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  • Simon, M., et al. (author)
  • Femtosecond nuclear motion of HCl probed by resonant x-ray Raman scattering in the Cl 1s region
  • 2006
  • In: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 73:2, s. 020706(R)-
  • Journal article (peer-reviewed)abstract
    • Femtosecond dynamics are observed by resonant x-ray Raman scattering (RXS) after excitation along the dissociative Cl 1s -> 6 sigma(*) resonance of gas-phase HCl. The short core-hole lifetime results in a complete breakdown of the common nondispersive behavior of soft-x-ray transitions between parallel potentials. We evidence a general phenomenon of RXS in the hard-x-ray region: a complete quenching of vibrational broadening. This opens up a unique opportunity for superhigh resolution x-ray spectroscopy beyond vibrational and lifetime limitations.
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Type of publication
journal article (1)
Type of content
peer-reviewed (1)
Author/Editor
Ågren, Hans (1)
Simon, M. (1)
Salek, Pawel (1)
Gelmukhanov, Faris (1)
Guillemin, R. (1)
Journel, L. (1)
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Stolte, W. C. (1)
Lindle, D. W. (1)
Carniato, S. (1)
Minkov, Ivaylo (1)
Taieb, R. (1)
Hudson, A. C. (1)
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University
Royal Institute of Technology (1)
Language
English (1)
Research subject (UKÄ/SCB)
Natural sciences (1)
Year
2006 (1)

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