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a A Resistance-Swit...
a A Resistance-Switchable and Ferroelectric Metal Organic Framework
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Pan, Liang (author)
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Liu, Gang (author)
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Li, Hui (author)
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Meng, Sheng (author)
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Han, Lei (author)
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Shang, Jie (author)
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Chen, Bin (author)
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- Platero-Prats, Ana E. (author)
- Stockholms universitet,Avdelningen för oorganisk kemi och strukturkemi
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Lu, Wei (author)
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- Zou, Xiaodong (author)
- Stockholms universitet,Avdelningen för oorganisk kemi och strukturkemi
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Li, Run-Wei (author)
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(creator_code:org_t)
- 2014-12-03
- 2014
- English.
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In: Journal of the American Chemical Society. - : American Chemical Society (ACS). - 0002-7863 .- 1520-5126. ; 136:50, s. 17477-17483
- Related links:
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
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- The ever-emerging demands on miniaturization of electronic devices have pushed the development of innovative materials with desired properties. One major endeavor is the development of organic- or organic-inorganic hybrid-based electronics as alternatives or supplements to silicon-based devices. Herein we report the first observation of the coexistence of resistance switching and ferroelectricity in a metal-organic framework (MOF) material, [InC16H11N2O8]center dot 1.5H(2)O, denoted as RSMOF-1. The electrical resistance of RSMOF-1 can be turned on and off repeatedly with a current ratio of 30. A first-principles molecular dynamics simulation suggests that the resistive switching effect is related to the ferroelectric transition of N center dot center dot center dot H-O center dot center dot center dot H-N bridge-structured dipoles of the guest water molecules and the amino-tethered MOF nanochannel. The discovery of the resistive switching effect and ferroelectricity in MOFs offers great potential for the physical implementation of novel electronics for next-generation digital processing and communication.
Subject headings
- NATURVETENSKAP -- Kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences (hsv//eng)
Publication and Content Type
- ref (subject category)
- art (subject category)
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- By the author/editor
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Pan, Liang
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Liu, Gang
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Li, Hui
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Meng, Sheng
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Han, Lei
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Shang, Jie
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show more...
-
Chen, Bin
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Platero-Prats, A ...
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Lu, Wei
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Zou, Xiaodong
-
Li, Run-Wei
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show less...
- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Chemical Science ...
- Articles in the publication
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Journal of the A ...
- By the university
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Stockholm University