)
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Beamline I511 at MAX II, capabilities and performance
- 1999
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In: JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA. - : ELSEVIER SCIENCE BV. - 0368-2048. ; 103, s. 971-977
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Journal article (other academic/artistic)abstract
- The new undulator beamline I511 at MAX-lab, now under commissioning, has been optimized for X-ray emission and photoelectron spectroscopies. Using an SX-700 high flux monochromator the accessible photon energy range is from 90 eV to about 1500 eV. The per
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7. |
- Fohlisch, A, et al.
(author)
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Beyond the chemical shift: Vibrationally resolved core-level photoelectron spectra of adsorbed CO
- 1998
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In: PHYSICAL REVIEW LETTERS. - : AMERICAN PHYSICAL SOC. - 0031-9007. ; 81:8, s. 1730-1733
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Journal article (other academic/artistic)abstract
- Vibrational fine structure has been observed in the Cls and O1s photoelectron lines of CO adsorbed on Ni(100). This allows a detailed separation of vibrational and electronic contributions to the line profile. The main line is found to represent the fully
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8. |
- Karis, O, et al.
(author)
-
Observation of short- and long-range hybridization of a buried Cu monolayer in Ni
- 2000
-
In: PHYSICAL REVIEW B. - 0163-1829. ; 62:24, s. R16239-R16242
-
Journal article (peer-reviewed)abstract
- The electronic structure of a Cu monolayer buried in Ni fcc(100) is studied by means of x-ray emission and absorption spectroscopies in combination with first principles calculations. The local character of the x-ray probes allows us to investigate change
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9. |
- Karis, O, et al.
(author)
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One-step and two-step description of deexcitation processes in weakly interacting systems
- 1996
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In: PHYSICAL REVIEW LETTERS. - : AMER INST PHYSICS. ; 76:8, s. 1380-1383
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Journal article (other academic/artistic)abstract
- The origin of one- and two-step behavior of core-hole decay processes is identified in connection with high resolution autoionization spectra for Ar/Pt(111). The spectra simultaneously show features of the two types (resonant Raman vs Auger-like behavior)
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10. |
- Magnuson, Martin, 1965-, et al.
(author)
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Coherent and Incoherent Processes in resonant Photoemission
- 1997
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In: Advanced Light Source. - California, USA : Ernest Orlando Lawrence Berkeley National Laboratory, University of California Berkeley. ; 65:2, s. 159-167
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Book chapter (pop. science, debate, etc.)
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