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Photon Up-Conversion via Epitaxial Surface-Supported Metal-Organic Framework Thin Films with Enhanced Photocurrent
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- Ahmad, Shargeel (author)
- Dalian Univ Technol, Inst Artificial Photosynth, State Key Lab Fine Chem, Dalian 116024, Peoples R China.
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- Liu, Jinxuan (author)
- Dalian Univ Technol, Inst Artificial Photosynth, State Key Lab Fine Chem, Dalian 116024, Peoples R China.
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- Gong, Chenghuan (author)
- Dalian Univ Technol, Inst Artificial Photosynth, State Key Lab Fine Chem, Dalian 116024, Peoples R China.
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- Dalian Univ Technol, Inst Artificial Photosynth, State Key Lab Fine Chem, Dalian 116024, Peoples R China Molekylär elektronik, CMD (creator_code:org_t)
- 2018-02-05
- 2018
- English.
- In: ACS Applied Energy Materials. - : American Chemical Society (ACS). - 2574-0962. ; 1:2, s. 249-253
- Journal article (peer-reviewed)
Abstract
Subject headings
Close
- We report a new triplet-triplet annihilation photon up-conversion (TTA-UC) system using an epitaxial Zn-perylene surface-supported metal-organic framework (SURMOF) grown on metal oxide surface as "emitter", and a platinum octaethylporphyrin (PtOEP) as "sensitizer" in [Co(bpy)(3)](2+/3+) acetonitrile solution. It has been demonstrated that the photocurrent can be significantly enhanced relative to epitaxial Zn-perylene SURMOF due to the TTA-UC mechanism. This initial result holds promising applications toward SURMOF-based solar energy conversion devices.
Subject headings
- NATURVETENSKAP -- Kemi -- Fysikalisk kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Physical Chemistry (hsv//eng)
Keyword
- triplet-triplet annihilation
- up-conversion
- metal-organic framework thin film
- photocurrent
Publication and Content Type
- ref (subject category)
- art (subject category)
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