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Microfluidic-Assist...
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Rodriguez-Martinez, XabierCSIC, Spain
(author)
Microfluidic-Assisted Blade Coating of Compositional Libraries for Combinatorial Applications: The Case of Organic Photovoltaics
- Article/chapterEnglish2020
Publisher, publication year, extent ...
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2020-07-23
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WILEY-V C H VERLAG GMBH,2020
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electronicrdacarrier
Numbers
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LIBRIS-ID:oai:DiVA.org:liu-168551
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https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-168551URI
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https://doi.org/10.1002/aenm.202001308DOI
Supplementary language notes
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Language:English
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Summary in:English
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Subject category:ref swepub-contenttype
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Subject category:art swepub-publicationtype
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Funding Agencies|Spanish Ministry of Economy, Industry and Competitiveness through the "Severo Ochoa" Programme for Centers of Excellence in RD [SEV-2015-0496, PGC2018-095411-B-I00]; European Research Council (ERC)European Research Council (ERC) [648901]; European Research Council Starting Grant microCrysFact (ERC-2015-STG) [677020]; Swiss National Science FoundationSwiss National Science Foundation (SNSF) [200021_181988]; ETH ZurichETH Zurich; Generalitat de CatalunyaGeneralitat de Catalunya; COFUND programme of the Marie Curie Actions of the 7th R&D Framework Programme of the European Union [BP-B 00256]
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Microfluidic technologies are highly adept at generating controllable compositional gradients in fluids, a feature that has accelerated the understanding of the importance of chemical gradients in biological processes. That said, the development of versatile methods to generate controllable compositional gradients in the solid-state has been far more elusive. The ability to produce such gradients would provide access to extensive compositional libraries, thus enabling the high-throughput exploration of the parametric landscape of functional solids and devices in a resource-, time-, and cost-efficient manner. Herein, the synergic integration of microfluidic technologies is reported with blade coating to enable the controlled formation of compositional lateral gradients in solution. Subsequently, the transformation of liquid-based compositional gradients into solid-state thin films using this method is demonstrated. To demonstrate efficacy of the approach, microfluidic-assisted blade coating is used to optimize blending ratios in organic solar cells. Importantly, this novel technology can be easily extended to other solution processable systems that require the formation of solid-state compositional lateral gradients.
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Sevim, SemihSwiss Fed Inst Technol, Switzerland
(author)
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Xu, XiaofengLinköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten,Ocean Univ China, Peoples R China(Swepub:liu)xiaxu02
(author)
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Franco, CarlosSwiss Fed Inst Technol, Switzerland
(author)
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Pamies-Puig, PaulaCSIC, Spain
(author)
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Corcoles-Guija, LauraCSIC, Spain
(author)
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Rodriguez-Trujillo, RomenCSIC, Spain; Univ Barcelona, Spain
(author)
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Javier del Campo, FranciscoEsfera UAB, Spain; Univ Basque Country, Spain; Ikerbasque, Spain
(author)
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Rodriguez San Miguel, DavidSwiss Fed Inst Technol, Switzerland
(author)
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deMello, Andrew J.Swiss Fed Inst Technol, Switzerland
(author)
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Pane, SalvadorSwiss Fed Inst Technol, Switzerland
(author)
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Amabilino, David B.Univ Nottingham, England
(author)
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Inganäs, OlleLinköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten(Swepub:liu)ollin59
(author)
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Puigmarti-Luis, JosepSwiss Fed Inst Technol, Switzerland
(author)
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Campoy-Quiles, MarianoCSIC, Spain
(author)
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CSIC, SpainSwiss Fed Inst Technol, Switzerland
(creator_code:org_t)
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In:Advanced Energy Materials: WILEY-V C H VERLAG GMBH10:331614-68321614-6840
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