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Nanoscale Transient Magnetization Gratings Created and Probed by Femtosecond Extreme Ultraviolet Pulses

Ksenzov, Dmitriy (author)
Maznev, Alexei A. (author)
Unikandanunni, Vivek (author)
Stockholms universitet,Fysikum
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Bencivenga, Filippo (author)
Capotondi, Flavio (author)
Caretta, Antonio (author)
Foglia, Laura (author)
Malvestuto, Marco (author)
Masciovecchio, Claudio (author)
Mincigrucci, Riccardo (author)
Nelson, Keith A. (author)
Pancaldi, Matteo (author)
Stockholms universitet,Fysikum
Pedersoli, Emanuele (author)
Randolph, Lisa (author)
Rahmann, Hendrik (author)
Urazhdin, Sergei (author)
Bonetti, Stefano (author)
Stockholms universitet,Fysikum,Ca’ Foscari University of Venice, Italy
Gutt, Christian (author)
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 (creator_code:org_t)
2021-03-16
2021
English.
In: Nano Letters. - : American Chemical Society (ACS). - 1530-6984 .- 1530-6992. ; 21:7, s. 2905-2911
  • Journal article (peer-reviewed)
Abstract Subject headings
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  • We utilize coherent femtosecond extreme ultraviolet (EUV) pulses from a free electron laser (FEL) to generate transient periodic magnetization patterns with periods as short as 44 nm. Combining spatially periodic excitation with resonant probing at the M-edge of cobalt allows us to create and probe transient gratings of electronic and magnetic excitations in a CoGd alloy. In a demagnetized sample, we observe an electronic excitation with a rise time close to the FEL pulse duration and similar to 0.5 ps decay time indicative of electron-phonon relaxation. When the sample is magnetized to saturation in an external field, we observe a magnetization grating, which appears on a subpicosecond time scale as the sample is demagnetized at the maxima of the EUV intensity and then decays on the time scale of tens of picoseconds via thermal diffusion. The described approach opens multiple avenues for studying dynamics of ultrafast magnetic phenomena on nanometer length scales.

Subject headings

NATURVETENSKAP  -- Fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences (hsv//eng)

Keyword

spin
X-rays
free-electron laser
membranes
heat transfer
nanoscale
magnetism
time-resolved imaging
transient grating

Publication and Content Type

ref (subject category)
art (subject category)

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