| 1. |
- Foltynowicz, Aleksandra, 1981-
(author)
-
Fiber-laser-based noise-immune cavity-enhanced optical heterodyne molecular spectrometry
- 2009
-
Doctoral thesis (other academic/artistic)abstract
- Noise-immune cavity-enhanced optical heterodyne molecular spectro-metry (NICE-OHMS) is one of the most sensitive laser-based absorption techniques. The high sensitivity of NICE-OHMS is obtained by a unique combination of cavity enhancement (for increased interaction length with a sample) with frequency modulation spectrometry (for reduction of noise). Moreover, sub-Doppler detection is possible due to the presence of high intensity counter-propagating waves inside an external resonator, which provides an excellent spectral selectivity. The high sensitivity and selectivity make NICE-OHMS particularly suitable for trace gas detection. Despite this, the technique has so far not been often used for practical applications due to its technical complexity, originating primarily from the requirement of an active stabilization of the laser frequency to a cavity mode.The main aim of the work presented in this thesis has been to develop a simpler and more robust NICE-OHMS instrumentation without compro-mising the high sensitivity and selectivity of the technique. A compact NICE-OHMS setup based on a fiber laser and a fiber-coupled electro-optic modulator has been constructed. The main advantage of the fiber laser is its narrow free-running linewidth, which significantly simplifies the frequency stabilization procedure. It has been demonstrated, using acetylene and carbon dioxide as pilot species, that the system is capable of detecting relative absorption down to 3 × 10-9 on a Doppler-broadened transition, and sub-Doppler optical phase shift down to 1.6 × 10-10, the latter corresponding to a detection limit of 1 × 10-12 atm of C2H2. Moreover, the potential of dual frequency modulation dispersion spectrometry (DFM-DS), an integral part of NICE-OHMS, for concentration measurements has been assessed.This thesis contributes also to the theoretical description of Doppler-broadened and sub-Doppler NICE-OHMS signals, as well as DFM-DS signals. It has been shown that the concentration of an analyte can be deduced from a Doppler-broadened NICE-OHMS signal detected at an arbitrary and unknown detection phase, provided that a fit of the theoretical lineshape to the experimental data is performed. The influence of optical saturation on Doppler-broadened NICE-OHMS signals has been described theoretically and demonstrated experimentally. In particular, it has been shown that the Doppler-broadened dispersion signal is unaffected by optical saturation in the Doppler limit. An expression for the sub-Doppler optical phase shift, valid for high degrees of saturation, has been derived and verified experimentally up to degrees of saturation of 100.
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| 2. |
- Buckland, Philip I., 1973-, et al.
(author)
-
The Strategic Environmental Archaeology Database : a resource for international, multiproxy and transdisciplinary studies of environmental and climatic change
- 2015
-
Conference paper (peer-reviewed)abstract
- Climate and environmental change are global challenges which require global data and infrastructure to investigate. These challenges also require a multi-proxy approach, integrating evidence from Quaternary science and archaeology with information from studies on modern ecology and physical processes among other disciplines. The Strategic Environmental Archaeology Database (SEAD http://www.sead.se) is a Swedish based international research e-infrastructure for storing, managing, analysing and disseminating palaeoenvironmental data from an almost unlimited number of analysis methods. The system currently makes available raw data from over 1500 sites (>5300 datasets) and the analysis of Quaternary fossil insects, plant macrofossils, pollen, geochemistry and sediment physical properties, dendrochronology and wood anatomy, ceramic geochemistry and bones, along with numerous dating methods. This capacity will be expanded in the near future to include isotopes, multi-spectral and archaeo-metalurgical data. SEAD also includes expandable climate and environment calibration datasets, a complete bibliography and extensive metadata and services for linking these data to other resources. All data is available as Open Access through http://qsead.sead.se and downloadable software. SEAD is maintained and managed at the Environmental Archaeology Lab and HUMlab at Umea University, Sweden. Development and data ingestion is progressing in cooperation with The Laboratory for Ceramic Research and the National Laboratory for Wood Anatomy and Dendrochronology at Lund University, Sweden, the Archaeological Research Laboratory, Stockholm University, the Geoarchaeological Laboratory, Swedish National Historical Museums Agency and several international partners and research projects. Current plans include expanding its capacity to serve as a data source for any system and integration with the Swedish National Heritage Board's information systems. SEAD is partnered with the Neotoma palaeoecology database (http://www.neotomadb.org) and a new initiative for building cyberinfrastructure for transdisciplinary research and visualization of the long-term human ecodynamics of the North Atlantic funded by the National Science Foundation (NSF).
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| 3. |
- Fredenberg, Erik, 1979-
(author)
-
Spectral Mammography with X-Ray Optics and a Photon-Counting Detector
- 2009
-
Doctoral thesis (other academic/artistic)abstract
- Early detection is vital to successfully treating breast cancer, and mammography screening is the most efficient and wide-spread method to reach this goal. Imaging low-contrast targets, while minimizing the radiation exposure to a large population is, however, a major challenge. Optimizing the image quality per unit radiation dose is therefore essential. In this thesis, two optimization schemes with respect to x-ray photon energy have been investigated: filtering the incident spectrum with refractive x-ray optics (spectral shaping), and utilizing the transmitted spectrum with energy-resolved photon-counting detectors (spectral imaging). Two types of x-ray lenses were experimentally characterized, and modeled using ray tracing, field propagation, and geometrical optics. Spectral shaping reduced dose approximately 20% compared to an absorption-filtered reference system with the same signal-to-noise ratio, scan time, and spatial resolution. In addition, a focusing pre-object collimator based on the same type of optics reduced divergence of the radiation and improved photon economy by about 50%. A photon-counting silicon detector was investigated in terms of energy resolution and its feasibility for spectral imaging. Contrast-enhanced tumor imaging with a system based on the detector was characterized and optimized with a model that took anatomical noise into account. Improvement in an ideal-observer detectability index by a factor of 2 to 8 over that obtained by conventional absorption imaging was found for different levels of anatomical noise and breast density. Increased conspicuity was confirmed by experiment. Further, the model was extended to include imaging of unenhanced lesions. Detectability of microcalcifications increased no more than a few percent, whereas the ability to detect large tumors might improve on the order of 50% despite the low attenuation difference between glandular and cancerous tissue. It is clear that inclusion of anatomical noise and imaging task in spectral optimization may yield completely different results than an analysis based solely on quantum noise.
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| 4. |
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| 5. |
- Volkov, Mikhail, 1982-
(author)
-
Solving the quantum scattering problem for systems of two and three charged particles
- 2011
-
Doctoral thesis (other academic/artistic)abstract
- A rigorous formalism for solving the Coulomb scattering problem is presented in this thesis. The approach is based on splitting the interaction potential into a finite-range part and a long-range tail part. In this representation the scattering problem can be reformulated to one which is suitable for applying exterior complex scaling. The scaled problem has zero boundary conditions at infinity and can be implemented numerically for finding scattering amplitudes. The systems under consideration may consist of two or three charged particles. The technique presented in this thesis is first developed for the case of a two body single channel Coulomb scattering problem. The method is mathematically validated for the partial wave formulation of the scattering problem. Integral and local representations for the partial wave scattering amplitudes have been derived. The partial wave results are summed up to obtain the scattering amplitude for the three dimensional scattering problem. The approach is generalized to allow the two body multichannel scattering problem to be solved. The theoretical results are illustrated with numerical calculations for a number of models. Finally, the potential splitting technique is further developed and validated for the three body Coulomb scattering problem. It is shown that only a part of the total interaction potential should be split to obtain the inhomogeneous equation required such that the method of exterior complex scaling can be applied. The final six-dimensional equation is reduced to a system of three dimensional equations using the full angular momentum representation. Such a system can be numerically implemented using the existing full angular momentum complex exterior scaling code (FAMCES). The code has been updated to solve the three body scattering problem.
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| 6. |
- Yakovlev, S. L., et al.
(author)
-
The impact of sharp screening on the Coulomb scattering problem in three dimensions
- 2010
-
In: Journal of Physics A. - Bristol, UK : IOP Publishing Ltd.. - 0305-4470 .- 1361-6447. ; 43:24, s. 245302-
-
Journal article (peer-reviewed)abstract
- The scattering problem for two particles interacting via theCoulomb potential isexamined for the case where the potential has a sharp cut-off at some distance.The problem is solved for two complementary situations, firstly, when theinterior part of the Coulomb potential is left in the Hamiltonian and, secondly,when the long-range tail is considered as the potential. The partial wave resultsare summed up to obtain the wavefunction in three dimensions. It is shownthat in the domains where the wavefunction is expected to be proportionalto the known solutions, the proportionality is given by an operator actingon the angular part of the wavefunction. The explicit representation for thisoperator is obtained in the basis of Legendre polynomials. We proposed adriven Schr¨odinger equation including an inhomogeneous term of the finiterange with purely outgoing asymptotics for its solution in the case of thethree-dimensional scattering problem with long-range potentials.
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| 7. |
- Grabowski, Alexander, 1993
(author)
-
VCSEL Equivalent Circuits and Silicon Photonics Integration
- 2022
-
Doctoral thesis (other academic/artistic)abstract
- The vertical-cavity surface-emitting laser (VCSEL) is a light source of great importance for numerous industrial and consumer products. The main application areas are datacom and sensing. The datacom industry uses GaAs-based VCSELs for optical interconnects, the short-reach fiber optical communication links used to transfer large amounts of data at high rates between units within data centers and supercomputers. In the area of sensing, VCSELs are largely used in consumer products such as smart phones (e.g. face ID and camera auto focus), computer mice, and automobiles (e.g. gesture recognition and LIDAR for autonomous driving). In this work, an advanced physics-based equivalent circuit model for datacom VCSELs has been developed. The model lends itself to co-design and co-optimization with driver and receiver ICs, thereby enabling higher data rate transceivers with bandwidth limited VCSELs and photodiodes. The model also facilitates an understanding of how each physical process within the VCSEL affects the VCSEL static and dynamic performance. It has been applied to study the impact of carrier transport and capture on VCSEL dynamics. The work also includes micro-transfer-printing of GaAs-based single-mode VCSELs on silicon nitride photonic integrated circuits (PICs). Such PICs are increasingly used for e.g. compact and highly functional bio-photonic sensors. Transfer printing of VCSELs enables the much-needed on-PIC integration of power efficient light sources. The bottom-emitting VCSELs are printed above grating couplers on the PIC and optical feedback is used to control the polarization for efficient coupling to the silicon nitride waveguide. Wavelength tuning, as required by the bio-sensing application, is achieved by direct current modulation.
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| 8. |
- Hartman, Henrik, et al.
(author)
-
The FERRUM project : experimental and theoretical transition rates of forbidden [Sc II] lines and radiative lifetimes of metastable ScII levels
- 2008
-
In: Astronomy and Astrophysics. - : EDP Sciences. - 0004-6361 .- 1432-0746. ; 480:2, s. 575-580
-
Journal article (peer-reviewed)abstract
- Context. In many plasmas, long-lived metastable atomic levels are depopulated by collisions (quenched) before they decay radiatively. In low-density regions, however, the low collision rate may allow depopulation by electric dipole (E1) forbidden radiative transitions, so-called forbidden lines (mainly M1 and E2 transitions). If the atomic transition data are known, these lines are indicators of physical plasma conditions and used for abundance determination. Aims. Transition rates can be derived by combining relative intensities between the decay channels, so-called branching fractions (BFs), and the radiative lifetime of the common upper level. We use this approach for forbidden [Sc II] lines, along with new calculations. Methods. Neither BFs for forbidden lines, nor lifetimes of metastable levels, are easily measured in a laboratory. Therefore, astrophysical BFs measured in Space Telescope Imaging Spectrograph (STIS) spectra of the strontium filament of Eta Carinae are combined with lifetime measurements using a laser probing technique on a stored ion-beam (CRYRING facility, MSL, Stockholm). These quantities are used to derive the absolute transition rates (A-values). New theoretical transition rates and lifetimes are calulated using the CIV3 code. Results. We report experimental lifetimes of the Sc II levels 3d(2) a(3)P(0,1,2) with lifetimes 1.28, 1.42, and 1.24 s, respectively, and transition rates for lines from these levels down to 3d4s a(3)D in the region 8270-8390 angstrom. These are the most important forbidden [Sc II] transitions. New calculations for lines and metastable lifetimes are also presented, and are in good agreement with the experimental data.
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| 9. |
- Sjöqvist, Erik, et al.
(author)
-
Conceptual aspects of geometric quantum computation
- 2016
-
In: Quantum Information Processing. - : Springer Science and Business Media LLC. - 1570-0755 .- 1573-1332. ; 15:10, s. 3995-4011
-
Journal article (peer-reviewed)abstract
- Geometric quantum computation is the idea that geometric phases can be used to implement quantum gates, i.e., the basic elements of the Boolean network that forms a quantum computer. Although originally thought to be limited to adiabatic evolution, controlled by slowly changing parameters, this form of quantum computation can as well be realized at high speed by using nonadiabatic schemes. Recent advances in quantum gate technology have allowed for experimental demonstrations of different types of geometric gates in adiabatic and nonadiabatic evolution. Here, we address some conceptual issues that arise in the realizations of geometric gates. We examine the appearance of dynamical phases in quantum evolution and point out that not all dynamical phases need to be compensated for in geometric quantum computation. We delineate the relation between Abelian and non-Abelian geometric gates, and find an explicit physical example where the two types of gates coincide. We identify differencies and similarities between adiabatic and nonadiabatic realizations of quantum computation based on non-Abelian geometric phases.
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| 10. |
- Errando-Herranz, Carlos, 1989-, et al.
(author)
-
Dynamic dispersion tuning of silicon photonicwaveguides by microelectromechanical actuation
- 2017
-
In: Optics InfoBase Conference Papers. - : Optical Society of America. - 9781943580279
-
Conference paper (peer-reviewed)abstract
- Efficient nonlinear silicon photonics rely on phase-matching through finewaveguide dispersion engineering. We experimentally demonstrate dynamic dispersion tuningof 800 ps/nm/km in a silicon waveguide ring resonator, by using microelectromechanicalactuation of an adjacent suspended waveguide rim.
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| 11. |
- Larson, Jonas, et al.
(author)
-
Spin-orbit-coupled Bose-Einstein condensate in a tilted optical lattice
- 2010
-
In: Physical Review A. Atomic, Molecular, and Optical Physics. - : APS. - 1050-2947 .- 1094-1622. ; 82:4, s. 043620-
-
Journal article (peer-reviewed)abstract
- Bloch oscillations appear for a particle in a weakly tilted periodic potential. The intrinsic spin Hall effect is an outcome of a spin-orbit coupling. We demonstrate that both of these phenomena can be realized simultaneously in a gas of weakly interacting ultracold atoms exposed to a tilted optical lattice and to a set of spatially dependent light fields inducing an effective spin-orbit coupling. It is found that both the spin Hall and the Bloch oscillation effects may coexist, showing, however, a strong correlation between the two. These correlations are manifested as a transverse spin current oscillating in-phase with the Bloch oscillations. On top of the oscillations originating from the periodicity of the model, a trembling motion is found which is believed to be atomic Zitterbewegung. It is argued that the damping of these Zitterbewegung oscillations may to a large extent be prevented in the present setup considering a periodic optical lattice potential.
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| 12. |
- Piscitelli, Francesco, et al.
(author)
-
Neutron reflectometry on highly absorbing films and its application to (B4C)-B-10-based neutron detectors
- 2016
-
In: Royal Society of London. Proceedings A. Mathematical, Physical and Engineering Sciences. - : The Royal Society. - 1364-5021 .- 1471-2946. ; 472:2185
-
Journal article (peer-reviewed)abstract
- Neutron reflectometry is a powerful tool used for studies of surfaces and interfaces. The absorption in the typical studied materials is neglected and this technique is limited only to the reflectivity measurement. For strongly absorbing nuclei, the absorption can be directly measured by using the neutron-induced fluorescence technique which exploits the prompt particle emission of absorbing isotopes. This technique is emerging from soft matter and biology where highly absorbing nuclei, in very small quantities, are used as a label for buried layers. Nowadays, the importance of absorbing layers is rapidly increasing, partially because of their application in neutron detection; a field that has become more active also due to the He-3-shortage. We extend the neutron-induced fluorescence technique to the study of layers of highly absorbing materials, in particular (B4C)-B-10. The theory of neutron reflectometry is a commonly studied topic; however, when a strong absorption is present the subtle relationship between the reflection and the absorption of neutrons is not widely known. The theory for a general stack of absorbing layers has been developed and compared to measurements. We also report on the requirements that a (B4C)-B-10 layer must fulfil in order to be employed as a converter in neutron detection.
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| 13. |
- Ulfat, I., et al.
(author)
-
Effects of nonuniform Mn distribution in (Ga,Mn)As
- 2014
-
In: Physical Review B Condensed Matter. - : American Physical Society. - 0163-1829 .- 1095-3795. ; 89:4, s. art no 045312-
-
Journal article (peer-reviewed)abstract
- Resonant in situ photoemission from Mn 3d states in Ga(1−x)MnxAs is reported for Mn concentrations down to the very dilute level of 0.1%. Concentration-dependent spectral features are analyzed on the basis of first-principles calculations for systems with selected impurity positions as well as for random alloys. Effects of direct Mn-Mn interaction are found for concentrations as low as 2.5%, and are ascribed to statistical (nonuniform) distribution of Mn atoms.
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| 14. |
- Ogier, Robin, 1987, et al.
(author)
-
Near-Complete Photon Spin Selectivity in a Metasurface of Anisotropic Plasmonic Antennas
- 2015
-
In: Physical Review X. - : American Physical Society. - 2160-3308. ; 5:4
-
Journal article (peer-reviewed)abstract
- Simple chiroptically active metamaterials are difficult to realize in practice but could pave the way for a range of important applications, such as sensitive optical biosensors, asymmetric catalysis, and novel polarization manipulation devices. We show that a metasurface based on a random arrangement of anisotropic but aligned gold nanoparticles can exhibit an almost perfect selectivity towards incident photon spin for evanescent excitation with visible to near-infrared light. The experimentally attained reflection contrast between left- and right-handed circularly polarized light peaks at similar to 90%, in excellent agreement with analytical theory. These results are important for the development of future photonic and plasmonic polarization-based technologies.
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| 15. |
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| 16. |
- Tidström, Jonas, et al.
(author)
-
Open system effects on slow light and electromagnetically induced transparency
- 2011
-
In: Journal of Physics B. - : IOP Publishing. - 0953-4075 .- 1361-6455. ; 44:13, s. 135501-
-
Journal article (peer-reviewed)abstract
- The coherence properties of a three-level $\Lambda$-system influenced by a Markovian environment are analyzed. A coherence vector formalism is used and a vector form of the Lindblad equation is derived. Together with decay channels from the upper state, open system channels acting on the subspace of the two lower states are investigated, i.e., depolarization, dephasing, and amplitude damping channels. We derive an analytic expression for the coherence vector and the concomitant optical susceptibility, and analyze how the different channels influence the optical response. This response depends non-trivially on the type of open system interaction present, and even gain can be obtained. We also present a geometrical visualization of the coherence vector as an aid to understand the system response.
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| 17. |
- Monsel, Juliette, 1994, et al.
(author)
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Dissipative and dispersive cavity optomechanics with a frequency-dependent mirror
- 2024
-
In: Physical Review A. - 2469-9934 .- 2469-9926. ; 109:4
-
Journal article (peer-reviewed)abstract
- An optomechanical microcavity can considerably enhance the interaction between light and mechanical motion by confining light to a subwavelength volume. However, this comes at the cost of an increased optical loss rate. Therefore, microcavity-based optomechanical systems are placed in the unresolved-sideband regime, preventing sideband-based ground-state cooling. A pathway to reduce optical loss in such systems is to engineer the cavity mirrors, i.e., the optical modes that interact with the mechanical resonator. In our work, we analyze such an optomechanical system, whereby one of the mirrors is strongly frequency dependent, i.e., a suspended Fano mirror. This optomechanical system consists of two optical modes that couple to the motion of the suspended Fano mirror. We formulate a quantum-coupled-mode description that includes both the standard dispersive optomechanical coupling as well as dissipative coupling. We solve the Langevin equations of the system dynamics in the linear regime showing that ground-state cooling from room temperature can be achieved even if the cavity is per se not in the resolved-sideband regime, but achieves effective sideband resolution through strong-optical-mode coupling. Importantly, we find that the cavity output spectrum needs to be properly analyzed with respect to the effective laser detuning to infer the phonon occupation of the mechanical resonator. Our work also predicts how to reach the regime of nonlinear quantum optomechanics in a Fano-based microcavity by engineering the properties of the Fano mirror.
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| 18. |
- Wersäll, Martin, 1985, et al.
(author)
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Directional Nanoplasmonic Antennas for Self-Referenced Refractometric Molecular Analysis
- 2014
-
In: Journal of Physical Chemistry C. - : American Chemical Society (ACS). - 1932-7447 .- 1932-7455. ; 118:36, s. 21075-21080
-
Journal article (peer-reviewed)abstract
- Localized surface-plasmon resonance (LSPR) sensors are typically based on tracing resonance peak shifts that precisely follow changes in the local refractive index. Such measurements usually require a spectrometer, a stable light source, and an accurate LSPR position tracing technique. As a simple but efficient alternative, we investigated a self-referenced single-wavelength sensing scheme based on angle-dependent and highly directional radiation patterns originating from a monolayer of asymmetric gold nanodimers. We found that one could easily trace a model biotinneutravidin recognition reaction as well as minute bulk refractive index changes, by measuring the intensity ratio between the light scattered in two different directions with respect to the dimers. The refractometric resolution of the methodology was estimated to be on the order of Delta n approximate to 10(-5) RIU. These results may be particularly useful for label-free biosensing applications that require a combination of simple and cost-effective optical readout with a reasonable sensitivity.
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| 19. |
- Le Breton, Michael, 1986, et al.
(author)
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Chlorine oxidation of VOCs at a semi-rural site in Beijing: significant chlorine liberation from ClNO2 and subsequent gas- and particle-phase Cl-VOC production
- 2018
-
In: Atmospheric Chemistry and Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 18:17, s. 13013-13030:18, s. 13013-13030
-
Journal article (peer-reviewed)abstract
- Nitryl chloride (ClNO2) accumulation at night acts as a significant reservoir for active chlorine and impacts the following day's photochemistry when the chlorine atom is liberated at sunrise. Here, we report simultaneous measurements of N2O5 and a suite of inorganic halogens including ClNO2 and reactions of chloride with volatile organic compounds (Cl-VOCs) in the gas and particle phases utilising the Filter Inlet for Gas and AEROsols time-of-flight chemical ionisation mass spectrometer (FIGAERO-ToF-CIMS) during an intensive measurement campaign 40 km northwest of Beijing in May and June 2016. A maximum mixing ratio of 2900 ppt of ClNO2 was observed with a mean campaign nighttime mixing ratio of 487 ppt, appearing to have an anthropogenic source supported by correlation with SO2, CO and benzene, which often persisted at high levels after sunrise until midday. This was attributed to such high mixing ratios persisting after numerous e-folding times of the photolytic lifetime enabling the chlorine atom production to reach 2.3 x 10(5) molecules cm(-3) from ClNO2 alone, peaking at 09:30 LT and up to 8.4 x 10(5) molecules cm(-3) when including the supporting inorganic halogen measurements. Cl-VOCs were observed in the particle and gas phases for the first time at high time resolution and illustrate how the iodide ToF-CIMS can detect unique markers of chlorine atom chemistry in ambient air from both biogenic and anthropogenic sources. Their presence and abundance can be explained via time series of their measured and steady-state calculated precursors, enabling the assessment of competing OH and chlorine atom oxidation via measurements of products from both of these mechanisms and their relative contribution to secondary organic aerosol (SOA) formation.
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| 20. |
- Ekström, Maria, 1988
(author)
-
Quantum acoustics with propagating phonons
- 2020
-
Doctoral thesis (other academic/artistic)abstract
- Surface acoustic waves (SAWs) are mechanical vibrations that propagate on the surface of solids while dissipating little power, consequently enabling them to propagate freely over long distances. The speed and wavelength of SAWs are reduced a five order of magnitude compared to when light is used as a carrier at gigahertz frequencies. The unique properties of SAWs combined with the possibility to let them interact with artificial atoms, discovered and shown for the very first time in appended Paper I of this thesis, open up for exploration of new regimes of quantum physics. The appended Paper II is a book chapter providing an overview of many of the new areas of research, as well as going into depth of the method and significance of the results ofthe appended Paper I. The essential interaction between artificial atoms and SAWs was further investigated by using Autler-Townes splitting to achieve fast control of the interactions. The appended Paper IV, shows a transmitted field extinction of 80 %, and provides proof of concept for a SAW router in the quantum regime. In addition, due to the artificial atom's highly frequency dependent coupling to SAWs, electromagnetically induced transparency (EIT) could be observed in the appended Paper V. Furthermore, the EIT region was distinguished from the Autler-Townes splitting region by a threshold in the applied power. The results produce parallel findings to quantum optics, but are perhaps best described as part of a different field, quantum acoustics. Among the many possible areas of research emerging as an outcome of this work, a variety of potential quantum experiments would benefit greatly from a higher conversion efficiency between electric signals and SAWs. Due to this, focus was put on improving this conversion efficiency by studying superconducting unidirectional transducers (UDTs), making use of advances in classical SAW devices. The appended Paper III shows that 99.4~\% of the acoustic power can be focused in a desired direction and that the conversion between electric signals and SAWs is greatly improved by using UDTs, thereby eliminating the largest source of loss of symmetric inter-digital transducers. There is, however, a trade-off between conversion efficiency and bandwidth. This finding allows tailoring of quantum experiments based on SAWs that may pave the way towards measuring quantum sound.
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| 21. |
- Ghorbani, Ramin, 1981-
(author)
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Real-time breath gas analysis of carbon monoxide : laser-based detection and pulmonary gas exchange modeling
- 2018
-
Doctoral thesis (other academic/artistic)abstract
- Breath gas analysis is a promising approach for non-invasive medical diagnostics and physiological monitoring. Real-time, breath-cycle resolved biomarker detection facilitates data interpretation and has the potential to improve the diagnostic value of breath tests as exhalation profiles carry spatiotemporal information about biomarker origin and gas exchange in the respiratory tract. This thesis presents and scrutinizes a novel methodology for the analysis of real-time breath data, where single-exhalation profiles are simulated using a pulmonary gas exchange model and least-squares fitted to measured expirograms to extract airway and alveolar contributions and diffusing capacities. The methodology is demonstrated on exhaled breath carbon monoxide (eCO), a candidate biomarker for oxidative stress and respiratory diseases. The thesis mainly covers (1) the construction of a compact optical sensor based on tunable diode laser absorption spectroscopy (TDLAS) in the mid-infrared region (4.7 μm) for selective and precise real-time detection of CO in breath and ambient air (detection limit 9 ± 5 ppb at 0.1 s), (2) the design of an advanced online breath sampling system, (3) the implementation of a trumpet model with axial diffusion (TMAD) to simulate the CO gas exchange, and (4) the application of extended eCO analysis in clinical studies to establish the healthy non-smoker baseline of the eCO parameters and to study the response to CO and wood smoke exposure. It is shown that the TMAD adequately describes the gas exchange during systemic CO elimination for different breathing patterns, and that there is no difference between eCO parameters from mouth- and nose exhalations. Expirogram shape and eCO parameters exhibit a dependence on the exhalation flow rate, but for a given breathing maneuverer, the parameters lie in a narrow range. Airway CO is close to and correlates with ambient air CO, indicating negligible airway production in the healthy population. The alveolar diffusing capacity is independent of endogenous CO, even after exposure to elevated exogenous CO, and could be used to assess lung diffusion abnormalities. Compared to CO exposure, no clear additional effect of exposure to wood smoke particles on eCO is observed. The discrimination between endogenous and exogenous CO sources remains a challenge.
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| 22. |
- Lestinsky, M., et al.
(author)
-
Physics book: CRYRING@ESR
- 2016
-
In: European Physical Journal: Special Topics. - : Springer Science and Business Media LLC. - 1951-6401 .- 1951-6355. ; 225:5, s. 797-882
-
Research review (peer-reviewed)abstract
- The exploration of the unique properties of stored and cooled beams of highly-charged ions as provided by heavy-ion storage rings has opened novel and fascinating research opportunities in the realm of atomic and nuclear physics research. Since the late 1980s, pioneering work has been performed at the CRYRING at Stockholm (Abrahamsson et al. 1993) and at the Test Storage Ring (TSR) at Heidelberg (Baumann et al. 1988). For the heaviest ions in the highest charge-states, a real quantum jump was achieved in the early 1990s by the commissioning of the Experimental Storage Ring (ESR) at GSI Helmholtzzentrum für Schwerionenforschung (GSI) in Darmstadt (Franzke 1987) where challenging experiments on the electron dynamics in the strong field regime as well as nuclear physics studies on exotic nuclei and at the borderline to atomic physics were performed. Meanwhile also at Lanzhou a heavy-ion storage ring has been taken in operation, exploiting the unique research opportunities in particular for medium-heavy ions and exotic nuclei (Xia et al. 2002).
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| 23. |
- Thiele, Illia, 1989, et al.
(author)
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Electron Beam Driven Generation of Frequency-Tunable Isolated Relativistic Subcycle Pulses
- 2019
-
In: Physical Review Letters. - 0031-9007 .- 1079-7114. ; 122
-
Journal article (peer-reviewed)abstract
- © 2019 American Physical Society. We propose a novel scheme for frequency-tunable subcycle electromagnetic pulse generation. To this end a pump electron beam is injected into an electromagnetic seed pulse as the latter is reflected by a mirror. The electron beam is shown to be able to amplify the field of the seed pulse while upshifting its central frequency and reducing its number of cycles. We demonstrate the amplification by means of 1D and 2D particle-in-cell simulations. In order to explain and optimize the process, a model based on fluid theory is proposed. We estimate that using currently available electron beams and terahertz pulse sources, our scheme is able to produce millijoule-strong midinfrared subcycle pulses.
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| 24. |
- Adesso, Gerardo, et al.
(author)
-
Optical implementation and entanglement distribution in Gaussian valence bond states
- 2007
-
In: Optics and Spectroscopy. - 0030-400X .- 1562-6911. ; 103:2, s. 178-186
-
Journal article (peer-reviewed)abstract
- We study Gaussian valence bond states of continuous variable systems, obtained as the outputs of projection operations from an ancillary space of M infinitely entangled bonds connecting neighboring sites, applied at each of $N$ sites of an harmonic chain. The entanglement distribution in Gaussian valence bond states can be controlled by varying the input amount of entanglement engineered in a (2M+1)-mode Gaussian state known as the building block, which is isomorphic to the projector applied at a given site. We show how this mechanism can be interpreted in terms of multiple entanglement swapping from the chain of ancillary bonds, through the building blocks. We provide optical schemes to produce bisymmetric three-mode Gaussian building blocks (which correspond to a single bond, M=1), and study the entanglement structure in the output Gaussian valence bond states. The usefulness of such states for quantum communication protocols with continuous variables, like telecloning and teleportation networks, is finally discussed.
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| 25. |
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| 26. |
- Bertilson, Michael, 1979-
(author)
-
Laboratory soft x-ray microscopy and tomography
- 2011
-
Doctoral thesis (other academic/artistic)abstract
- Soft x-ray microscopy in the water-window (λ = 2.28 nm – 4.36 nm) is based on zone-plate optics and allows high-resolution imaging of, e.g., cells and soils in their natural or near-natural environment. Three-dimensional imaging is provided via tomographic techniques, soft x-ray cryo tomography. However, soft x-ray microscopes with such capabilities have been based on large-scale synchrotron x‑ray facilities, thereby limiting their accessibility for a wider scientific community. This Thesis describes the development of the Stockholm laboratory soft x-ray microscope to three-dimensional cryo tomography and to new optics-based contrast mechanisms. The microscope relies on a methanol or nitrogen liquid-jet laser-plasma source, normal-incidence multilayer or zone-plate condenser optics, in-house fabricated zone-plate objectives, and allows operation at two wavelengths in the water-window, λ = 2.48 nm and λ = 2.48 nm. With the implementation of a new state-of-the-art normal-incidence multilayer condenser for operation at λ = 2.48 nm and a tiltable cryogenic sample stage the microscope now allows imaging of dry, wet or cryo-fixed samples. This arrangement was used for the first demonstration of laboratory soft x-ray cryo microscopy and tomography. The performance of the microscope has been demonstrated in a number of experiments described in this Thesis, including, tomographic imaging with a resolution of 140 nm, cryo microscopy and tomography of various cells and parasites, and for studies of aqueous soils and clays. The Thesis also describes the development and implementation of single-element differential-interference and Zernike phase-contrast zone-plate objectives. The enhanced contrast provided by these optics reduce exposure times or lowers the dose in samples and are of major importance for harder x-ray microscopy. The implementation of a high-resolution 50 nm compound zone-plate objective for sub-25-nm resolution imaging is also described. All experiments are supported by extensive numerical modelling for improved understanding of partially coherent image formation and stray light in soft x-ray microscopes. The models are useful tools for studying effects of zone plate optics or optical design of the microscope on image formation and quantitative accuracy in soft x-ray tomography.
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| 27. |
- Cavar, Elizabeta, et al.
(author)
-
A single h-BN layer on Pt(111)
- 2008
-
In: Surface Science. - : Elsevier BV. - 0039-6028 .- 1879-2758. ; 602:9, s. 1722-1726
-
Journal article (peer-reviewed)abstract
- The structure and formation of an ultrathin hexagonal boron nitride (h-BN) film on Pt(111) has been studied by a combination of scanning tunneling microscopy, low energy electron diffraction, low energy electron microscopy, X-ray absorption and high resolution core level spectroscopy. The study shows that a single boron nitride layer is formed on Pt(111), resulting in a coincidence structure. High resolution scanning tunneling microscopy (STM) images of the h-BN ultrathin film display only one of the atomic species in the unit cell. Probing the boron and nitrogen related local density of states by near edge X-ray absorption fine structure measurements we conclude that the nitrogen sublattice is visible in STM images. The growth of the single hexagonal boron nitride layer by vapourized borazine in the pressure range of 1 x 10(-6)-1 x 10(-8) at 800 degrees C is further studied by low energy electron microscopy, and reveals that the number of nucleation sites and the perfection of the growth is strongly pressure dependent. A model for the single, hexagonal, boron nitride layer on Pt(111) is proposed.
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| 28. |
- Ericsson, Marie, et al.
(author)
-
Measurement of geometric phase for mixed states using single photon interferometry
- 2005
-
In: Physical Review Letters. - 0031-9007 .- 1079-7114. ; 94:5, s. 050401-
-
Journal article (peer-reviewed)abstract
- Geometric phase may enable inherently fault-tolerant quantum computation. However, due to potential decoherence effects, it is important to understand how such phases arise for {\it mixed} input states. We report the first experiment to measure mixed-state geometric phases in optics, using a Mach-Zehnder interferometer, and polarization mixed states that are produced in two different ways: decohering pure states with birefringent elements; and producing a nonmaximally entangled state of two photons and tracing over one of them, a form of remote state preparation.
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| 29. |
- Gel'mukhanov, Faris, et al.
(author)
-
Doppler effects in resonant x-ray Raman scattering
- 1998
-
In: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 57:4, s. 2511-2526
-
Journal article (peer-reviewed)abstract
- Theory for Doppler effects in resonant x-ray Raman scattering (RXS) is presented. It is shown that the "electron" Doppler effect is important in nonradiative RXS for decay transitions between continuum nuclear states lying above the dissociation threshold, and that the averaging of the RXS cross section over molecular orientations can lead to strong non-lorentzian broadenings of the atomiclike resonances. The Doppler effect is found to give a unique possibility to distinguish dissociating identical atoms, because different peaks correspond to atoms with opposite Doppler shifts. Spectral features of the atomiclike profile are predicted and analyzed. Strong oscillations of the RXS cross section will occur as a consequence of the interference of the Auger electrons. Due to the Doppler effect and the interference, the atomiclike profile can be associated with supernarrow spectral features, the width of which goes below the lifetime broadening and is practically independent of the spectral distribution of the incident radiation. As another consequence of the oscillations and strong anisotropy caused by the interference, we predict parity selection rules for Auger decay transitions in both bound and dissociative systems. The corresponding experiments can be realized by measurements of resonant Auger of surface adsorbed molecules and for molecules by the electron-ion coincidence technique.
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| 30. |
- Magnuson, Martin, et al.
(author)
-
Competition between decay and dissociation of core-excited carbonyl sulfide studied by x-ray scattering
- 1999
-
In: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 59:6, s. 4281-4287
-
Journal article (peer-reviewed)abstract
- We show evidence of dissociation during resonant inelastic soft x-ray scattering Carbon and oxygen K-shell and sulfur L-shell resonant and nonresonant x-ray emission spectra were measured using monochromatic synchrotron radiation for excitation and ionization. After sulfur L-2,L-3-->pi*, sigma* excitation, atomic lines are observed in the emission spectra as a consequence of competition between de-excitation and dissociation. In contrast thr carbon and oxygen spectra show weaker line-shape variations and no atomic Lines. The spectra are compared to results from ab initio calculations. The discussion of the dissociation paths is based on calculated potential energy surfaces and atomic transition energies.
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| 31. |
- Rippe, Lars
(author)
-
Quantum computing with naturally trapped sub-nanometre-spaced ions
- 2006
-
Doctoral thesis (other academic/artistic)abstract
- The main aim of this work, was to lay the foundations for the experimental realisation of a quantum mechanical controlled NOT gate in rare-earth-metal-ion-doped crystals. Small amounts of rare-earth elements, added during the growth of some inorganic crystals, will become substituted into the crystal lattice as trivalent ions. The trivalent rare-earth-metal ions between cerium, with atomic number 58, and ytterbium, with atomic number 70, have a partly filled 4f shell, which does not extend spatially outside the full 5s and 5p shells. The 4f vacancies make electronic inner shell transitions possible between spectroscopic 4f terms. Some of these optical transitions have coherence times of the order of milliseconds, when the crystals are cooled down to ~ 4 K. There are several reasons for these extraordinary coherence times, which are approximately 8 orders of magnitude greater than those typical for electronic transitions in solids. The most important one is the cage-like shield which the outer 5s and 5p shells provide for the 4f electrons. Furthermore, since these ions are naturally trapped inside the crystal lattice there is no Doppler broadening of the line-width. The coherence properties of these optical transitions is one of the features that makes these materials attractive for use as a solid-state platform for quantum computing, using these ions as qubits. Another appealing characteristic is the fact that different ions have different optical resonance frequencies, which means that ions belonging to different qubits, which only have nm separation, can still be addressed separately by using different laser frequencies. Since the inter-ion spacing is so small, it is possible to make two ions interact strongly, although they are well shielded, through a permanent dipole-dipole interaction. This interaction can be turned on and off by switching between two different ways of encoding the qubit, a most useful feature. When the qubit is represented as a superposition between two ground state hyperfine levels, the interaction is turned off. The interaction is turned on selectively by transferring this superposition to the optical transition with a pi-pulse, for the specific ions that are to interact. This thesis describes how peaks of ions, absorbing on a single transition, residing in spectral pits with no other ions, have been isolated. It is shown how these ions can be coherently transferred between hyperfine levels via the optically excited state, how the interaction between such peaks of ions representing qubits can be turned on and off, and how subgroups of ions with strong interaction can be distilled out. All the work described here has been performed using the ensemble approach. The ensemble approach will, however, be difficult to scale up to large numbers of qubits. A method employing a single ion in each qubit, using a specialised ion for readout, has therefore also been proposed. The rare-earth-metal-ion-based quantum computing experiments require a laser with coherence properties which at least match those of the material. To this end a frequency stabilisation system was developed for a dye laser. This system uses a transient spectral hole in a rare-earth-metal-ion-doped crystal, of the same kind that is used in the experiments, as frequency reference, and is to the authors knowledge the first demonstration of locking a dye laser to a spectral hole. This system provides a line-width of 1 kHz on a 10 microseconds timescale and a frequency drift below 1 kHz/s.
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| 32. |
- Salek, Pawel, et al.
(author)
-
Generalized Franck-Condon principle for resonant photoemission
- 1999
-
In: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 60:4, s. 2786-2791
-
Journal article (peer-reviewed)abstract
- A generalized Franck-Condon (GFC) principle for resonant x-ray Raman scattering and for resonant photoemission in particular is derived and numerically investigated. The GFC amplitudes differ from ordinary FC amplitudes by the presence of photon and photoelectron phase factors which describe the coupling-or interference-of the x-ray photons or Anger electrons with the nuclear motion. With the GFC amplitudes, a Kramers-Heisenberg relation is obtained for vibronic transitions that corrects the so-called lifetime-vibrational interference formula. For resonant photoemission in the soft-x-ray region involving typical bound potential surfaces, the generalization gives a contribution to the FC factors that can amount to 20%. For core excitation above the dissociation threshold, the GFC principle relates to Doppler effects on the ejected photoelectron both for the so-called "molecular'' and "atomic" bands. The role of the GFC principle in direct photoionization is briefly discussed.
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| 33. |
- Schuch, Reinhold, et al.
(author)
-
Guiding of highly charged ions through insulating nanocapillaries
- 2008
-
In: Canadian journal of physics (Print). - 0008-4204 .- 1208-6045. ; 86:1, s. 327-330
-
Journal article (peer-reviewed)abstract
- The guiding of highly charged ions through nanocapillaries in different insulating materials, such as polyethylene terephthalate, SiO2, and Al2O3 has been investigated by our group, using 7 keV Ne7+ ions. We find transmission of ions incident at angles larger than the angle given by the capillary aspect ratio in all these materials. The measured angular distributions, however, vary with the membrane material. In this report we compare the experimental findings with the different membranes.
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| 34. |
- Skog, Patrik, et al.
(author)
-
Evidence of Sequentially Formed Charge Patches Guiding Ions through Nanocapillaries
- 2008
-
In: Physical Review Letters. - 0031-9007 .- 1079-7114. ; 101:22, s. 223202-
-
Journal article (peer-reviewed)abstract
- We investigated the time evolution of the dynamically shifting distribution of 7 keV Ne7+ ions guided through nanocapillaries in SiO2. We present evidence for a small number of charge patches, formed sequentially in the charging-up process, guiding the ions. We show that the charge patches are distributed along the whole length of the capillaries and that they are maintained in the equilibrium state of transmission. The interpretations are supported by model calculations.
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| 35. |
- von Hofsten, Olof, 1982-
(author)
-
Phase-Contrast and High-Resolution Optics for X-Ray Microscopy
- 2010
-
Doctoral thesis (other academic/artistic)abstract
- X-ray microscopy is a well-established technique for nanoscale imaging. Zone plates are used as microscope objectives and provide high resolution, approaching 10 nm, currently limited by fabrication issues. This Thesis presents zone plate optics that achieve either high resolution or phase contrast in x-ray microscopy. The high-resolution optics use high orders of the zone plate, which alleviates the demands on fabrication, and the phase-contrast optics are single-element diffractive optical elements that produce contrast by Zernike or differential-interference contrast methods. The advantage of phase contrast in x-ray microscopy is shorter exposure times, and is crucial in the hard x-ray regime. Microscopy in the absorption‑contrast region of the water-window (2.34 - 4.37 nm) also benefits from these optics. The development of the optics for a laboratory soft x-ray microscope spans from theoretical and numerical analysis of coherence and stray light to experimental implementation and testing. The laboratory microscope uses laser-produced plasma-sources in the water-window and is unique in its design and performance. It will be shown that the laboratory microscope in its current form is a user-oriented and stable instrument, and has been used in a number of applications. The implementation of a cryogenic sample stage for tomographic imaging of biological samples in their natural environment has enabled applications in biology, and 3D x-ray microscopy of cells was performed for the first time with a laboratory instrument.
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| 36. |
- Zhang, Hongqiang, et al.
(author)
-
Dynamics of Guiding Highly Charged Ions through SiO2 Nanocapillaries
- 2010
-
In: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 82:052901
-
Journal article (peer-reviewed)abstract
- Time evolution of angular distributions of transmitted ions through SiO2 nanocapillaries wasmeasured under defined initial conditions: already charged, as well as fully dischargedcapillaries. We find distinct charge patterns and describe them quantitatively with the help of amodel calculation. This results in a pattern of a few number of charge patches, guiding ions inthe stationary state of transmission. For the already charged capillary membrane, we show a“memory effect” in the form of a double peak structure in the transmitted angulardistributions. The time evolution of these structures reflects charge relaxation andrearrangement of the charge patches. The re-arrangement of the charge patches is much fasterthan the discharge, suggesting that the charge relaxation inside the capillaries can be drivenby the incident charges, such as a Frenkel-Poole process.
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| 37. |
- Zhang, Hongqiang, 1980-
(author)
-
Guiding of highly charged ions through insulating nanocapillaries
- 2010
-
Doctoral thesis (other academic/artistic)abstract
- This thesis contains experimental work on guiding of highly charged ions through insulating nanocapillaries. We have studied the time evolution of angular distributions of transmitted ions under well defined initial conditions: already charged, as well as fully discharged nanocapillaries, by using a two-dimensional position sensitive Micro Channel Plate detector with a data acquisition system working in event mode. Time-dependent features in the ion-guiding properties have been found. For the initially discharged capillaries, a shift and broadening of transmitted angular distribution have been observed in the charge-up process. This is interpreted by the formation of charged patches downstream of the entrance patch. We have, with the help of a model calculation, quantitatively derived distinct charge patterns, resulting in the time evolution of the transmitted angular distributions. We show that all charge patches are maintained in the stationary state of transmission by the followed discharging and recharging measurements. For already charged nanocapillaries, a double peak structure in the angular distribution has been found, which is attributed to a memory effect and the re-arrangement of charge patches. When the tilt angle of the capillaries is changed, the existing charge patches from the previous tilt angle can affect the ion trajectories and the formation of new patches. The preliminary results of highly charged ions transmitted through muscovite mica capillaries of rhombic cross section are also presented in this thesis. We have shown the transmission profiles for various orientations of the rhombi. A rectangular shape of the transmission profile has been found. We have performed a simulation by considering the image force from the four sides of the rhombus. To our surprise, this effect gives an angular distribution that agrees well with the transmission profile obtained by the experiment.
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| 38. |
- Zhang, Hongqiang, et al.
(author)
-
Guiding of slow highly charged ions through insulating nano-capillaries
- 2009
-
In: Journal of Physics, Conference Series. - : IOP Publishing. - 1742-6588 .- 1742-6596. ; 163:1
-
Journal article (peer-reviewed)abstract
- The guiding of highly charged ions through SiO2 nano-capillaries has been investigated by our group, using 7 keV Ne7+-ions. We studied in particular the transmission of ions incident at angles greater than the angle given by the capillary aspect ratio as a function of charge incident on the capillary membrane. In this report we show the re-arrangement of charge patches inside the capillary by observing the evolution of the two-dimensional angular distributions of the transmitted ions.
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| 39. |
- Baggioli, Matteo, et al.
(author)
-
Holographic plasmon relaxation with and without broken translations
- 2019
-
In: Journal of High Energy Physics (JHEP). - : SPRINGER. - 1126-6708 .- 1029-8479. ; :9
-
Journal article (peer-reviewed)abstract
- We study the dynamics and the relaxation of bulk plasmons in strongly coupled and quantum critical systems using the holographic framework. We analyze the dispersion relation of the plasmonic modes in detail for an illustrative class of holographic bottom-up models. Comparing to a simple hydrodynamic formula, we entangle the complicated interplay between the three least damped modes and shed light on the underlying physical processes. Such as the dependence of the plasma frequency and the effective relaxation time in terms of the electromagnetic coupling, the charge and the temperature of the system. Introducing momentum dissipation, we then identify its additional contribution to the damping. Finally, we consider the spontaneous symmetry breaking (SSB) of translational invariance. Upon dialing the strength of the SSB, we observe an increase of the longitudinal sound speed controlled by the elastic moduli and a decrease in the plasma frequency of the gapped plasmon. We comment on the condensed matter interpretation of this mechanism.
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| 40. |
- Manzetti, Sergio, et al.
(author)
-
A Korteweg-DeVries type model for helical soliton solutions for quantum and continuum phenomena
- 2021
-
In: International Journal of Modern Physics C. - : World Scientific. - 0129-1831. ; 32:03
-
Journal article (peer-reviewed)abstract
- Quantum mechanical states are normally described by the Schrödinger equation, which generates real eigenvalues and quantizable solutions which form a basis for the estimation of quantum mechanical observables, such as momentum and kinetic energy. Studying transition in the realm of quantum physics and continuum physics is however more difficult and requires different models. We present here a new equation which bears similarities to the Korteweg–DeVries (KdV) equation and we generate a description of transitions in physics. We describe here the two- and three-dimensional form of the KdV like model dependent on the Plank constant ℏ and generate soliton solutions. The results suggest that transitions are represented by soliton solutions which arrange in a spiral-fashion. By helicity, we propose a conserved pattern of transition at all levels of physics, from quantum physics to macroscopic continuum physics.
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| 41. |
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| 42. |
- Niskanen, Johannes, et al.
(author)
-
Photoelectron angular distribution and linear magnetic dichroism in the 4p photoemission from Rb atoms
- 2010
-
In: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 81:1, s. 013406-
-
Journal article (peer-reviewed)abstract
- The angular distribution of photoelectrons and linear magnetic dichroism in the angular distribution for the 4p photoemission from Rb atoms in the ground state, oriented by laser pumping, were measured in the photon energy range from 50 to 100 eV. The experimental results are compared with the multiconfiguration Dirac-Fock (MCDF) calculations. We show that the zero-crossing of the dichroism as a function of energy is connected with the Cooper minimum in the cross section. This fact can be used for an accurate determination of the position of the Cooper minimum.
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| 43. |
- Sun, Yu-Ping, et al.
(author)
-
Propagation of a strong x-ray pulse : Pulse compression, stimulated Raman scattering, amplified spontaneous emission, lasing without inversion, and four-wave mixing
- 2010
-
In: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 81:1
-
Journal article (peer-reviewed)abstract
- We study the compression of strong x-ray pulses from x-ray free-electron lasers (XFELs) propagating through the resonant medium of atomic argon. The simulations are based on the three-level model with the frequency of the incident x-ray pulse tuned in the 2p(3/2)-4s resonance. The pulse propagation is accompanied by the self-seeded stimulated resonant Raman scattering (SRRS). The SRRS starts from two channels of amplified spontaneous emission (ASE), 4s-2p(3/2) and 3s-2p(3/2), which form the extensive ringing pattern and widen the power spectrum. The produced seed field triggers the Stokes ASE channel 3s-2p(3/2). The population inversion is quenched for longer propagation distances where the ASE is followed by the lasing without inversion (LWI), which amplifies the Stokes component. Both ASE and LWI reshape the input pulse: The compressed front part of the pulse (up to 100 as) is followed by the long tail of the ringing and beating between the pump and Stokes frequencies. The pump pulse also generates weaker Stokes and anti-Stokes fields caused by four-wave mixing. These four spectral bands have fine structures caused by the dynamical Stark effect. A slowdown of the XFEL pulse up to 78% of the speed of light in vacuum is found because of a large nonlinear refractive index.
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| 44. |
- Dahl, Ingolf, 1950
(author)
-
How to measure the Mueller matrix of liquid-crystal cells
- 2001
-
In: Meas. Sci. Technol.. - 0957-0233. ; 12, s. 1938-1948
-
Journal article (peer-reviewed)abstract
- The Mueller matrix is the transfer matrix in the Stokes algebra that describes the polarization of natural light. This matrix is very versatile for the task of characterizing the optical properties of liquid-crystal cells, since it can be used for comparison with theoretical calculations, the determination of material parameters and the modelling of the cell as an optical building block for technological use. We have constructed a Mueller-matrix spectrometer, with the ability to perform fast, dynamic measurements of the Mueller matrix of small areas of liquid-crystal cells throughout the visible range. To illustrate the potential of the instrument, dynamic measurements on a ferroelectric-liquid-crystal cell are presented and analysed. The optical measurements indicate that there is an asymmetry between the up and the down state, tilted smectic layers and polarization reversal initiated at the boundaries.
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| 45. |
- Tello Marmolejo, Javier, 1995, et al.
(author)
-
A water droplet as a toy atom
- 2022
-
In: Proceedings of SPIE - The International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. ; 12198
-
Conference paper (peer-reviewed)abstract
- Common atomic physics courses jump from the square and harmonic well potentials straight to the hydrogen atom. However, there is a missing link in between, the spherical well potential. Although it is included in some textbooks, the lack of an experimental backing means the problem quickly becomes mathematically complex. Here we have built an optical toy atom using the scattering of an optically levitated, evaporating water droplet. We find a greatly simplified Mie scattering spectrum composed of a series of evolving Fano resonances organized in a set of combs. The whole spectrum can be intuitively explained through an analogy to a quantum spherical well potential. This produces a model of an atom including ground and excited states, quantized angular momentum, and tunneling.
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| 46. |
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| 47. |
- Muralidhar, Shreyas, et al.
(author)
-
Femtosecond Laser Pulse Driven Caustic Spin Wave Beams
- 2021
-
In: Physical Review Letters. - : American Physical Society (APS). - 0031-9007 .- 1079-7114. ; 126:3
-
Journal article (peer-reviewed)abstract
- © 2021 authors. Controlling the directionality of spin waves is a key ingredient in wave-based computing methods such as magnonics. In this Letter, we demonstrate this particular aspect by using an all-optical pointlike source of continuous spin waves based on frequency comb rapid demagnetization. The emitted spin waves contain a range of k vectors and by detuning the applied magnetic field slightly off the ferromagnetic resonance (FMR), we observe X-shaped caustic spin wave patterns at 70° propagation angles as predicted by theory. When the harmonic of the light source approaches the FMR, the caustic pattern gives way to uniaxial spin wave propagation perpendicular to the in-plane component of the applied field. This field-controlled propagation pattern and directionality of optically emitted short-wavelength spin waves provide additional degrees of freedom when designing magnonic devices.
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| 48. |
- Grabowski, Alexander, 1993, et al.
(author)
-
Impact of Carrier Transport and Capture on VCSEL Dynamics
- 2023
-
In: IEEE Journal of Quantum Electronics. - 0018-9197 .- 1558-1713. ; 59:1, s. 1-6
-
Journal article (peer-reviewed)abstract
- Using a vertical-cavity surface-emitting laser (VCSEL) equivalent circuit model based on two carrier rate equations to include effects of carrier dynamics, we study the impact of carrier transport and capture on the small- and large-signal modulation response of high-speed VCSELs. The model also accounts for parasitics, current-induced self-heating, and gain compression. A variation of the effective capture time from 1 to 15 ps is found to have a large impact on the small-signal modulation response, with the 3 dB bandwidth decreasing from 40 to 15 GHz and the response transitioning from under-damped to over-damped. This is primarily due to the increasing low frequency parasitic-like roll-off with increasing effective capture time. A significant effect on the optical waveforms produced by the VCSEL under 56 Gbit/s on-off keying (OOK) non-return-to-zero (NRZ) and pulse-amplitude modulation 4 (PAM4) modulation is observed, with a short effective capture time leading to horizontal eye closure caused by timing jitter (TJ) and intersymbol interference (ISI) and a long effective capture time leading to vertical eye closure caused by long rise- and fall-times. However, for high modulation speed, a short effective capture time is needed and the photon lifetime should be set for clear eye opening. We also show the impact of the effective capture time on the output power vs current characteristics and map the dependence of internal temperature, carrier densities, carrier escape and leakage rates, and spontaneous recombination rates on current for different effective capture times.
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| 49. |
- Wild, W., et al.
(author)
-
Millimetron—a large Russian-European submillimeter space observatory
- 2009
-
In: Experimental Astronomy. - : Springer Science and Business Media LLC. - 0922-6435 .- 1572-9508. ; 23:1, s. 221-244
-
Journal article (peer-reviewed)abstract
- Millimetron is a Russian-led 12 m diameter submillimeter and far-infrared space observatory which is included in the Space Plan of the Russian Federation for launch around 2017. With its large collecting area and state-of-the-art receivers, it will enable unique science and allow at least one order of magnitude improvement with respect to the Herschel Space Observatory. Millimetron will be operated in two basic observing modes: as a single-dish observatory, and as an element of a ground-space very long baseline interferometry (VLBI) system. As single-dish, angular resolutions on the order of 3 to 12 arc sec will be achieved and spectral resolutions of up to a million employing heterodyne techniques. As VLBI antenna, the chosen elliptical orbit will provide extremely large VLBI baselines (beyond 300,000 km) resulting in micro-arc second angular resolution.
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| 50. |
- Hamberg, Mathias, et al.
(author)
-
Experimental studies of the dissociative recombination processes for the dimethyl ether ions CD3OCD2+ and (CD3)2OD
- 2010
-
In: Astronomy and Astrophysics. - : EDP Sciences. - 0004-6361 .- 1432-0746. ; 514, s. A83-
-
Journal article (peer-reviewed)abstract
- Aims: Determination of branching fractions, cross sections and thermal rate coefficients for the dissociative recombination of CD3OCD2+ (0-0.3 eV) and (CD3)2OD+ (0-0.2 eV) at the low relative kinetic energies encountered in the interstellar medium. Methods: The measurements were carried out using merged electron and ion beams at the CRYRING storage ring, Stockholm, Sweden. Results: For (CD3)2OD+ we have experimentally determined the branching fraction for ejection of a single hydrogen atom in the DR process to be maximally 7% whereas 49% of the reactions involve the break up of the COC chain into two heavy fragments and 44% ruptures both C-O bonds. The DR of CD3OCD2+ is dominated by fragmentation of the COC chain into two heavy fragments. The measured thermal rate constants and cross sections are k(T) =1.7 ± 0.5 × 10−6(T/300)−0.77±0.01 cm3s−1, σ= 1.2 ± 0.4 × 10−15(Ecm[eV])−1.27 ± 0.01 cm2 and k(T) = 1.7 ± 0.6 × 10−6(T/300)−0.70±0.02 cm3s−1,σ= 1.7 ± 0.6 × 10−15(Ecm[eV])−1.20±0.02 cm2 for CD3OCD2+ and (CD3)2OD+, respectively.
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