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Search: WFRF:(van Grinsven Bart)

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  • Siang Yeap, Weng, et al. (author)
  • Boron-Doped Diamond Functionalization by an Electrografting/Alkyne-Azide Click Chemistry Sequence
  • 2014
  • In: ChemElectroChem. - : Wiley. - 2196-0216. ; 1:7, s. 1145-1154
  • Journal article (peer-reviewed)abstract
    • A straightforward protocol for the covalent functionalization of boron-doped diamond electrodes with either ferrocene or single-stranded deoxyribonucleic acid (DNA) is reported. The functionalization method is based on a combination of diazonium salt electrografting and click chemistry. An azide-terminated organic layer is first electrografted onto the diamond surface by electrochemical reduction of 4-azidophenyldiazonium chloride. The azidophenyl-modified surface then reacts rapidly and efficiently with molecules bearing a terminal alkyne moiety by means of Cu-1-catalyzed alkyne-azide cycloaddition. Covalent attachment of ferrocene moieties was analyzed by X-ray photoelectron spectroscopy and cyclic voltammetry, whereas impedance spectroscopy was applied for the characterization of the immobilized DNA.
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Type of publication
journal article (1)
Type of content
peer-reviewed (1)
Author/Editor
Fahlman, Mats (1)
Liu, Xianjie (1)
Ameloot, Marcel (1)
Maes, Wouter (1)
Wagner, Patrick (1)
Haenen, Ken (1)
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Siang Yeap, Weng (1)
Sharif Murib, Mohamm ... (1)
Cuypers, Wim (1)
van Grinsven, Bart (1)
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University
Linköping University (1)
Language
English (1)
Research subject (UKÄ/SCB)
Natural sciences (1)
Year
2014 (1)

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