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Origins of the open...
Origins of the open-circuit voltage in ternary organic solar cells and design rules for minimized voltage losses
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- Wang, Yuming (author)
- Linköpings universitet,Elektroniska och fotoniska material,Tekniska fakulteten,Hasselt Univ, Belgium; IMEC, Belgium,Linköping University,Universiteit Hasselt
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- Yu, Jianwei (author)
- Linköpings universitet,Elektroniska och fotoniska material,Tekniska fakulteten,Linköping University
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- Zhang, Rui (author)
- Linköpings universitet,Elektroniska och fotoniska material,Tekniska fakulteten,Linköping University
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- Yuan, Jun (author)
- Linköpings universitet,Elektroniska och fotoniska material,Tekniska fakulteten,Cent South Univ, Peoples R China,Linköping University,Central South University
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- Hultmark, Sandra, 1994 (author)
- Chalmers Univ Technol, Sweden,Chalmers tekniska högskola,Chalmers University of Technology
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- Johnson, Catherine E. (author)
- Imperial Coll London, England,Imperial College of Science, Technology and Medicine
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- Gallop, Nathaniel P. (author)
- Imperial Coll London, England,Imperial College of Science, Technology and Medicine
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- Siegmund, Bernhard (author)
- Hasselt Univ, Belgium; IMEC, Belgium,Universiteit Hasselt
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- Qian, Deping (author)
- Linköpings universitet,Elektroniska och fotoniska material,Tekniska fakulteten,Linköping University
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- Zhang, Huotian (author)
- Linköpings universitet,Elektroniska och fotoniska material,Tekniska fakulteten,Linköping University
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- Zou, Yingping (author)
- Cent South Univ, Peoples R China,Central South University
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- Kemerink, Martijn (author)
- Linköpings universitet,Elektroniska och fotoniska material,Tekniska fakulteten,Heidelberg Univ, Germany,Ruprecht-Karls-Universität Heidelberg,Heidelberg University,Linköping University
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- Bakulin, Artem A. (author)
- Imperial Coll London, England,Imperial College of Science, Technology and Medicine
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- Müller, Christian, 1980 (author)
- Chalmers Univ Technol, Sweden,Chalmers tekniska högskola,Chalmers University of Technology
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- Vandewal, Koen (author)
- Hasselt Univ, Belgium; IMEC, Belgium,Universiteit Hasselt
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- Chen, Xian-Kai (author)
- Soochow Univ, Peoples R China; Soochow Univ, Peoples R China,Soochow University
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- Gao, Feng (author)
- Linköpings universitet,Elektroniska och fotoniska material,Tekniska fakulteten,Linköping University
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(creator_code:org_t)
- NATURE PORTFOLIO, 2023
- 2023
- English.
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In: Nature Energy. - : NATURE PORTFOLIO. - 2058-7546. ; 8:9, s. 978-988
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Abstract
Subject headings
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- The power conversion efficiency of ternary organic solar cells (TOSCs), consisting of one host binary blend and one guest component, remains limited by large voltage losses. The fundamental understanding of the open-circuit voltage (V-OC) in TOSCs is controversial, limiting rational design of the guest component. In this study, we systematically investigate how the guest component affects the radiative and non-radiative related parts of V-OC of a series of TOSCs using the detailed balanced principle. We highlight that the thermal population of charge-transfer and local exciton states provided by the guest binary blend (that is, the guest-component-based binary blend) has a significant influence on the non-radiative voltage losses. Ultimately, we provide two design rules for enhancing the V-OC in TOSCs: high emission yield for the guest binary blend and similar charge-transfer-state energies for host/guest binary blends; high miscibility of the guest component with the low gap component in the host binary blend. The performance of ternary organic solar cells is limited by voltage losses. Using the detailed balance principle, Wang et al. show how the third component of the blend affects the open-circuit voltage and delineate molecular design rules.
Subject headings
- TEKNIK OCH TEKNOLOGIER -- Elektroteknik och elektronik -- Annan elektroteknik och elektronik (hsv//swe)
- ENGINEERING AND TECHNOLOGY -- Electrical Engineering, Electronic Engineering, Information Engineering -- Other Electrical Engineering, Electronic Engineering, Information Engineering (hsv//eng)
- TEKNIK OCH TEKNOLOGIER -- Maskinteknik -- Energiteknik (hsv//swe)
- ENGINEERING AND TECHNOLOGY -- Mechanical Engineering -- Energy Engineering (hsv//eng)
Publication and Content Type
- ref (subject category)
- art (subject category)
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- By the author/editor
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Wang, Yuming
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Yu, Jianwei
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Zhang, Rui
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Yuan, Jun
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Hultmark, Sandra ...
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Johnson, Catheri ...
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show more...
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Gallop, Nathanie ...
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Siegmund, Bernha ...
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Qian, Deping
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Zhang, Huotian
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Zou, Yingping
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Kemerink, Martij ...
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Bakulin, Artem A ...
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Müller, Christia ...
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Vandewal, Koen
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Chen, Xian-Kai
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Gao, Feng
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show less...
- About the subject
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- ENGINEERING AND TECHNOLOGY
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ENGINEERING AND ...
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and Electrical Engin ...
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and Other Electrical ...
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- ENGINEERING AND TECHNOLOGY
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ENGINEERING AND ...
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and Mechanical Engin ...
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and Energy Engineeri ...
- Articles in the publication
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Nature Energy
- By the university
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Linköping University
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Chalmers University of Technology