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- Maclot, SylvainKTH Royal Institute of Technology,Lund University,Lunds universitet,KTH,Biomedicinsk fysik och röntgenfysik,Department of Physics, Lund University, P.O. Box 118, Lund, 22100, Sweden,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Departments at LTH,Faculty of Engineering, LTH (author)
Dissociation dynamics of the diamondoid adamantane upon photoionization by XUV femtosecond pulses
- Article/chapterEnglish2020
Publisher, publication year, extent ...
- 2020-02-19
- Nature Research,2020
- printrdacarrier
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- LIBRIS-ID:oai:DiVA.org:kth-276266
- https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-276266URI
- https://doi.org/10.1038/s41598-020-59649-1DOI
- https://lup.lub.lu.se/record/3aa95e7a-05bd-4f06-a4ae-2e8b164aae06URI
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- Language:English
- Summary in:English
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- QC 20200622
- This work presents a photodissociation study of the diamondoid adamantane using extreme ultraviolet femtosecond pulses. The fragmentation dynamics of the dication is unraveled by the use of advanced ion and electron spectroscopy giving access to the dissociation channels as well as their energetics. To get insight into the fragmentation dynamics, we use a theoretical approach combining potential energy surface determination, statistical fragmentation methods and molecular dynamics simulations. We demonstrate that the dissociation dynamics of adamantane dications takes place in a two-step process: barrierless cage opening followed by Coulomb repulsion-driven fragmentation.
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- Lahl, JanLund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH(Swepub:lu)fysi-jlh (author)
- Peschel, JasperLund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH(Swepub:lu)ja7503pe (author)
- Wikmark, HampusLund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH(Swepub:lu)fysi-hwr (author)
- Rudawski, PiotrLund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH(Swepub:lu)fysi-prr (author)
- Brunner, FabianLund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH(Swepub:lu)fa5684br (author)
- Coudert-Alteirac, HélèneLund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH(Swepub:lu)fysi-hco (author)
- Indrajith, S.University of Caen Normandy (author)
- Huber, B. A.University of Caen Normandy (author)
- Díaz-Tendero, S.Autonomous University of Madrid (author)
- Aguirre, N. F.Los Alamos National Laboratory (author)
- Rousseau, P.University of Caen Normandy (author)
- Johnsson, PerLund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH(Swepub:lu)fysi-pj0 (author)
- KTHBiomedicinsk fysik och röntgenfysik (creator_code:org_t)
Related titles
- In:Scientific Reports: Nature Research10:12045-2322
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- https://doi.org/10.1038/s41598-020-59649-1Fulltext
- https://www.nature.com/articles/s41598-020-59649-1.pdf
- http://dx.doi.org/10.1038/s41598-020-59649-1FULLTEXT
- https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-276266
- https://doi.org/10.1038/s41598-020-59649-1
- https://lup.lub.lu.se/record/3aa95e7a-05bd-4f06-a4ae-2e8b164aae06
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