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An n-n Heterojuncti...
An n-n Heterojunction Configuration for Efficient Electron Transport in Organic Photovoltaic Devices
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- Li, Yaohui (author)
- Jinan Univ, Peoples R China
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- Wu, Xiang (author)
- Jinan Univ, Peoples R China
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- Zuo, Guangzheng (author)
- Fudan Univ, Peoples R China
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- Wang, Yufei (author)
- Jinan Univ, Peoples R China
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- Liu, Xianjie, 1971- (author)
- Linköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten
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- Ma, Yanxian (author)
- South China Univ Technol, Peoples R China
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- Li, Bolun (author)
- Jinan Univ, Peoples R China
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- Zhu, Xu-Hui (author)
- South China Univ Technol, Peoples R China
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- Wu, Hongbin (author)
- South China Univ Technol, Peoples R China
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- Qing, Jian (author)
- Jinan Univ, Peoples R China
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- Hou, Lintao (author)
- Jinan Univ, Peoples R China
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- Cai, Wanzhu (author)
- Jinan Univ, Peoples R China
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(creator_code:org_t)
- 2022-12-21
- 2023
- English.
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In: Advanced Functional Materials. - : WILEY-V C H VERLAG GMBH. - 1616-301X .- 1616-3028. ; 33:9
- Related links:
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
Subject headings
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- Selective electron transport and extraction are essential to the operation of photovoltaic devices. Electron transport layer (ETL) is therefore critical to organic photovoltaics (OPV). Herein, an ETL configuration is presented comprising a solution-processed n-n organic heterojunction to enhance electron transport and hole blocking, and boost power conversion efficiency (PCE) in OPV. Specifically, the n-n heterojunction is constructed by stacking a narrow-band n-type conjugated polymer layer (PNDIT-F3N) and a wide-band n-type conjugated molecule layer (Phen-NaDPO). Based on the ultraviolet photoelectron spectroscopy measurement and numerical simulation of current density-voltage characteristics, the formation of the built-in potential is investigated. In three OPVs with different active layers, substantial improvements are observed in performance following the introduction of this ETL configuration. The performance enhancement arises from the combination of selective carrier transport properties and reduced recombination. Another contributing factor is the good film-forming quality of the new ETL configuration, where the surface energies of the related materials are well-matched. The n-n organic heterojunction represents a viable and promising ETL construction strategy for efficient OPV devices.
Subject headings
- NATURVETENSKAP -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Condensed Matter Physics (hsv//eng)
Keyword
- electron transport layers; n-n heterojunctions; organic photovoltaic devices; selective carrier transports
Publication and Content Type
- ref (subject category)
- art (subject category)
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- By the author/editor
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Li, Yaohui
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Wu, Xiang
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Zuo, Guangzheng
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Wang, Yufei
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Liu, Xianjie, 19 ...
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Ma, Yanxian
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show more...
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Li, Bolun
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Zhu, Xu-Hui
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Wu, Hongbin
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Qing, Jian
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Hou, Lintao
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Cai, Wanzhu
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show less...
- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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and Condensed Matter ...
- Articles in the publication
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Advanced Functio ...
- By the university
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Linköping University