2. |
- Kimberg, Victor, et al.
(author)
-
Stimulated X-ray Raman scattering : a critical assessment of the building block of nonlinear X-ray spectroscopy
- 2016
-
In: Faraday discussions. - : Royal Society of Chemistry. - 1359-6640 .- 1364-5498.
-
Journal article (peer-reviewed)abstract
- With the invention of femtosecond X-ray free-electron lasers (XFELs), studies of light-induced chemical reaction dynamics and structural dynamics reach a new era, allowing for time-resolved X-ray diffraction and spectroscopy. To ultimately probe coherent electron and nuclear dynamics on their natural time and length scales, coherent nonlinear X-ray spectroscopy schemes have been proposed. In this contribution, we want to critically assess the experimental realisation of nonlinear X-ray spectroscopy at current-day XFEL sources, by presenting first experimental attempts to demonstrate stimulated resonant X-ray Raman scattering in molecular gas targets.
|
|