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Selective gating to...
Selective gating to vibrational modes through resonant X-ray scattering
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- C. Couto, Rafael, 1987- (author)
- KTH,Teoretisk kemi och biologi,Theoretical Chemistry and Biology
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- Vaz da Cruz, Vinícius (author)
- KTH,Teoretisk kemi och biologi,Theoretical Chemistry and Biology
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- Ertan, Emelie (author)
- Stockholms universitet,Fysikum
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Eckert, Sebastian (author)
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Fondell, Mattis (author)
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Dantz, Marcus (author)
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Kennedy, Brian (author)
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Schmitt, Thorsten (author)
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Pietzsch, Annette (author)
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F. Guimarães, Freddy (author)
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- Ågren, Hans (author)
- KTH,Teoretisk kemi och biologi,Theoretical Chemistry and Biology
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- Gel’mukhanov, Faris (author)
- KTH,Teoretisk kemi och biologi,Theoretical Chemistry and Biology
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- Odelius, Michael (author)
- Stockholms universitet,Fysikum
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- Kimberg, Victor (author)
- KTH,Teoretisk kemi och biologi,Theoretical Chemistry and Biology
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Föhlisch, Alexander (author)
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(creator_code:org_t)
- 2017-01-20
- 2017
- English.
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In: Nature Communications. - : Macmillan Publishers Ltd.. - 2041-1723. ; 8, s. 14165-1-14165-7
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https://doi.org/10.1...
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http://www.nature.co...
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https://doi.org/10.1...
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Abstract
Subject headings
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- The dynamics of fragmentation and vibration of molecular systems with a large number of coupled degrees of freedom are key aspects for understanding chemical reactivity and properties. Here we present a resonant inelastic X-ray scattering (RIXS) study to show how it is possible to break down such a complex multidimensional problem into elementary components. Local multimode nuclear wave packets created by X-ray excitation to different core-excited potential energy surfaces (PESs) will act as spatial gates to selectively probe the particular ground-state vibrational modes and, hence, the PES along these modes. We demonstrate this principle by combining ultra-high resolution RIXS measurements for gas-phase water with state-of-the-art simulations.
Subject headings
- NATURVETENSKAP -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)
- NATURVETENSKAP -- Kemi -- Teoretisk kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Theoretical Chemistry (hsv//eng)
- NATURVETENSKAP -- Fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences (hsv//eng)
Keyword
- water
- resonant inelastic x-ray scattering
- vibrational modes
- RIXS
- Teoretisk kemi och biologi
- Theoretical Chemistry and Biology
- kemisk fysik
Publication and Content Type
- ref (subject category)
- art (subject category)
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To the university's database
- By the author/editor
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C. Couto, Rafael ...
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Vaz da Cruz, Vin ...
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Ertan, Emelie
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Eckert, Sebastia ...
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Fondell, Mattis
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Dantz, Marcus
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show more...
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Kennedy, Brian
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Schmitt, Thorste ...
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Pietzsch, Annett ...
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F. Guimarães, Fr ...
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Ågren, Hans
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Gel’mukhanov, Fa ...
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Odelius, Michael
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Kimberg, Victor
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Föhlisch, Alexan ...
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show less...
- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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and Atom and Molecul ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Chemical Science ...
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and Theoretical Chem ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
- Articles in the publication
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Nature Communica ...
- By the university
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Royal Institute of Technology
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Stockholm University