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Core-level nonlinea...
Core-level nonlinear spectroscopy triggered by stochastic X-ray pulses
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- Kayser, Yves (author)
- Phys Tech Bundesanstalt, Abbestr 2-12, D-10587 Berlin, Germany;Paul Scherrer Inst, CH-5232 Villigen, Switzerland
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- Milne, Chris (author)
- Paul Scherrer Inst, CH-5232 Villigen, Switzerland
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- Juranic, Pavle (author)
- Paul Scherrer Inst, CH-5232 Villigen, Switzerland
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- Sala, Leonardo (author)
- Paul Scherrer Inst, CH-5232 Villigen, Switzerland
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- Czapla-Masztafiak, Joanna (author)
- Polish Acad Sci, Inst Nucl Phys, PL-31342 Krakow, Poland
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- Follath, Rolf (author)
- Paul Scherrer Inst, CH-5232 Villigen, Switzerland
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- Kavcic, Matjaz (author)
- Inst Jozef Stefan, Jamova 39, Ljubljana 1000, Slovenia
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- Knopp, Gregor (author)
- Paul Scherrer Inst, CH-5232 Villigen, Switzerland
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- Rehanek, Jens (author)
- Paul Scherrer Inst, CH-5232 Villigen, Switzerland;Adv Accelerator Technol AG, CH-5234 Villigen, Switzerland
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- Blachucki, Wojciech (author)
- Polish Acad Sci, Inst Phys Chem, PL-01224 Warsaw, Poland
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- Delcey, Mickael G (author)
- Uppsala universitet,Teoretisk kemi
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- Lundberg, Marcus, 1974- (author)
- Uppsala universitet,Teoretisk kemi
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- Tyrala, Krzysztof (author)
- Polish Acad Sci, Inst Nucl Phys, PL-31342 Krakow, Poland
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- Zhu, Diling (author)
- SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA
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- Alonso-Mori, Roberto (author)
- SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA
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- Abela, Rafael (author)
- Paul Scherrer Inst, CH-5232 Villigen, Switzerland
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- Sá, Jacinto (author)
- Uppsala universitet,Fysikalisk kemi,Polish Acad Sci, Inst Phys Chem, PL-01224 Warsaw, Poland
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- Szlachetkc, Jakub (author)
- Polish Acad Sci, Inst Nucl Phys, PL-31342 Krakow, Poland
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(creator_code:org_t)
- 2019-10-18
- 2019
- English.
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In: Nature Communications. - : Springer Nature. - 2041-1723. ; 10:1
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Abstract
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- Stochastic processes are highly relevant in research fields as different as neuroscience, economy, ecology, chemistry, and fundamental physics. However, due to their intrinsic unpredictability, stochastic mechanisms are very challenging for any kind of investigations and practical applications. Here we report the deliberate use of stochastic X-ray pulses in two-dimensional spectroscopy to the simultaneous mapping of unoccupied and occupied electronic states of atoms in a regime where the opacity and transparency properties of matter are subject to the incident intensity and photon energy. A readily transferable matrix formalism is presented to extract the electronic states from a dataset measured with the monitored input from a stochastic excitation source. The presented formalism enables investigations of the response of the electronic structure to irradiation with intense X-ray pulses while the time structure of the incident pulses is preserved.
Subject headings
- NATURVETENSKAP -- Kemi -- Fysikalisk kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Physical Chemistry (hsv//eng)
Publication and Content Type
- ref (subject category)
- art (subject category)
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- By the author/editor
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Kayser, Yves
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Milne, Chris
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Juranic, Pavle
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Sala, Leonardo
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Czapla-Masztafia ...
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Follath, Rolf
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show more...
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Kavcic, Matjaz
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Knopp, Gregor
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Rehanek, Jens
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Blachucki, Wojci ...
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Delcey, Mickael ...
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Lundberg, Marcus ...
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Tyrala, Krzyszto ...
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Zhu, Diling
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Alonso-Mori, Rob ...
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Abela, Rafael
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Sá, Jacinto
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Szlachetkc, Jaku ...
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- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Chemical Science ...
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and Physical Chemist ...
- Articles in the publication
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Nature Communica ...
- By the university
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Royal Institute of Technology
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Uppsala University