Search: onr:"swepub:oai:DiVA.org:kth-290069" > Vibrational wavepac...
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000 | 12022naa a2200949 4500 | |
001 | oai:DiVA.org:kth-290069 | |
003 | SwePub | |
008 | 210212s2020 | |||||||||||000 ||eng| | |
009 | oai:DiVA.org:uu-407449 | |
009 | oai:lup.lub.lu.se:1ecf1f3d-2ed2-48cc-9e30-6a91fa52a822 | |
024 | 7 | a https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-2900692 URI |
024 | 7 | a https://doi.org/10.1038/s41467-020-14468-w2 DOI |
024 | 7 | a https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-4074492 URI |
024 | 7 | a https://lup.lub.lu.se/record/1ecf1f3d-2ed2-48cc-9e30-6a91fa52a8222 URI |
040 | a (SwePub)kthd (SwePub)uud (SwePub)lu | |
041 | a engb eng | |
042 | 9 SwePub | |
072 | 7 | a ref2 swepub-contenttype |
072 | 7 | a art2 swepub-publicationtype |
100 | 1 | a Kunnus, Kristjanu Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut |
245 | 1 0 | a Vibrational wavepacket dynamics in Fe carbene photosensitizer determined with femtosecond X-ray emission and scattering |
264 | c 2020-01-31 | |
264 | 1 | b Springer Nature,c 2020 |
338 | a electronic2 rdacarrier | |
500 | a QC 20210215 | |
520 | a The non-equilibrium dynamics of electrons and nuclei govern the function of photoactive materials. Disentangling these dynamics remains a critical goal for understanding photoactive materials. Here we investigate the photoinduced dynamics of the [Fe(bmip)2]2+ photosensitizer, where bmip = 2,6-bis(3-methyl-imidazole-1-ylidine)-pyridine, with simultaneous femtosecond-resolution Fe Kα and Kβ X-ray emission spectroscopy (XES) and X-ray solution scattering (XSS). This measurement shows temporal oscillations in the XES and XSS difference signals with the same 278 fs period oscillation. These oscillations originate from an Fe-ligand stretching vibrational wavepacket on a triplet metal-centered (3MC) excited state surface. This 3MC state is populated with a 110 fs time constant by 40% of the excited molecules while the rest relax to a 3MLCT excited state. The sensitivity of the Kα XES to molecular structure results from a 0.7% average Fe-ligand bond length shift between the 1 s and 2p core-ionized states surfaces. | |
650 | 7 | a NATURVETENSKAPx Kemix Fysikalisk kemi0 (SwePub)104022 hsv//swe |
650 | 7 | a NATURAL SCIENCESx Chemical Sciencesx Physical Chemistry0 (SwePub)104022 hsv//eng |
650 | 7 | a NATURVETENSKAPx Fysikx Atom- och molekylfysik och optik0 (SwePub)103022 hsv//swe |
650 | 7 | a NATURAL SCIENCESx Physical Sciencesx Atom and Molecular Physics and Optics0 (SwePub)103022 hsv//eng |
700 | 1 | a Vacher, Morganeu Uppsala University,Uppsala universitet,Teoretisk kemi4 aut0 (Swepub:uu)morva594 |
700 | 1 | a Harlang, Tobias C.B.u Lund University,Lunds universitet,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,Technical University of Denmark4 aut0 (Swepub:lu)chem-tbh |
700 | 1 | a Kjaer, Kasper S.u Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA;Lund Univ, Dept Chem Phys, POB 12, S-422100 Lund, Sweden;Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark4 aut |
700 | 1 | a Haldrup, Kristofferu Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark,Technical University of Denmark4 aut |
700 | 1 | a Biasin, Elisau Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA;Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark,Stanford Linear Accelerator Center (SLAC),Technical University of Denmark4 aut |
700 | 1 | a van Driel, Tim B.u SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut |
700 | 1 | a Papai, Matyasu Tech Univ Denmark, Dept Chem, Kemitorvet 207, DK-2800 Lyngby, Denmark,Technical University of Denmark4 aut |
700 | 1 | a Chabera, Pavelu Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Kemisk fysik,Enheten för fysikalisk och teoretisk kemi,Kemiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Chemical Physics,Physical and theoretical chemistry,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH4 aut0 (Swepub:lu)chem-pcr |
700 | 1 | a Liu, Yizhuu Lund University,Lunds universitet,Centrum för analys och syntes,Kemiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Kemisk fysik,Enheten för fysikalisk och teoretisk kemi,Centre for Analysis and Synthesis,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH,Chemical Physics,Physical and theoretical chemistry,Faculty of Engineering, LTH4 aut0 (Swepub:lu)orga-yhl |
700 | 1 | a Tatsuno, Hideyukiu Lund University,Lunds universitet,Kemisk fysik,Enheten för fysikalisk och teoretisk kemi,Kemiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Chemical Physics,Physical and theoretical chemistry,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH4 aut0 (Swepub:lu)hi2364ta |
700 | 1 | a Timm, Corneliau Lund Univ, Dept Chem Phys, POB 12, S-422100 Lund, Sweden,Lund University4 aut |
700 | 1 | a Källman, Erik,c PhDu Uppsala University,Uppsala universitet,Teoretisk kemi4 aut0 (Swepub:uu)erika993 |
700 | 1 | a Delcey, Mickaëlu Uppsala University,Uppsala universitet,Teoretisk kemi4 aut0 (Swepub:lu)teok-mdl |
700 | 1 | a Hartsock, Robert W.u Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut |
700 | 1 | a Reinhard, Marco E.u Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut |
700 | 1 | a Koroidov, Sergeyu Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut |
700 | 1 | a Laursen, Mads G.u Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark,Technical University of Denmark4 aut |
700 | 1 | a Hansen, Frederik B.u Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark,Technical University of Denmark4 aut |
700 | 1 | a Persson, Petteru Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Beräkningskemi,Enheten för fysikalisk och teoretisk kemi,Kemiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Computational Chemistry,Physical and theoretical chemistry,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH4 aut0 (Swepub:lu)chem-ppn |
700 | 1 | a Christensen, Mortenu Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark,Technical University of Denmark4 aut |
700 | 1 | a Sandberg, Liseu Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark;Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark,Technical University of Denmark,Niels Bohr Institute4 aut |
700 | 1 | a Nemeth, Zoltanu Hungarian Acad Sci, Wigner Res Ctr Phys, POB 49, H-1525 Budapest, Hungary,Wigner Research Centre for Physics, Hungarian Academy of Sciences4 aut |
700 | 1 | a Szemes, Dorottya Sarosineu Hungarian Acad Sci, Wigner Res Ctr Phys, POB 49, H-1525 Budapest, Hungary,Wigner Research Centre for Physics, Hungarian Academy of Sciences4 aut |
700 | 1 | a Bajnoczi, Evau Hungarian Acad Sci, Wigner Res Ctr Phys, POB 49, H-1525 Budapest, Hungary,Wigner Research Centre for Physics, Hungarian Academy of Sciences4 aut |
700 | 1 | a Alonso-Mori, Robertou SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut |
700 | 1 | a Glownia, James M.u SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut |
700 | 1 | a Nelson, Silkeu SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut |
700 | 1 | a Sikorski, Marcinu SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut |
700 | 1 | a Sokaras, Dimosthenisu SLAC Natl Accelerator Lab, SSRL, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut |
700 | 1 | a Lemke, Henrik T.u SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut |
700 | 1 | a Canton, Sophie E.u ELI HU Nonprofit Ltd, ELI ALPS, H-6720 Szeged, Hungary;DESY, Notkestr 85, D-22607 Hamburg, Germany,German Electron Synchrotron (DESY),ELI-HU Non-profit Ltd4 aut0 (Swepub:lu)chem-sca |
700 | 1 | a Moller, Klaus B.u Tech Univ Denmark, Dept Chem, Kemitorvet 207, DK-2800 Lyngby, Denmark,Technical University of Denmark4 aut |
700 | 1 | a Nielsen, Martin M.u Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark,Technical University of Denmark4 aut |
700 | 1 | a Vank, Gyorgyu Hungarian Acad Sci, Wigner Res Ctr Phys, POB 49, H-1525 Budapest, Hungary,Wigner Research Centre for Physics, Hungarian Academy of Sciences4 aut |
700 | 1 | a Wärnmark, Kennethu Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Centrum för analys och syntes,Kemiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Centre for Analysis and Synthesis,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH4 aut0 (Swepub:lu)orgk1-kw |
700 | 1 | a Sundström, Villyu Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Kemisk fysik,Enheten för fysikalisk och teoretisk kemi,Kemiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Chemical Physics,Physical and theoretical chemistry,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH4 aut0 (Swepub:lu)chph-vs |
700 | 1 | a Persson, Petteru Lund Univ, Theoret Chem Div, POB 12422100, Lund, Sweden4 aut |
700 | 1 | a Lundberg, Marcus,d 1974-u Uppsala University,Uppsala universitet,Teoretisk kemi4 aut0 (Swepub:uu)marlu250 |
700 | 1 | a Uhlig, Jensu Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Kemisk fysik,Enheten för fysikalisk och teoretisk kemi,Kemiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Chemical Physics,Physical and theoretical chemistry,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH4 aut0 (Swepub:lu)chem-jnu |
700 | 1 | a Gaffney, Kelly J.u Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut |
700 | 1 | a Kjær, Kasper S.u Lund University,Lunds universitet,Kemisk fysik,Enheten för fysikalisk och teoretisk kemi,Kemiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Chemical Physics,Physical and theoretical chemistry,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH,Stanford Linear Accelerator Center (SLAC),Technical University of Denmark4 aut0 (Swepub:lu)chem-kkr |
710 | 2 | a Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USAb Stanford Linear Accelerator Center (SLAC)4 org |
773 | 0 | t Nature Communicationsd : Springer Natureg 11:1q 11:1x 2041-1723 |
856 | 4 | u https://doi.org/10.1038/s41467-020-14468-wy Fulltext |
856 | 4 | u https://kth.diva-portal.org/smash/get/diva2:1527953/FULLTEXT01.pdfx primaryx Raw objecty fulltext:print |
856 | 4 | u https://www.nature.com/articles/s41467-020-14468-w.pdf |
856 | 4 | u https://uu.diva-portal.org/smash/get/diva2:1416740/FULLTEXT01.pdfx primaryx Raw objecty fulltext:print |
856 | 4 | u http://dx.doi.org/10.1038/s41467-020-14468-wx freey FULLTEXT |
856 | 4 8 | u https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-290069 |
856 | 4 8 | u https://doi.org/10.1038/s41467-020-14468-w |
856 | 4 8 | u https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-407449 |
856 | 4 8 | u https://lup.lub.lu.se/record/1ecf1f3d-2ed2-48cc-9e30-6a91fa52a822 |
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