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Synthesis of MAX phases Nb2CuC and Ti2(Al0.1Cu0.9)N by A-site replacement reaction in molten salts

Ding, Haoming (author)
State Key Laboratory for Mechanical Behavior of Materials, Xi’an Jiaotong University, Xi’an, People’s Republic of China; bEngineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, People’s Republic of China
Li, Youbing (author)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, People’s Republic of China; University of Chinese Academy of Sciences, Beijing, People’s Republic of China
Lu, Jun (author)
Linköpings universitet,Tunnfilmsfysik,Tekniska fakulteten
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Luo, Kan (author)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, People’s Republic of China
Chen, Ke (author)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, People’s Republic of China
Li, Mian (author)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, People’s Republic of China
Persson, Per O. Å., 1971- (author)
Linköpings universitet,Tunnfilmsfysik,Tekniska fakulteten
Hultman, Lars, Professor, 1960- (author)
Linköpings universitet,Tunnfilmsfysik,Tekniska fakulteten
Eklund, Per, Docent, 1977- (author)
Linköpings universitet,Tunnfilmsfysik,Tekniska fakulteten
Du, Shiyu (author)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, People’s Republic of China
Huang, Zhengren (author)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, People’s Republic of China
Chai, Zhifang (author)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, People’s Republic of China
Wang, Hongjie (author)
State Key Laboratory for Mechanical Behavior of Materials, Xi’an Jiaotong University, Xi’an, People’s Republic of China
Huang, Ping (author)
aState Key Laboratory for Mechanical Behavior of Materials, Xi’an Jiaotong University, Xi’an, People’s Republic of China
Huang, Qing (author)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, People’s Republic of China
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 (creator_code:org_t)
2019-10-01
2019
English.
In: Materials Research Letters. - : Taylor & Francis. - 2166-3831. ; 7:12, s. 510-516
Related links:
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https://doi.org/10.1...
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  • Journal article (peer-reviewed)
Abstract Subject headings
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  • New MAX phases Ti2(AlxCu1−x)N and Nb2CuC were synthesized by A-site replacement by reacting Ti2AlN and Nb2AlC, respectively, with CuCl2 or CuI molten salt. X-ray diffraction, scanning electron microscopy, and atomically resolved scanning transmission electron microscopy showed complete A-site replacement in Nb2AlC, which lead to the formation of Nb2CuC. However, the replacement of Al in Ti2AlN phase was only close to complete at Ti2(Al0.1Cu0.9)N. Density-functional theory calculations corroborated the structural stability of Nb2CuC and Ti2CuN phases. Moreover, the calculated cleavage energy in these Cu-containing MAX phases are weaker than in their Al-containing counterparts.The preparation of MAX phases Nb2CuC and Ti2(Al0.1Cu0.9)N were realized by A-site replacement in Ti2AlN and Nb2AlN, respectively.

Subject headings

NATURVETENSKAP  -- Fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences (hsv//eng)

Keyword

MAX phase
replacement reaction
copper
density-functional theory

Publication and Content Type

ref (subject category)
art (subject category)

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