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- Based on a recent ab initio interaction-induced dipole surface of collisionally interacting molecular hydrogen pairs H2–H2, we compute the binary absorption coefficients at wavelengths near 5 micrometers at temperatures of 77.5 and 297 K for comparison with existing laboratory measurements. We observe satisfactory agreement of the measurements with our calculations, thereby concluding an earlier study [Gustafsson et al., J. Chem. Phys. 119, 12264 (2003)], which was based on an ab initio interaction-induced dipole surface that was inadequate for the 5 micrometer band.
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