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1.	Burt, Michael, et al. (author) Coulomb-explosion imaging of concurrent CH2BrI photodissociation dynamics 2017 In: Physical Review A: covering atomic, molecular, and optical physics and quantum information. - 2469-9926 .- 2469-9934. ; 96:4 Journal article (peer-reviewed)abstract The dynamics following laser-induced molecular photodissociation of gas-phase CH2BrI at 271.6 nm were investigated by time-resolved Coulomb-explosion imaging using intense near-IR femtosecond laser pulses. The observed delay-dependent photofragment momenta reveal that CH2BrI undergoes C-I cleavage, depositing 65.6% of the available energy into internal product states, and that absorption of a second UV photon breaks the C-Br bond of C(H)2Br. Simulations confirm that this mechanism is consistent with previous data recorded at 248 nm, demonstrating the sensitivity of Coulomb-explosion imaging as a real-time probe of chemical dynamics.

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Author/Editor: Underwood, Jonathan (1); Burt, Michael (1); Amini, Kasra (1); Boll, Rebecca (1); Kockert, Hansjochen (1); Olshin, Pavel K. (1); show more...; Bari, Sadia (1); Bomme, Cedric (1); Brausse, Felix (1); de Miranda, Barbara ... (1); Duesterer, Stefan (1); Erk, Benjamin (1); Geleoc, Marie (1); Geneaux, Romain (1); Gentleman, Alexander ... (1); Goldsztejn, Gildas (1); Guillemin, Renaud (1); Holland, David M. P. (1); Ismail, Iyas (1); Johnsson, Per (1); Journel, Loic (1); Kuepper, Jochen (1); Lahl, Jan (1); Lee, Jason W. L. (1); Maclot, Sylvain (1); Mackenzie, Stuart R. (1); Manschwetus, Bastian (1); Mereshchenko, Andrey ... (1); Palaudoux, Jerome (1); Piancastelli, Maria ... (1); Penent, Francis (1); Rompotis, Dimitrios (1); Rouzee, Arnaud (1); Ruchon, Thierry (1); Rudenko, Artem (1); Savelyev, Evgeny (1); Simon, Marc (1); Schirmel, Nora (1); Stapelfeldt, Henrik (1); Techert, Simone (1); Travnikova, Oksana (1); Trippel, Sebastian (1); Vallance, Claire (1); Wiese, Joss (1); Ziaee, Farzaneh (1); Brouard, Mark (1); Marchenko, Tatiana (1); Rolles, Daniel (1); Treusch, Rolf (1); Mueller, Erland (1); show less...

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