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  • Trost, Fabian, et al. (author)
  • Imaging via Correlation of X-Ray Fluorescence Photons
  • 2023
  • In: Physical Review Letters. - : American Physical Society. - 0031-9007 .- 1079-7114. ; 130:17
  • Journal article (peer-reviewed)abstract
    • We demonstrate that x-ray fluorescence emission, which cannot maintain a stationary interference pattern, can be used to obtain images of structures by recording photon-photon correlations in the manner of the stellar intensity interferometry of Hanbury Brown and Twiss. This is achieved utilizing femtosecondduration pulses of a hard x-ray free-electron laser to generate the emission in exposures comparable to the coherence time of the fluorescence. Iterative phasing of the photon correlation map generated a model-free real-space image of the structure of the emitters. Since fluorescence can dominate coherent scattering, this may enable imaging uncrystallised macromolecules.
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