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  • Cappel, Ute B.Uppsala universitet,KTH,Tillämpad fysik,Molekyl- och kondenserade materiens fysik,KTH Royal Inst Technol, Div Appl Phys Chem, Dept Chem, Stockholm, Sweden (author)

Electronic Structure Characterization of Cross-Linked Sulfur Polymers

  • Article/chapterEnglish2018

Publisher, publication year, extent ...

  • 2018-02-27
  • WILEY-V C H VERLAG GMBH,2018
  • printrdacarrier

Numbers

  • LIBRIS-ID:oai:DiVA.org:kth-228264
  • https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-228264URI
  • https://doi.org/10.1002/cphc.201800043DOI
  • https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-356387URI

Supplementary language notes

  • Language:English
  • Summary in:English

Part of subdatabase

Classification

  • Subject category:ref swepub-contenttype
  • Subject category:art swepub-publicationtype

Notes

  • QC 20180523
  • Cross-linked polymers of elemental sulfur are of potential interest for electronic applications as they enable facile thin-film processing of an abundant and inexpensive starting material. Here, we characterize the electronic structure of a cross-linked sulfur/diisopropenyl benzene (DIB) polymer by a combination of soft and hard X-ray photoelectron spectroscopy (SOXPES and HAXPES). Two different approaches for enhancing the conductivity of the polymer are compared: the addition of selenium in the polymer synthesis and the addition of lithium bis(trifluoromethanesulfonyl)imide (LiTFSI) during film preparation. For the former, we observe the incorporation of Se into the polymer structure resulting in a changed valence-band structure. For the latter, a Fermi level shift in agreement with p-type doping of the polymer is observed and also the formation of a surface layer consisting mostly of TFSI anions.

Subject headings and genre

Added entries (persons, corporate bodies, meetings, titles ...)

  • Liu, PengKTH,Tillämpad materialfysik,Molekylär elektronik, CMD,KTH Royal Inst Technol, Div Appl Phys Chem, Dept Chem, SE-10044 Stockholm, Sweden(Swepub:kth)u1zkvq1z (author)
  • Johansson, FredrikUppsala universitet,Molekyl- och kondenserade materiens fysik(Swepub:uu)frejo210 (author)
  • Philippe, Bertrand,Dr.1986-Uppsala universitet,Molekyl- och kondenserade materiens fysik(Swepub:uu)phibe331 (author)
  • Giangrisostomi, ErikaHelmholtz Zentrum Berlin GmbH, Inst Methods & Instrumentat Synchrotron Radiat Re, Albert Einstein Str 15, D-12489 Berlin, Germany. (author)
  • Ovsyannikov, RuslanHelmholtz Zentrum Berlin GmbH, Inst Methods & Instrumentat Synchrotron Radiat Re, Albert Einstein Str 15, D-12489 Berlin, Germany. (author)
  • Lindblad, AndreasUppsala universitet,Molekyl- och kondenserade materiens fysik(Swepub:uu)anlin087 (author)
  • Kloo, LarsKTH,Molekylär elektronik, CMD,KTH Royal Inst Technol, Div Appl Phys Chem, Dept Chem, SE-10044 Stockholm, Sweden(Swepub:kth)u1jrdr1m (author)
  • Gardner, James M.,1982-KTH,Molekylär elektronik, CMD,KTH Royal Inst Technol, Div Appl Phys Chem, Dept Chem, SE-10044 Stockholm, Sweden(Swepub:kth)u1r55ysm (author)
  • Rensmo, HåkanUppsala universitet,Molekyl- och kondenserade materiens fysik(Swepub:uu)hakanrm (author)
  • KTHTillämpad fysik (creator_code:org_t)

Related titles

  • In:ChemPhysChem: WILEY-V C H VERLAG GMBH19:9, s. 1041-10471439-42351439-7641

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