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  • Punkkinen, M. P. J. (author)

Bismuth-stabilized (2x1) and (2x4) reconstructions on GaAs(100) surfaces : Combined first-principles, photoemission, and scanning tunneling microscopy study

  • Article/chapterEnglish2008

Publisher, publication year, extent ...

  • 2008
  • printrdacarrier

Numbers

  • LIBRIS-ID:oai:DiVA.org:kth-18114
  • https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-18114URI
  • https://doi.org/10.1103/PhysRevB.78.195304DOI
  • https://research.chalmers.se/publication/87568URI
  • https://lup.lub.lu.se/record/1375987URI
  • https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-137370URI

Supplementary language notes

  • Language:English
  • Summary in:English

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  • Subject category:ref swepub-contenttype
  • Subject category:art swepub-publicationtype

Notes

  • QC 20100525
  • Bismuth adsorbate-stabilized (2x1) and (2x4) reconstructions of the GaAs(100) surfaces have been studied by first-principles calculations, valence-band and core-level photoelectron spectroscopies, and scanning tunneling microscopy. It is demonstrated that large Bi atom size leads to the formation of the pseudogap at the Fermi energy and to the lower energy of an adsorbate-derived surface band, which contributes to the stabilization of the exceptional Bi/GaAs(100)(2x1) reconstruction. It is proposed that the Bi/GaAs(100)(2x4) reconstructions include asymmetric mixed Bi-As dimers, in addition to the Bi-Bi dimers. Based on the calculations, we solve the atomic origins of the surface core-level shifts (SCLSs) of the Bi 5d photoemission spectra from the Bi/GaAs(100)(2x4) surfaces. This allows for resolving the puzzle related to the identification of two SCLS components often found in the measurements of the Bi 5d and Sb 4d core-level emissions of the Bi/III-V and Sb/III-V(100)(2x4) surfaces. Finally, the reason for the absence of the common (2x4)-beta 2 structure and additional support for the stability of the (2x1) structure on the Bi/III-V(100) surfaces are discussed in terms of Bi atom size and subsurface stress.

Subject headings and genre

Added entries (persons, corporate bodies, meetings, titles ...)

  • Laukkanen, P. (author)
  • Komsa, H. P. (author)
  • Ahola-Tuomi, M. (author)
  • Rasanen, N. (author)
  • Kokko, K. (author)
  • Kuzmin, M. (author)
  • Adell, Johan,1980Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory(Swepub:lu)maxl-jae (author)
  • Sadowski, JanuszLund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory(Swepub:lu)maxl-jsa (author)
  • Perala, R. E. (author)
  • Ropo, M. (author)
  • Rantala, T. T. (author)
  • Vayrynen, I. J. (author)
  • Pessa, M. (author)
  • Vitos, LeventeUppsala universitet,KTH,Tillämpad materialfysik,Materialteori(Swepub:uu)lvi21721 (author)
  • Kollar, J. (author)
  • Mirbt, SusanneUppsala universitet,Materialteori(Swepub:uu)susamirb (author)
  • Johansson, BörjeUppsala universitet,KTH,Tillämpad materialfysik,Materialteori(Swepub:uu)borjejs (author)
  • Lunds universitetMAX IV-laboratoriet (creator_code:org_t)

Related titles

  • In:Physical Review B. Condensed Matter and Materials Physics78, s. 195304-1098-01211550-235X
  • In:Physical Review B78, s. 195304-

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