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1.
  • Seidel, M., et al. (author)
  • Multi-pass Cell Based Nonlinear Pulse Compression of Yb : YAG Pump-Probe Lasers at FLASH
  • 2023
  • In: X-Ray Free-Electron Lasers : Advances in Source Development and Instrumentation VI - Advances in Source Development and Instrumentation VI. - 0277-786X .- 1996-756X. - 9781510662827 ; 12581
  • Conference paper (peer-reviewed)abstract
    • The majority of user experiments at the high repetition-rate free electron laser (FEL) facility FLASH are of pump-probe type, combining the extreme ultraviolet (XUV) or soft x-ray radiation from the FEL with ultrashort pulses generated by optical lasers. In this contribution, we demonstrate the advantages of using high-power Yb:YAG lasers with subsequent nonlinear pulse compression stages based on multi-pass cells (MPC). The approach enables the combination of hundreds of kHz to MHz repetition-rates, hundreds of watts of average powers and excellent intensity stabilities. We present the characteristics of the MPC-based pump-probe laser at the FLASH plane-grating beamlines. Furthermore, we report pulse compression to 8.2 fs pulse duration and the seeding of an optical parametric amplifier generating mid-IR radiation tunable from 1.4 µm to 16 µm.
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2.
  • Abrahamsson, Christoffer, et al. (author)
  • Scatter correction of transmission NIR spectra by photon migration data - Quantitative analysis of solids
  • 2005
  • In: Proceedings of SPIE - The International Society for Optical Engineering. - : SPIE. - 1996-756X .- 0277-786X. ; 6009, s. 60090-60090
  • Conference paper (peer-reviewed)abstract
    • The scope of this presentation is a new methodology to correct conventional NIR data for scattering effects. The technique aims at measuring the absorption coefficient of the samples rather than the total attenuation, measured by conventional NIR spectroscopy. The main advantage of this is that the absorption coefficient is independent of the path length of the light inside the sample, and therefore independent of the scattering effects. The measurements in this work were made using a novel system for time-resolved measurements, based on short light continuum pulses generated in an index-guided crystal fibre and a spectrometer-equipped streak camera. The system enables spectral recordings in the wavelength range 500 - 1200 nm with a spectral resolution of 5 nm and a temporal resolution of 30 ps. The evaluation scheme is based on modeling of light transport by diffusion theory, that provides an independent measure of the scattering properties of the samples, that later is used to correct conventional NIR data. This yields a clear advantage over other pre-processing techniques, where scattering effects are estimated and corrected for by using the shape of the measured spectrum only. PLS calibration models shows that, by using the proposed evaluation scheme, the predictive ability is improved by 50% as compared to models based on conventional NIR data. The method also makes it possible to predict the concentration of active substance in samples with physical properties different from those of the samples included in the calibration model.
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3.
  • Achilles, Silvio, et al. (author)
  • GPU-Accelerated Coupled Ptychographic Tomography
  • 2022
  • In: Developments in X-Ray Tomography XIV. - : SPIE. - 1996-756X .- 0277-786X. - 9781510654686 ; 12242
  • Conference paper (peer-reviewed)abstract
    • Scanning coherent X-ray microscopy (ptychography) has gained considerable interest during the last decade since the performance of this indirect imaging technique does not necessarily rely on the quality of the X-ray optics and, in principle, can achieve highest spatial resolution in X-ray imaging. The method can be easily extended to 3D by adding standard tomographic reconstruction schemes. However, the tomographic reconstruction is often applied in a subsequent step using a sequence of aligned ptychographic 2D projections. In this contribution, we outline current developments of a GPU-accelerated framework for direct 3D ptychography, coupling 2D ptychography and tomography. The program utilizes a custom GPU-accelerated framework for ptychography that offers three distinct ptychographic reconstruction algorithms. The tomographic reconstruction runs simultaneously and uses numerical routines of the ASTRA Toolbox. This parallel-computing approach results in a high performance increase considerably reducing the reconstruction time of 3D ptychographic datasets.
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4.
  • Adler, Alexandre, et al. (author)
  • Modelling ground pickup for microwave telescopes
  • 2022
  • In: Proceedings of SPIE, the International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. ; 12190
  • Journal article (peer-reviewed)abstract
    • Microwave telescopes require an ever-increasing control of experimental systematics in their quest to measure the Cosmic Microwave Background (CMB) to exquisite levels of precision. One important systematic for ground and balloon-borne experiments is ground pickup, where beam sidelobes detect the thermal emission of the much warmer ground while the main beam is scanning the sky. This generates scan-synchronous noise in experiment timestreams, which is difficult to filter out without also deleting some of the signal from the sky. Therefore, efficient modelling of pickup can help guide the design of experiments and of analysis pipelines. In this work, we present an extension to the BEAMCONV algorithm that enables us to generate time-ordered data (TOD) from beam-convolved sky and ground maps simultaneously. We simulate ground pickup for both a ground-based experiment and a telescope attached to a stratospheric balloon. Ground templates for the balloon experiment are obtained by re-projecting satellite maps of the Earth's microwave emission. 
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5.
  • Afanasiev, Sergey V., et al. (author)
  • Experimental apparatus to study crystal channeling in an external SPS beamline
  • 2007
  • In: Proceedings of SPIE, the International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. ; 6634
  • Journal article (peer-reviewed)abstract
    • For the new generation of high intensity hadronic machines as, for instance, LHC, halo collimation is a necessary issue for the accelerator to operate at the highest possible luminosity and to prevent the damage of superconductor magnets.1 We propose an experiment aimed to systematic study of the channeling phenomenology and of the newly observed "volume reflection" effect. This experiment will be performed for an external SPS beamline and will make use of a primary proton beam with 400 GeV/c momentum and very small (∼ 3 μrad) divergence. The advantage of a proposed experiment is precise tracking of particles that interacted with a crystal, so that to determine the single-pass efficiency for all the processes involved. For this purpose, a telescope equipped with high-resolution silicon microstrip detectors will be used. New generation silicon crystals and an extra-precise goniometer are mandatory issues. Main goal of the experiment is to get the precise information on channeling of relativistic particles and, ultimately, on the feasibility of such technique for halo collimation at LHC. In this contribution we review the status of the setting-up of experimental apparatus and its future development in sight of the planned run in September 2006.
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6.
  • Alexander, Naomi E., et al. (author)
  • IMAGINE project : A low cost, high performance, monolithic passive mm-wave imager front-end
  • 2012
  • In: Proceedings of SPIE - The International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. - 9780819492852
  • Conference paper (peer-reviewed)abstract
    • The FP7 Research for SME project IMAGINE - a low cost, high performance monolithic passive mm-wave imager front-end is described in this paper. The main innovation areas for the project are: i) the development of a 94 GHz radiometer chipset and matching circuits suitable for monolithic integration. The chipset consists of a W-band low noise amplifier, fabricated using the commercially available OMMIC D007IH GaAs mHEMT process, and a zero bias resonant interband tunneling diode, fabricated using a patented epi-layer structure that is lattice matched to the same D007IH process; ii) the development of a 94 GHz antenna adapted for low cost manufacturing methods with performance suitable for real-time imaging; iii) the development of a low cost liquid crystal polymer PCB build-up technology with performance suitable for the integration and assembly of a 94 GHz radiometer module; iv) the assembly of technology demonstrator modules. The results achieved in these areas are presented.
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7.
  • Alfredson, J. (author)
  • Individual differences in visual behaviour in simulated flight
  • 2002
  • In: Proceedings of SPIE, the International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. ; 4662, s. 494-502
  • Conference paper (other academic/artistic)abstract
    • Flying an aircraft is highly visually demanding. It is very important to map pilot visual behaviour, both for the purpose of evaluating the cockpit interface and to effectively integrate it with future adaptive interfaces and decision support systems. Pilots' visual behaviour was studied in two experiments. In the first experiment commercial aviation pilots were flying a commercial aviation scenario and eye point of gaze, and eye blinks were collected. In the second experiment military pilots were flying an air-to-air combat scenario and the visual behaviour was video recorded. In both of the experiments the results show individual differences in the pilots' visual behaviour. In the second experiment two different categories of eye blinks were found that might help explain the individual differences in visual behaviour. One category can be related to the systematic eye blinks found to occur when the eye point of gaze was changed between head-up/head-down and head-down/head-up. The other category could be related to other reasons, such as, mental workload or visual demands.
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8.
  • Andersen, Torben, et al. (author)
  • A new concept for large deformable mirrors for extremely large telescopes
  • 2006
  • In: Proceedings of the SPIE - The International Society for Optical Engineering. - : SPIE. - 1996-756X .- 0277-786X. ; 6272:1, s. 324-331
  • Conference paper (peer-reviewed)abstract
    • For extremely large telescopes, there is strong need for thin deformable mirrors in the 3-4 m class. So far, feasibility of such mirrors has not been demonstrated. Extrapolation from existing techniques suggests that the mirrors could be highly expensive. We give a progress report on a study of an approach for construction of large deformable mirrors with a moderate cost. We have developed low-cost actuators and deflection sensors that can absorb mounting tolerances in the millimeter range, and we have tested prototypes in the laboratory. Studies of control laws for mirrors with thousands of sensors and actuators are in good progress and simulations have been carried out. Manufacturing of thin, glass mirror blanks is being studied and first prototypes have been produced by a slumping technique. Development of polishing procedures for thin mirrors is in progress
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9.
  • Andersen, Torben, et al. (author)
  • A parallel integrated model of the Euro50
  • 2004
  • In: Proceedings of the SPIE - The International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. ; 5497:1, s. 251-265
  • Conference paper (peer-reviewed)abstract
    • The Euro50 is an astronomical extremely large telescope for optical and infrared wavelength with a 50 m primary mirror. The telescope will have an elaborate control system ("live optics") to correct for atmospheric and telescope aberrations. To study and predict performance of the complete telescope system, an integrated model combining the structural model of the telescope, optics models, the control systems, and the adaptive optics has been established. Wind is taken into account on the basis of wind tunnel measurements and computer fluid dynamics calculations. Atmospheric aberrations are included using a seven-layer atmosphere model. The integrated model is written in Matlab and is run on a cluster computer to achieve acceptable execution times. Dedicated ordinary differential equation solvers have been written and a special toolkit for communication between Matlab processes on different nodes of the cluster computer has been set up. Preliminary results from the complete integrated model, including adaptive optics, are shown
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10.
  • Andersen, Torben, et al. (author)
  • An Integrated Model of the European Extremely Large Telescope
  • 2008
  • In: MODELLING, SYSTEMS ENGINEERING, AND PROJECT MANAGEMENT FOR ASTRONOMY III. - : SPIE. - 1996-756X .- 0277-786X. ; 7017, s. 216-227
  • Conference paper (peer-reviewed)abstract
    • Integrated models including optics, structures, control systems, and disturbances are important design tools for Extremely Large Telescopes (ELTs). An integrated model has keen formulated for the European ELT and it includes telescope structure, main servos, primary mirror segment control system, wind, optics, wavefront sensor, deformable mirror, and an AO reconstructor and controller. There are three model phases: Initialization, execution of a solver to determine time responses, and post-processing. In near future, the model will be applied for performance studies and design trade-offs for the European ELT.
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11.
  • Andersen, Torben, et al. (author)
  • An integrated simulation model of the Euro50
  • 2002
  • In: Proceedings of SPIE - The International Society for Optical Engineering. - : SPIE. - 1996-756X .- 0277-786X. ; 4757, s. 84-92
  • Conference paper (peer-reviewed)abstract
    • The Euro50 is a proposed optical telescope with an equivalent aperture of 50 m. It will have a segmented primary mirror and full adaptive optics. To study the interaction of the telescope structure, the control system and the optics, an integrated simulation model has been formulated. The mechanical model is a modal version of an Ansys finite element model. The optics model is based on ray tracing and physical optics. The segments model takes the alignment servos and the segment dynamics into account. Wind variation over the primary mirror is included. Segment control system modeling is in progress. First results clearly demonstrate that a good enclosure is needed to protect the telescope well against wind. The results also suggest that the segment alignment system must have a bandwidth well above the lowest eigenfrequencies of the telescope.
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12.
  • Andersen, Torben, et al. (author)
  • Euro50
  • 2003
  • In: Proceedings of the SPIE - The International Society for Optical Engineering. - : SPIE. - 1996-756X .- 0277-786X. ; 5382:1, s. 169-182
  • Conference paper (peer-reviewed)abstract
    • The Euro50 is a telescope for optical and infrared wavelengths. It has an aspherical primary mirror with a size of 50 meters and 618 segments. The optical configuration is of Gregorian type and the secondary mirror is deformable for adaptive optics. Observations can take place in prime focus, Gregorian foci, and Nasmyth foci using additional relay mirrors. The telescope provides seeing limited observations, partial adaptive optics with ground layer correction, single conjugate adaptive optics and dual-conjugate adaptive optics. For prime focus observations, a clam-shell corrector with a doublet lens is used. The primary mirror segments can be polished using the precessions polishing technique. "Live Optics" denotes the joint segment alignment system, secondary mirror control system, adaptive optics and main axes servos. An overview is given of the live optics architecture, including feedback from wavefront sensors for natural and laser guide stars, and from primary mirror segment edge sensors. A straw man concept of the laser guide star system using sum-frequency YAG lasers is presented together with a solution to the laser guide star perspective elongation problem. The structural design involves a large steel structure and a tripod of carbon fiber reinforced polymer to support the secondary mirror. Integrated models have been set up to simulate telescope performance. Results show that an enclosure is needed to protect the telescope against wind during observations. The enclosure is very large box-shaped steel structure
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13.
  • Andersen, Torben, et al. (author)
  • Integrated modeling of the Euro50
  • 2003
  • In: Proceedings of the SPIE - The International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. ; 5382:1, s. 366-378
  • Conference paper (peer-reviewed)abstract
    • The Euro50 is a proposed 50 m optical and infrared telescope. It will have thousands of control loops to keep the optics aligned under influence of wind, gravity and thermal loads. Cross-disciplinary integrated modeling is used to study the overall performance of the Euro50. A sub-model of the mechanical structure originates from finite element modeling. The optical performance is determined using ray tracing, both non-linear and linearized. The primary mirror segment alignment control system is modeled with the 618 segments taken as rigid bodies. Adaptive optics is included using a layered model of the atmosphere and sub-models of the wavefront sensor, reconstructor and controller. The deformable mirror is, so far, described by a simple influence function and a second order dynamical transfer function but more detailed work is in progress. The model has been implemented using Matlab/Simulink on individual computers but it will shortly be implemented on a Beowulf cluster within a trusted network. Communication routines between Matlab on the cluster processors have been written and are being benchmarked. Representative results from the simulations are shown
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14.
  • Andersen, Torben, et al. (author)
  • Status of the Euro50 project
  • 2004
  • In: Proceedings of the SPIE - The International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. ; 5489:1, s. 407-416
  • Conference paper (peer-reviewed)abstract
    • The Euro50 is an extremely large telescope for optical and infrared wavelength with a 50 m primary mirror. It has a segmented, aspherical primary mirror and an aspherical, deformable secondary in a Gregorian layout. A tentative conceptual design exists and has been documented in a study report. Recent activities have concentrated on the science case for extremely large telescopes in the 50 m class and on identification of potential technical "show stoppers". The science case investigation has identified four fields of particular interest. The studies of critical technical issues have concentrated on atmospheric dispersion effects for high-resolution adaptive optics for extremely large telescopes, and on the influence of wind and other disturbances on wavefront control. Wind load on the telescope, the primary mirror and the enclosure has been studied using wind tunnel measurements and computational fluid dynamics. The impact of wind on the total system has been investigated using an integrated model that includes the telescope structure, the primary mirror segment alignment system, the secondary mirror alignment system, and single conjugate adaptive optics using the deformable secondary mirror. The first, tentative results show that wind disturbances may be significant and that the task of correcting for wind residuals may be at least as large for the adaptive optics system as that of correcting for atmospheric aberrations. The results suggest that use of extremely large telescopes for observations of earth-like planets around nearby stars may imply a considerable challenge
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15.
  • Andersson-Engels, Stefan, et al. (author)
  • Integrated system for interstitial photodynamic therapy
  • 2003
  • In: Proceedings of SPIE - The International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. ; 5142, s. 42-49
  • Conference paper (peer-reviewed)abstract
    • A novel photodynamic therapy system based on interstitial illumination using multiple fibres is under development. The aim with this system is to enable treatment of large tumour volumes and also to utilise real-time measurements to allow on-line dosimetry. Important dosimetric parameters to measure are light fluence rate, sensitizer fluorescence intensity and local blood oxygenation. A construction which allows all functions to be readily performed with a single system is presented. We believe that interstitial PDT utilising this technique may be attractive in many clinical situations.
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16.
  • Andersson-Engels, Stefan, et al. (author)
  • Integrated system for interstitial photodynamic therapy
  • 2002
  • In: Advanced Optical Devices, Technologies, and Medical Applications. - : SPIE. - 0277-786X .- 1996-756X. ; 5123, s. 293-302
  • Conference paper (peer-reviewed)abstract
    • To develop PDT beyond treatment of thin superficial tumours, to also be an efficient treatment alternative for deeply located and/or thick tumours, a system based on interstitial illumination using multiple fibres has been developed. Conditions that could benefit from such a treatment modality are for instance malignant brain tumours and tumours in the oral cavity. In interstitial PDT one needs to use multiple fibres for light delivery in order to allow treatments of tumours larger than a few millimetres in diameter. Our system consists of a laser light source, a beam-splitting system dividing the light into three or six output fibres and a custom-made dosimetry programme. The concept is then to use these fibres not only for delivering the treatment light but also to measure parameters of interest for the treatment outcome. The fluence rate of the light emitted by each fibre is measured at the positions of the other fibre tips. From these results the light dose at all positions could be recalculated. Changes in optical properties as well as bleaching and concentration of the photosensitizer during the treatment could be monitored and compensated for in the dosimetry. Tumours have been treated both in experimental studies and in patients with thick superficial Basal Cell Carcinomas. Almost all treated skin lesions responded with complete response.
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17.
  • Andersson, I., et al. (author)
  • Increasing spatial resolution by using an image sequence
  • 2001
  • In: Proceedings of SPIE, the International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. ; 4380, s. 542-551
  • Conference paper (other academic/artistic)abstract
    • In this paper we present two methods for increasing the spatial resolution of images using image sequences where all frames contain the same static scene with unknown shifts. Because of the subpixel shifts, aliased frequencies appear in a slightly different way in all images, making it possibly to reconstruct frequencies above the Nyqvist frequency, thus improving the resolution. To this end, we estimate parameters in the affine transform relating the images to each other from the sequence. To show the applicability of the algorithms, many experiments have been carried out mainly using image sequences captured by a TV-camera and not only using synthetic image sequences. The results from one TV-camera sequence are presented in this report. Measurements of PSF and MTF have been carried out and the results show that we can increase the spatial resolution by almost a factor of two. This technique can be used for target identification/recognition as well as for visualization. The second method (interpolation) is possible to implement in real time.
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18.
  • Andersson, Mikael, et al. (author)
  • Modelling and Design of Admission Control Mechanisms for Web Servers using Non-linear Control Theory
  • 2003
  • In: Performance and control of next-generation communication networks : [ITCom's Conference on Performance and Control of Next-Generation Communication Networks] ; 9 - 10 September 2003, Orlando, Florida, USA (SPIE proceedings series ; vol. 5244). - : SPIE. - 1996-756X .- 0277-786X. - 0819451274 ; 5244:1, s. 53-64
  • Conference paper (peer-reviewed)abstract
    • Web sites are exposed to high rates of incoming requests. Since web sites are sensitive to overload, admission control mechanisms are often implemented. The purpose of such a mechanism is to prevent requests from entering the web server during high loads. This paper presents how admission control mechanisms can be designed and implemented with a combination of queueing theory and control theory. Since web servers behave non-linear and stochastic, queueing theory can be used for web server modelling. However, there are no mathematical tools in queueing theory to use when designing admission control mechanisms. Instead, control theory contains the needed mathematical tools. By analysing queueing systems with control theoretic methods, good admission control mechanisms can be designed for web server systems. In this paper we model an Apache web server as a GI/G/1-system. Then, we use control theory to design a PI-controller, commonly used in automatic control, for the web server. In the paper we describe the design of the controller and also how itcan be implemented in a real system. The controller has been implemented and tested together with the Apache web server. The server was placed in a laboratory network together with a traffic generator which was used to represent client requests. Measurements in the laboratory setup show how robust the implemented controller is, and how it correspond to the results from the theoretical analysis.
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19.
  • Andreani, P., et al. (author)
  • The European ALMA Regional Centre: a model of user support
  • 2014
  • In: Proceedings of SPIE - The International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. - 9780819496171 ; 9149, s. Art. no. 91490Y-
  • Conference paper (peer-reviewed)abstract
    • The ALMA Regional Centres (ARCs) form the interface between the ALMA observatory and the user community from the proposal preparation stage to the delivery of data and their subsequent analysis. The ARCs provide critical services to both the ALMA operations in Chile and to the user community. These services were split by the ALMA project into core and additional services. The core services are financed by the ALMA operations budget and are critical to the successful operation of ALMA. They are contractual obligations and must be delivered to the ALMA project. The additional services are not funded by the ALMA project and are not contractual obligations, but are critical to achieve ALMA full scientific potential. A distributed network of ARC nodes (with ESO being the central ARC) has been set up throughout Europe at the following seven locations: Bologna, Bonn-Cologne, Grenoble, Leiden, Manchester, Ondrejov, Onsala. These ARC nodes are working together with the central node at ESO and provide both core and additional services to the ALMA user community. This paper presents the European ARC, and how it operates in Europe to support the ALMA community. This model, although complex in nature, is turning into a very successful one, providing a service to the scientific community that has been so far highly appreciated. The ARC could become a reference support model in an age where very large collaborations are required to build large facilities, and support is needed for geographically and culturally diverse communities.
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20.
  • Andrekson, Peter, 1960, et al. (author)
  • Nonlinearity-based all-optical sampling of ultrahigh-bandwidth optical signals
  • 2004
  • In: Proceedings of SPIE - The International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. ; 5596, s. 319-331
  • Conference paper (peer-reviewed)abstract
    • We demonstrate an all-optical waveform sampling system with simultaneous sub-mW optical signal sensitivity (20 dB SNR) and sub-picosecond temporal resolution over more than 60 nm optical bandwidth. The optical sampling was implemented by four-wave mixing in a 10 m highly nonlinear fiber using a sampling pulse source with a sampling pulse peak power of only 16 W. The sampling performance was evaluated in terms of sensitivity, temporal resolution and optical bandwidth with respect to fiber length, sampling pulse source wavelength offset from the zero-dispersion wavelength of the highly nonlinear fiber, sampling pulse peak power and walk-off due to chromatic dispersion. We also present a summary of the available methods to achieve polarization-independent optical sampling.
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21.
  • Antosiewicz, Tomasz, 1981, et al. (author)
  • Bi-metal coated aperture SNOM probes
  • 2011
  • In: Proceedings of SPIE - The International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. - 9780819486608 ; 8070
  • Conference paper (peer-reviewed)abstract
    • Aperture probes of scanning near-field optical microscopes (SNOM) offer resolution which is limited by a sum of the aperture diameter at the tip of a tapered waveguide probe and twice the skin depth in metal used for coating. An increase of resolution requires a decrease of the aperture diameter. However, due to low energy throughput of such probes aperture diameters usually are larger than 50 nm. A groove structure at fiber core-metal coating interface for photon-to-plasmon conversion enhances the energy throughput 5-fold for Al coated probes and 30-fold for Au coated probes due to lower losses in the metal. However, gold coated probes have lower resolution, first due to light coupling from the core to plasmons at the outside of the metal coating, and second due to the skin depth being larger than for Al. Here we report on the impact of a metal bilayer of constant thickness for coating aperture SNOM probes. The purpose of the bilayer of two metals of which the outer one is aluminum and the inner is a noble metal is to assure low losses, hence larger transmission. Using body-of-revolution finite-difference time-domain simulations we analyze properties of probes without corrugations to measure the impact of using a metal bilayer and choose an optimum bi-metal configuration. Additionally we investigate how this type of metalization works in the case of grooved probes.
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22.
  • Antosiewicz, Tomasz, 1981, et al. (author)
  • Magnetic probe for material characterization at optical frequencies
  • 2011
  • In: Proceedings of SPIE - The International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. - 9780819486608 ; 8070
  • Conference paper (peer-reviewed)abstract
    • Rapid development of novel, functional metamaterials made of purely dielectric, plasmonic, or composite structures which exhibit tunable optical frequency magnetic responses creates a need for new measurement techniques. We propose a method of actively measuring magnetic responses, i.e. magnetic dispersion, of such metamaterials within a wide range of optical frequencies with a single probe by exciting individual elementary cells within a larger matrix. The probe is made of a tapered optical fiber with a radially corrugated metal coating. It concentrates azimuthally polarized light in the near-field below the apex into a subwavelength size focus of the longitudinal magnetic field component. An incident azimuthally polarized beam propagates in the core until it reaches the metal stripes of constant angular width running parallel to the axis. For a broad frequency range light-to-plasmon coupling is assured as the lattice constant changes with the radius due to constant angular width. Bound plasmonic modes in slits between the metal stripes propagate toward the apex where circular currents in stripes and displacement currents in slits generate a strong longitudinal magnetic field. The energy density of the longitudinal magnetic component in the vicinity of the axis is much stronger than that of all the other components combined, what allows for pure magnetic excitation of magnetic resonances rather than by the electric field. The scattered signal is then measured in the far-field and analyzed.
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23.
  • Antosiewicz, Tomasz, 1981, et al. (author)
  • On the optical properties of plasmonic glasses
  • 2014
  • In: Proceedings of SPIE - The International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. - 9781628415568 ; 9441, s. Art. no. 94411G-
  • Conference paper (peer-reviewed)abstract
    • We report on the optical properties of plasmonic glasses which are metal-dielectric composites composed of metallic inclusions in a host dielectric medium. The investigated structures are of quasi-random nature, described by the pair correlation function, featuring a minimum center-to-center distance between metallic inclusions and long range randomness. Plasmonic glasses exhibiting short-range order only may be fabricated using bottom-up, self-assembly methods and have been utilized in a number of applications such as plasmonic sensing or plasmon-enhanced solar harvesting, and may be also employed for certain non-linear applications. It is therefore important to quantify their properties. Using theoretical methods we investigate optical of 1D, 2D, and 3D structures composed of amorphous distributions of metallic spheres. It is shown, that the response of the constituent element, i.e. The single sphere localized surface plasmon resonance, is modified by the scattered fields of the other spheres in such a way that its peak position, peak amplitude, and full-width at half-maximum exhibit damped oscillations. The oscillation amplitude is set by the particle density and for the peak position may vary by up to 0.3 eV in the optical regime. Using a modified coupled dipole approach we calculate the effective (average) polarizability of plasmonic glasses and discuss their spectra as a function of the dimensionality, angle of incidence and polarization, and the minimum center-to-center distance. The analytical model is complemented and validated by T-Matrix calculations of the optical cross-sections of amorphous arrays of metallic spheres obtained using a modification of the Random Sequential Adsorption algorithm for lines, surfaces, and volumes.
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24.
  • Antosiewicz, Tomasz, 1981, et al. (author)
  • Optical activity of catalytic elements of hetero-metallic nanostructures
  • 2015
  • In: Proceedings of SPIE - The International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. - 9781628416237 ; 9502
  • Conference paper (peer-reviewed)abstract
    • Interaction of light with metals in the form of surface plasmons is used in a wide range of applications in which the scattering decay channel is important. The absorption channel is usually thought of as unwanted and detrimental to the efficiency of the device. This is true in many applications, however, recent studies have shown that maximization of the decay channel of surface plasmons has potentially significant uses. One of these is the creation of electron-hole pairs or hot electrons which can be used for e.g. catalysis. Here, we study the optical properties of hetero-metallic nanostructures that enhance light interaction with the catalytic elements of the nanostructures. A hybridized LSPR that matches the spectral characteristic of the light source is excited. This LSPR through coupling between the plasmonic elements maximizes light absorption in the catalytic part of the nanostructure. Numerically calculated visible light absorption in the catalytic nanoparticles is enhanced 12-fold for large catalytic disks and by more 30 for small nanoparticles on the order of 5 nm. In experiments we measure a sizable increase in the absorption cross section when small palladium nanoparticles are coupled to a large silver resonator. These observations suggest that heterometallic nanostructures can enhance catalytic reaction rates.
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25.
  • Antosiewicz, Tomasz, 1981, et al. (author)
  • Sensing (un)binding events via surface plasmons: Effects of resonator geometry
  • 2016
  • In: Proceedings of SPIE - The International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. - 9781510601291 ; 9884
  • Conference paper (peer-reviewed)abstract
    • The resonance conditions of localized surface plasmon resonances (LSPRs) can be perturbed in any number ways making plasmon nanoresonators viable tools in detection of e.g. phase changes, pH, gasses, and single molecules. Precise measurement via LSPR of molecular concentrations hinge on the ability to confidently count the number of molecules attached to a metal resonator and ideally to track binding and unbinding events in real-time. These two requirements make it necessary to rigorously quantify relations between the number of bound molecules and response of plasmonic sensors. This endeavor is hindered on the one hand by a spatially varying response of a given plasmonic nanosensor. On the other hand movement of molecules is determined by stochastic effects (Brownian motion) as well as deterministic flow, if present, in microfluidic channels. The combination of molecular dynamics and the electromagnetic response of the LSPR yield an uncertainty which is little understood and whose effect is often disregarded in quantitative sensing experiments. Using a combination of electromagnetic finite-difference time-domain (FDTD) calculations of the plasmon resonance peak shift of various metal nanosensors (disk, cone, rod, dimer) and stochastic diffusion-reaction simulations of biomolecular interactions on a sensor surface we clarify the interplay between position dependent binding probability and inhomogeneous sensitivity distribution. We show, how the statistical characteristics of the total signal upon molecular binding are determined. The proposed methodology is, in general, applicable to any sensor and any transduction mechanism, although the specifics of implementation will vary depending on circumstances. In this work we focus on elucidating how the interplay between electromagnetic and stochastic effects impacts the feasibility of employing particular shapes of plasmonic sensors for real-time monitoring of individual binding reactions or sensing low concentrations - which characteristics make a given sensor optimal for a given task. We also address the issue of how particular illumination conditions affect the level of uncertainty of the measured signal upon molecular binding.
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