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  • Jakobsson, Mattias, et al. (author)
  • Hole mobility and transport mechanisms in lambda-DNA
  • 2009
  • In: Journal of Chemical Physics. - : AIP Publishing. - 0021-9606 .- 1089-7690. ; 131:15, s. 155102-
  • Journal article (peer-reviewed)abstract
    • We have performed a study of charge transport in lambda-DNA using a recently developed model based on Marcus theory and dynamic Monte Carlo simulations. The model accounts for charge delocalization over multiple adjacent identical nucleobases. Such delocalized states are found to act as traps for charge transport and therefore have a negative impact on the charge carrier (hole) mobility. Both the electric field and temperature dependence of the mobility in lambda-DNA is reported in this paper. Furthermore, the detailed information produced by the simulation allow us to plot the progress of a hole propagating through the DNA sequence and this is used to identify the bottlenecks that limits the charge transport process.
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Type of publication
journal article (1)
Type of content
peer-reviewed (1)
Author/Editor
Jakobsson, Mattias (1)
Stafström, Sven (1)
University
Linköping University (1)
Language
English (1)
Year
2009 (1)

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