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Band-to-band transitions and critical points in the near-infrared to vacuum ultraviolet dielectric functions of single crystal urania and thoria

Mock, Alyssa (author)
Linköpings universitet,Halvledarmaterial,Tekniska fakulteten,Univ Nebraska, NE 68588 USA
Dugan, Christina (author)
US Air Force, OH 45433 USA
Knight, Sean (author)
Univ Nebraska, NE 68588 USA
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Korlacki, Rafal (author)
Univ Nebraska, NE 68588 USA
Mann, J. Matthew (author)
US Air Force, OH 45433 USA
Kimani, Martin M. (author)
US Air Force, OH 45433 USA; KBRwyle, OH 45431 USA
Petrosky, James C. (author)
US Air Force, OH 45433 USA
Dowben, Peter A. (author)
Univ Nebraska, NE 68588 USA
Schubert, Mathias (author)
Linköpings universitet,Halvledarmaterial,Tekniska fakulteten,Univ Nebraska, NE 68588 USA; Leibniz Inst Polymer Res Dresden, Germany
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 (creator_code:org_t)
AMER INST PHYSICS, 2019
2019
English.
In: Applied Physics Letters. - : AMER INST PHYSICS. - 0003-6951 .- 1077-3118. ; 114:21
  • Journal article (peer-reviewed)
Abstract Subject headings
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  • Band-to-band transition energy parameters for single-crystal actinide samples of uranium oxide and thorium oxide were determined and compared using spectroscopic ellipsometry and critical-point dielectric function analyses. Spectroscopic ellipsometry measurements from the near-infrared to the vacuum ultraviolet spectral region were used to determine the dielectric functions of uranium oxide and thorium oxide. The critical-point structure is similar between UO2 and ThO2 but strongly blue shifted for ThO2. We find bandgap energies of 2.1eV and 5.4eV for UO2 and ThO2, respectively.

Subject headings

NATURVETENSKAP  -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)

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