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Thermal expansion and steam oxidation of uranium mononitride analysed via in situ neutron diffraction

Liu, Jiatu (author)
UNSW, Sch Mech & Mfg Engn, Sydney, NSW 2033, Australia.
Gasparrini, Claudia (author)
UNSW, Sch Mech & Mfg Engn, Sydney, NSW 2033, Australia.;Imperial Coll London, Dept Mat, Exhibit Rd, London SW 7 2AZ, England.;Imperial Coll London, Ctr Nucl Engn, Exhibit Rd, London SW 7 2AZ, England.
White, Joshua T. (author)
Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM USA.
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Johnson, Kyle (author)
KTH,Kärnenergiteknik
Lopes, Denise Adorno (author)
KTH,Kärnenergiteknik
Peterson, Vanessa K. (author)
Australian Nucl Sci & Technol Org, Locked Bag 2001, Kirrawee Dc, NSW 2232, Australia.;Univ Wollongong, Sch Mech Mat & Mechatron Engn, Wollongong, NSW 2522, Australia.
Studer, Andrew (author)
Australian Nucl Sci & Technol Org, Locked Bag 2001, Kirrawee Dc, NSW 2232, Australia.
Griffiths, Grant J. (author)
Australian Nucl Sci & Technol Org, Locked Bag 2001, Kirrawee Dc, NSW 2232, Australia.
Lumpkin, Gregory R. (author)
Australian Nucl Sci & Technol Org, Locked Bag 2001, Kirrawee Dc, NSW 2232, Australia.
Wenman, Mark R. (author)
Imperial Coll London, Dept Mat, Exhibit Rd, London SW 7 2AZ, England.;Imperial Coll London, Ctr Nucl Engn, Exhibit Rd, London SW 7 2AZ, England.
Burr, Patrick A. (author)
UNSW, Sch Mech & Mfg Engn, Sydney, NSW 2033, Australia.
Sooby, Elizabeth S. (author)
Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA.
Obbard, Edward G. (author)
UNSW, Sch Mech & Mfg Engn, Sydney, NSW 2033, Australia.
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UNSW, Sch Mech & Mfg Engn, Sydney, NSW 2033, Australia UNSW, Sch Mech & Mfg Engn, Sydney, NSW 2033, Australia.;Imperial Coll London, Dept Mat, Exhibit Rd, London SW 7 2AZ, England.;Imperial Coll London, Ctr Nucl Engn, Exhibit Rd, London SW 7 2AZ, England. (creator_code:org_t)
Elsevier BV, 2023
2023
English.
In: Journal of Nuclear Materials. - : Elsevier BV. - 0022-3115 .- 1873-4820. ; 575, s. 154215-
Related links:
https://urn.kb.se/re...
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https://doi.org/10.1...
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  • Journal article (peer-reviewed)
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  • In situ neutron powder diffraction experiments are applied to physical, kinetic, and microstructural characterization of uranium mononitride as a promising light water reactor fuel material. The temperaturevariable coefficient of thermal expansion and isotropic Debye Waller factors are obtained by sequential Rietveld refinement over 499-1873 K. Oxidation of a UN pellet (95.2% density) under flow of 11 mg/min D 2 O is observed to initiate above 623 K and the rate increases by a factor of approximately 10 from 673 to 773 K, with activation energy 50.6 +/- 1.3 kJ/mol; uranium oxide is the only solid corrosion product.Crown Copyright

Subject headings

NATURVETENSKAP  -- Kemi -- Materialkemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences -- Materials Chemistry (hsv//eng)

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ref (subject category)
art (subject category)

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