| 1. |
- Andersson, Patrik, 1974, et al.
(author)
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Framtidsbilder för samhällsbyggnad
- 2006
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Reports (other academic/artistic)abstract
- Framtidsbilder för samhällsbyggnad 2020De kommande 15 åren står institutionen för Bygg- och miljöteknik inför stora förändringar. Därför har institutionen initierat projektet Framtidsbilder 2020 där man engagerat en framtidspanel bestående av elva yngre disputerade forskare. Arbetet inleddes med ett breddgruppsmöte där 110 personer representerande institutionens personal och studenter deltog. Vid mötet identifierades ett antal trender och osäkra utvecklingar som påverkar framtiden inom samhällsbyggnadsområdet. Deltagarna bidrog också med idéer till en önskvärd utveckling, vilket har sammanställts och utgör grunden till en gemensam önskvärd framtid/vision för institutionen. Materialet från breddgruppsmötet har bearbetats av Framtidspanelen och resulterat i fyra scenarier som beskriver hur samhällsbyggnadsområdet kan se ut år 2020. Syftet med framtidsbilderna är att de ska vara vägledande för institutionens beslut och förhållningssätt under de kommande åren.Fyra scenarierTurning TorsoSamhället präglas av en ekonomi som är på uppgång, och av ett nytänkande och öppet samhälle. Materiell status och individualism är viktigt. Detta leder till en hög arbetsbelastning samt krav på exklusiva varor av hög kvali-tet. Det finns en stor medvetenhet om miljöpåverkan och klimatförändringar och lösningarna för att klara energiförsörjningen är innovativa.Eco-metropolenDet sveper en grön våg genom dagens samhälle. Under de senaste 15 åren har vi insett att jorden skall vara en bebolig plats även åt dem som kommer efter oss. Vi söker ständigt efter nya, mer förfinade metoder att tillvarata de resurser vi har. Samhället och individen är i balans. Ekonomin är god och vi är miljömedvetna, trygga och integrerade. Nytänkande premieras och icke- materialistiska värderingar står högt i kurs. Vi tänker individuellt, men agerar mer än gärna för kollektivets bästa. Utbildning är gratis TrädgårdsstadenEtt samhälle där vi lärt oss hantera stress, men känner oss otrygga och helst umgås i slutna sociala sammanhang. Vi bor enkelt inne i stan, eller gärna på landsbygden nära storstäderna. Minskade behov av högutbildade i samhället gör att vi har svårt att rekrytera studenter till teknikutbildningar. Det traditionella tankesättet leder till kulturkrockar med företag och personer från andra länder.Gated communitiesFörsämrad ekonomi och ökad egoism har lett fram till ett stressat, otryggt och segregerat samhälle. Accelererande klimatförändringar och ökad miljö-påverkan skrämmer oss, men trots det åtgärdar vi inte problemen, utan koncentrerar oss på konsekvenserna. Arbetslöshet i samhällsbyggnadssek-torn leder till sänkt status för samhällsbyggaren. Vi har därför svårt att rekrytera studenter, och även forskningen har låg status.
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| 2. |
- Andersson, Pontus, 1971, et al.
(author)
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Isobar Selective Laser Photodetachment In Trace Element Analysis
- 2009
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In: AIP Conference Proceedings. ; 1104
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Conference paper (peer-reviewed)abstract
- We are investigating the possibility to use laser photodetachment of negative ions as an isobaric selective filter in accelerator mass spectrometry (AMS). If successful, this method can be used to obtain higher sensitivity realized through better selectivity by suppression of molecular and/or elemental isobaric interference in different investigations using ultra rare isotopes in the 10−13 range and below.
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| 3. |
- Andersson, Pontus, 1971
(author)
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Laser Photodetachment of Negative Ions - Fundamental Research and Applications
- 2009
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Doctoral thesis (other academic/artistic)abstract
- Photodetachment studies of atomic and molecular negative ions in the gas phase are presented. Negative ions are loosely bound quantum systems whose existence is strongly dependent on the correlations between the electrons. This makes sophisticated calculations of the structure and dynamics for these systems complex and experimental data are needed for verification. Negative ions are also important in applications such as plasma etching and atmospheric studies. One of the most important applications for negative ions is as the state of matter for injection in tandem accelerators used in Accelerator Mass Spectrometry (AMS), the most sensitive method for ultra trace isotope analysis. Using negative ions in the injection stage provides isobar suppression in cases where the contaminating isobar does not form stable negative ions. Several experiments on laser interaction with a beam of mass-selected negative ions are presented. The objective for these studies can be divided into three subgroups: structure studies, dynamic studies, and proof-of-principle experiments for applications of negative ions. In the first group, the value for the electron affinity and the fine structure splitting of phosphorus is refined. The value of the electron affinity of tungsten is improved and the origin of the photodetachment signal below threshold is discussed. Resonant structure in the cross section and the electron affinity of cerium is treated. Finally, a predicted excited state in platinum is observed experimentally for the first time. The second group consists of the lifetime measurements of metastable excited states for tellurium, selenium and silicon. These measurements were made at the magnetic heavy ion storage ring CRYRING at Manne Siegbahn Laboratories in Stockholm. The third and last group are proof-of-principle experiments of isobar and neighboring isotope suppression by laser interaction. Suppression of up to four orders of magnitude is reached and the implementation into mass spectrometric systems are discussed.
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| 4. |
- Andersson, Pontus, 1971, et al.
(author)
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Observation of the 2S1/2 metastable state in Pt−
- 2009
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In: PHYSICAL REVIEW A. - 1050-2947. ; 79, s. 022502 -
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Journal article (peer-reviewed)abstract
- We have experimentally investigated the structure of the Pt− ion using laser photodetachment threshold spectroscopy. The experiment was conducted using a collinear laser-ion beam apparatus, in which the residual atoms created in the photodetachment process were detected. A p-wave threshold was observed in the photo- detachment spectrum at an energy of 6851͑13͒ cm−1. We conclude that this onset originates from a photode- tachment transition in which the initial state of Pt− is the previously unobserved 5d106s 2S1/2 state and the final state of Pt is the 5d96s 3D3 ground state. The excitation energy of the 2S1/2 state is determined to be 10 289͑13͒ cm−1. This value can be compared with a multiconfiguration Dirac-Fock calculation performed by Thøgersen et al. ͓Phys. Rev. Lett. 76, 2870 ͑1996͔͒, which yielded an excitation energy of 11 301 cm−1. Our data show no indication of the presence of any other state of Pt−. We conclude that the structure of the Pt− ion is now fully known.
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| 5. |
- Andersson, Pontus, 1971, et al.
(author)
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Radiative lifetimes of metastable states of negative ions
- 2006
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In: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622 .- 2469-9926 .- 2469-9934. ; 73, s. 032705-
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Journal article (peer-reviewed)abstract
- We present a technique for measuring the radiative lifetimes of metastable states of negative ions that involves the use of a heavy-ion storage ring. The method has been applied to investigate the radiative decay of the np(3) P-2(1/2) levels of Te-(n=5) and Se-(n=4) and the 3p(3) D-2 state of Si- for which the J=3/2 and 5/2 levels were unresolved. All of these states are metastable and decay primarily by emission of E2 and M1 radiation. Multi Configuration Dirac-Hartree-Fock calculations of rates for the transitions in Te- and Se- yielded lifetimes of 0.45 s and 4.7 s, respectively. The measured values agree well with these predicted values. In the case of the D-2 state of Si-, however, our measurement was only able to set a lower limit on the lifetime. The upper limit of the lifetime that can be measured with our apparatus is set by how long the ions can be stored in the ring, a limit determined by the rate of collisional detachment. Our lower limit of 1 min for the lifetime of the D-2 state is consistent with both the calculated lifetimes of 162 s for the D-2(3/2) level and 27.3 h for the D-2(5/2) level reported by O'Malley and Beck and 14.5 h and 12.5 h, respectively, from our Breit-Pauli calculations.
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| 6. |
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| 7. |
- Andersson, Pontus, 1971, et al.
(author)
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The electron affinity of phosphorus
- 2007
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In: Journal of Physics B-Atomic Molecular and Optical Physics. ; 40:20, s. 4097-4107
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Journal article (peer-reviewed)
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| 8. |
- Bilodeau, R. C., et al.
(author)
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High-charge-state formation following inner-shell photodetachment from S-
- 2005
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In: Physical Review A. - 1050-2947. ; 72, s. 050701-
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Journal article (peer-reviewed)abstract
- The formation of S+, S2+, S3+, and S4+ is observed following inner-shell photodetachment of S–. The photodetachment spectra for all possible ionic products are obtained over a large region of photon energies covering both the 2p and 2s thresholds (S5+, is energetically allowed at the higher photon energies, but not observed), and are placed on an absolute scale. The 2s threshold energy is measured to be 224.6(5) eV, allowing the determination of the neutral atomic S 2s–13s23p5 inner-shell excited state energy for the first time. The S– 2s–13s23p6 2S1/2 state is observed as a Feshbach resonance 2.3(5) eV below the 2s threshold in the S+, S2+, and S3+ product channels.
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| 9. |
- Forstner, O., et al.
(author)
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Isobar suppression in AMS using laser photodetachment
- 2008
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In: Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms. ; 266:19-20, s. 4565-4568
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Journal article (peer-reviewed)abstract
- We are investigating the possibility of using laser photodetachment of negative atomic and molecular ions as an additional isobaric selection filter in accelerator mass spectrometry. The aim of this study is to find a possibility to further improve the detection limit for long-lived heavy radionuclides at AMS facilities. We will focus on the astrophysical relevant radionuclide 182Hf, which is one of the isotopes measured with the 3 MV tandem AMS facility VERA (Vienna Environmental Research Accelerator) at the University of Vienna. Laser-induced isobar suppression is also of importance for radioactive-beam facilities. The present detection limit for measuring the isotope ratio 182Hf/Hf at VERA is 1×10-11. The limiting factor is the strong background of the stable isobar 182W. Currently this background is suppressed using suitable molecular ions in the injection stage. Selective laser photodetachment of the negative ions at the injector can lead to an additional suppression of the interfering isobar. Test experiments have been carried out at the negative ion laser spectroscopy setup at Göteborg University. In a small ion beam apparatus pulsed tunable laser radiation is used to measure the photodetachment cross-section of different atomic and molecular negative ions. We will present studies of the photodetachment process for various tungsten and hafnium molecules with the aim to find a selective isobaric suppression scheme using laser photodetachment spectroscopy in combination with AMS.
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| 10. |
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| 11. |
- Walter, C. W., et al.
(author)
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Infrared photodetachment of Ce-: Threshold spectroscopy and resonance structure
- 2007
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In: Physical Review A. - 1050-2947. ; 76, s. 052702-
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Journal article (peer-reviewed)abstract
- The negative ion of cerium is investigated using tunable laser photodetachment threshold spectroscopy. The relative cross section for photodetachment from Ce− is measured over the photon energy range 0.61–0.75 eV using a crossed laser-beam–ion-beam technique. The spectrum of neutral atom production reveals a photodetachment threshold at 0.65 eV, which is interpreted as the threshold for the Ce− (4f5d26s2 4H7/2) to Ce (4f5d6s2 1G4) ground-state to ground-state transition yielding the electron affinity of Ce to be 0.65(3) eV. At least five narrow peaks are observed in the cross section over the range 0.62–0.70 eV due to negative ion resonances, and their energies and widths are measured. The results are compared to other recent experimental and theoretical studies of Ce−.
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