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Novel Zinc Complex with an Ethylenediamine Schiff Base for High-Luminance Blue Fluorescent OLED Applications

Gusev, Alexey N. (author)
Russian Acad Sci, NS Kurnakov Inst Gen & Inorgan Chem, Moscow 119991, Russia.
Kiskin, Mikhail A. (author)
Russian Acad Sci, NS Kurnakov Inst Gen & Inorgan Chem, Moscow 119991, Russia.
Braga, Elena V. (author)
Russian Acad Sci, NS Kurnakov Inst Gen & Inorgan Chem, Moscow 119991, Russia.
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Chapran, Marian (author)
Lodz Univ Technol, Dept Mol Phys, Zeromskiego 116, PL-90924 Lodz, Poland.
Wiosna-Salyga, Gabriela (author)
Lodz Univ Technol, Dept Mol Phys, Zeromskiego 116, PL-90924 Lodz, Poland.
Baryshnikov, Gleb V. (author)
KTH,Teoretisk kemi och biologi,Tomsk State Univ, 36 Lenin Ave, Tomsk 634050, Russia.
Minaeva, Valentina A. (author)
Bohdan Khmelnytsky Natl Univ, Dept Chem & Nanomat Sci, UA-18031 Cherkassy, Ukraine.
Minaev, Boris F. (author)
Bohdan Khmelnytsky Natl Univ, Dept Chem & Nanomat Sci, UA-18031 Cherkassy, Ukraine.
Ivaniuk, Khrystyna (author)
Lviv Polytech Natl Univ, Stepan Bandera 12, UA-79013 Lvov, Ukraine.
Stakhira, Pavlo (author)
Lviv Polytech Natl Univ, Stepan Bandera 12, UA-79013 Lvov, Ukraine.
Ågren, Hans (author)
KTH,Teoretisk kemi och biologi,Tomsk State Univ, 36 Lenin Ave, Tomsk 634050, Russia.
Linert, Wolfgang (author)
Vienna Univ Technol, Inst Appl Synthet Chem, Getreidemarkt 9-163 AC, A-1060 Vienna, Austria.
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Russian Acad Sci, NS Kurnakov Inst Gen & Inorgan Chem, Moscow 119991, Russia Lodz Univ Technol, Dept Mol Phys, Zeromskiego 116, PL-90924 Lodz, Poland. (creator_code:org_t)
2019-04-11
2019
English.
In: The Journal of Physical Chemistry C. - : AMER CHEMICAL SOC. - 1932-7447 .- 1932-7455. ; 123:18, s. 11850-11859
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  • Journal article (peer-reviewed)
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  • To explore the photophysical properties of coordination compounds with bright blue fluorescence, an azomethin-zinc complex was synthesized and characterized by various techniques (elemental analysis, thermogravimetry, and IR-mass-spectroscopy). The crystal structure was determined by X-ray diffraction analysis. Through thermal characterization, this complex was proved to have good thermal stability. Photoluminescence spectra were recorded, both in solution and in the solid state, and the complexes showed noteworthy photoluminescence with a maximum in the blue region. The results of time-dependent density functional theory calculations indicated that the origin of luminescence for the title complex is a combination of monomer and excimer emissions. The light emission performance of the zinc complex in organic light emitting diodes was investigated, and the results indicated superior electroluminescence properties as a blue fluorescent light source (max. brightness 17 000 cd/m(2), max. EQE = 5%).

Subject headings

NATURVETENSKAP  -- Kemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences (hsv//eng)

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