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Rational molecular ...
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Xu, Weidong,1988-Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten,Key Laboratory of Flexible Electronics (KLOFE) and Institute of Advanced Materials (IAM), Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), Nanjing Tech University (NanjingTech), Nanjing, China
(author)
Rational molecular passivation for high-performance perovskite light-emitting diodes
- Article/chapterEnglish2019
Publisher, publication year, extent ...
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2019-03-25
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Springer Nature Publishing AG,2019
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electronicrdacarrier
Numbers
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LIBRIS-ID:oai:DiVA.org:liu-157707
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https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-157707URI
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https://doi.org/10.1038/s41566-019-0390-xDOI
Supplementary language notes
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Language:English
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Summary in:English
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Subject category:ref swepub-contenttype
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Subject category:art swepub-publicationtype
Notes
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Funding agencies: ERC Starting Grant [717026]; National Basic Research Program of China (973 Program) [2015CB932200]; National Natural Science Foundation of China [61704077, 51572016, 51721001, 61634001, 61725502, 91733302, U1530401]; Natural Science Foundation of Jiangsu
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A major efficiency limit for solution-processed perovskite optoelectronic devices, for example light-emitting diodes, is trap-mediated non-radiative losses. Defect passivation using organic molecules has been identified as an attractive approach to tackle this issue. However, implementation of this approach has been hindered by a lack of deep understanding of how the molecular structures influence the effectiveness of passivation. We show that the so far largely ignored hydrogen bonds play a critical role in affecting the passivation. By weakening the hydrogen bonding between the passivating functional moieties and the organic cation featuring in the perovskite, we significantly enhance the interaction with defect sites and minimize non-radiative recombination losses. Consequently, we achieve exceptionally high-performance near-infrared perovskite light-emitting diodes with a record external quantum efficiency of 21.6%. In addition, our passivated perovskite light-emitting diodes maintain a high external quantum efficiency of 20.1% and a wall-plug efficiency of 11.0% at a high current density of 200 mA cm−2, making them more attractive than the most efficient organic and quantum-dot light-emitting diodes at high excitations.
Subject headings and genre
Added entries (persons, corporate bodies, meetings, titles ...)
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Hu, QiKey Laboratory of Flexible Electronics (KLOFE) and Institute of Advanced Materials (IAM), Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), Nanjing Tech University (NanjingTech), Nanjing, China
(author)
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Bai, Sai,1988-Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten(Swepub:liu)saiba14
(author)
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Bao, Chunxiong,1986-Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten,International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology, Shenzhen University, Shenzhen, China(Swepub:liu)chuba17
(author)
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Miao, YanfengKey Laboratory of Flexible Electronics (KLOFE) and Institute of Advanced Materials (IAM), Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), Nanjing Tech University (NanjingTech), Nanjing, China
(author)
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Yuan, Zhongcheng,1989-Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten(Swepub:liu)zhoyu49
(author)
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Borzda, TetianaCenter for Nano Science and Technology @Polimi, Istituto Italiano di Tecnologia, Milan, Italy
(author)
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Barker, Alex J.Center for Nano Science and Technology @Polimi, Istituto Italiano di Tecnologia, Milan, Italy
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Tyukalova, ElizavetaSchool of Materials Science and Engineering, Nanyang Technological University (NTU), Singapore, Singapore
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Hu, Zhang-Jun,Dr.1978-Linköpings universitet,Molekylär ytfysik och nanovetenskap,Tekniska fakulteten(Swepub:liu)zhahu14
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Kawecki, MaciejLaboratory for Nanoscale Materials Science, Empa, Dubendorf, Switzerland; Department of Physics, University of Basel, Basel, Switzerland
(author)
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Wang, Heyong,1989-Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten(Swepub:liu)heywa58
(author)
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Yan, Zhibo,1980-Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten,Laboratory of Solid State Microstructures and Innovation Center of Advanced Microstructures, Nanjing University, Nanjing, P. R. China(Swepub:liu)zhiya29
(author)
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Liu, Xianjie,Ph.D.1971-Linköpings universitet,Ytors Fysik och Kemi,Tekniska fakulteten(Swepub:liu)xiali21
(author)
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Shi, Xiaobo,1987-Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten(Swepub:liu)xiash13
(author)
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Uvdal, Kajsa,1961-Linköpings universitet,Molekylär ytfysik och nanovetenskap,Tekniska fakulteten(Swepub:liu)kajuv09
(author)
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Fahlman, Mats,1967-Linköpings universitet,Ytors Fysik och Kemi,Tekniska fakulteten(Swepub:liu)matfa21
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Zhang, WenjingInternational Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology, Shenzhen University, Shenzhen, China
(author)
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Duchamp, MartialSchool of Materials Science and Engineering, Nanyang Technological University (NTU), Singapore, Singapore
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Liu, Jun-MingLaboratory of Solid State Microstructures and Innovation Center of Advanced Microstructures, Nanjing University, Nanjing, P. R. China
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Petrozza, AnnamariaCenter for Nano Science and Technology @Polimi, Istituto Italiano di Tecnologia, Milan, Italy
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Wang, JianpuKey Laboratory of Flexible Electronics (KLOFE) and Institute of Advanced Materials (IAM), Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), Nanjing Tech University (NanjingTech), Nanjing, China
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Liu, Li-MinBeijing Computational Science Research Center, Beijing, China; School of Physics, Beihang University, Beijing, China
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Huang, WeiKey Laboratory of Flexible Electronics (KLOFE) and Institute of Advanced Materials (IAM), Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), Nanjing Tech University (NanjingTech), Nanjing, China; Shaanxi Institute of Flexible Electronics (SIFE), Northwestern Polytechnical University (NPU), Xi’an, China
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Gao, Feng,1981-Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten(Swepub:liu)fenga88
(author)
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Linköpings universitetBiomolekylär och Organisk Elektronik
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In:Nature Photonics: Springer Nature Publishing AG13:6, s. 418-4241749-48851749-4893
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Xu, Weidong, 198 ...
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Hu, Qi
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Bai, Sai, 1988-
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Bao, Chunxiong, ...
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Miao, Yanfeng
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Yuan, Zhongcheng ...
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Borzda, Tetiana
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Barker, Alex J.
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Tyukalova, Eliza ...
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Hu, Zhang-Jun, D ...
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Kawecki, Maciej
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Wang, Heyong, 19 ...
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Yan, Zhibo, 1980 ...
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Liu, Xianjie, Ph ...
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Shi, Xiaobo, 198 ...
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Uvdal, Kajsa, 19 ...
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Fahlman, Mats, 1 ...
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Zhang, Wenjing
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Duchamp, Martial
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Liu, Jun-Ming
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Petrozza, Annama ...
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Wang, Jianpu
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Liu, Li-Min
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Huang, Wei
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Gao, Feng, 1981-
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