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1.	Nookuea, Worrada, et al. (author) Comparison of Mass Transfer Models on Rate-Based Simulation of CO2 Absorption and Desorption Processes 2017 In: Proceedings of the 9th International Conference on Applied Energy. - : Elsevier. ; 142, s. 3747-3752 Conference paper (peer-reviewed)abstract The effective technology for capturing CO2 at the low concentration is chemical absorption, due to the high reactivity between CO2 and aqueous amine solutions. To capture CO2, the process involves complex reactive separations. The accurate calculation of hydrodynamic properties, and mass and energy transfer are of importance for the design of the absorber and desorber columns. This paper performs the rate-based simulations of CO2 absorption by Monoethanolamine in Aspen Plus. In the calculation of the mass transfer coefficients, different mass transfer models were implemented. In comparison with the desorber, the impacts of mass transfer models were more significant in the simulation of the absorber. For both columns, the impacts of the mass transfer models on the concentration profiles were more significant than those on the temperature profiles. For the absorber, the maximum deviations occur at the bottom of the column for both the concentration and the temperature profiles. Different from the absorber, for the desorber, the maximum deviations occur close to the top of the column.

Nookuea, Worrada, et al. (author)
Comparison of Mass Transfer Models on Rate-Based Simulation of CO2 Absorption and Desorption Processes
2017
In: Proceedings of the 9th International Conference on Applied Energy. - : Elsevier. ; 142, s. 3747-3752
Conference paper (peer-reviewed)abstract
- The effective technology for capturing CO2 at the low concentration is chemical absorption, due to the high reactivity between CO2 and aqueous amine solutions. To capture CO2, the process involves complex reactive separations. The accurate calculation of hydrodynamic properties, and mass and energy transfer are of importance for the design of the absorber and desorber columns. This paper performs the rate-based simulations of CO2 absorption by Monoethanolamine in Aspen Plus. In the calculation of the mass transfer coefficients, different mass transfer models were implemented. In comparison with the desorber, the impacts of mass transfer models were more significant in the simulation of the absorber. For both columns, the impacts of the mass transfer models on the concentration profiles were more significant than those on the temperature profiles. For the absorber, the maximum deviations occur at the bottom of the column for both the concentration and the temperature profiles. Different from the absorber, for the desorber, the maximum deviations occur close to the top of the column.

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