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Electronic coupling between the unoccupied states of the organic and inorganic sublattices of methylammonium lead iodide : A hybrid organic-inorganic perovskite single crystal

Man, Gabriel (author)
Uppsala universitet,Energimaterialens fysik,Uppsala Univ, Condensed Matter Phys Energy Mat, Div Xray Photon Sci, Dept Phys & Astron, Box 516, S-75121 Uppsala, Sweden.
Sterling, Cody M. (author)
Stockholms universitet,Fysikum,Stockholm Univ, Dept Phys, AlbaNova Univ Ctr, S-10691 Stockholm, Sweden.
Kamal, Chinnathambi (author)
Stockholms universitet,Fysikum,Raja Ramanna Centre for Advanced Technology, India,Stockholm Univ, Dept Phys, AlbaNova Univ Ctr, S-10691 Stockholm, Sweden.;Raja Ramanna Ctr Adv Technol, Theory & Simulat Lab, HRDS, Indore 452013, India.
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Simonov, Konstantin, 1988- (author)
Uppsala universitet,Energimaterialens fysik,Uppsala Univ, Condensed Matter Phys Energy Mat, Div Xray Photon Sci, Dept Phys & Astron, Box 516, S-75121 Uppsala, Sweden.;Swerim AB, S-16407 Stockholm, Sweden.
Svanström, Sebastian (author)
Uppsala universitet,Energimaterialens fysik,Uppsala Univ, Condensed Matter Phys Energy Mat, Div Xray Photon Sci, Dept Phys & Astron, Box 516, S-75121 Uppsala, Sweden.
Acharya, Joydev (author)
Tata Inst Fundamental Res, TIFR Ctr Interdisciplinary Sci, 36-P Gopanpally Village, Hyderabad 500046, India.
Johansson, Fredrik O. L. (author)
Uppsala universitet,Energimaterialens fysik,Uppsala Univ, Condensed Matter Phys Energy Mat, Div Xray Photon Sci, Dept Phys & Astron, Box 516, S-75121 Uppsala, Sweden.
Giangrisostomi, Erika (author)
Helmholtz Zentrum Berlin GmbH, Inst Methods & Instrumentat Synchrotron Radiat Re, Albert Einstein Str 15, D-12489 Berlin, Germany.
Ovsyannikov, Ruslan (author)
Helmholtz Zentrum Berlin GmbH, Inst Methods & Instrumentat Synchrotron Radiat Re, Albert Einstein Str 15, D-12489 Berlin, Germany.
Huthwelker, Thomas (author)
Paul Scherrer Inst, WLGA 212,Forschungsstr 111, CH-5232 Villigen, Switzerland.
Butorin, Sergei (author)
Uppsala universitet,Energimaterialens fysik,Uppsala Univ, Condensed Matter Phys Energy Mat, Div Xray Photon Sci, Dept Phys & Astron, Box 516, S-75121 Uppsala, Sweden.
Nayak, Pabitra K. (author)
Tata Inst Fundamental Res, TIFR Ctr Interdisciplinary Sci, 36-P Gopanpally Village, Hyderabad 500046, India.
Odelius, Michael (author)
Stockholms universitet,Fysikum,Stockholm Univ, Dept Phys, AlbaNova Univ Ctr, S-10691 Stockholm, Sweden.
Rensmo, Håkan (author)
Uppsala universitet,Energimaterialens fysik,Uppsala Univ, Condensed Matter Phys Energy Mat, Div Xray Photon Sci, Dept Phys & Astron, Box 516, S-75121 Uppsala, Sweden.
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American Physical Society, 2021
2021
English.
In: Physical Review B. - : American Physical Society. - 2469-9950 .- 2469-9969. ; 104:4
Related links:
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https://uu.diva-port... (primary) (Raw object)
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  • Journal article (peer-reviewed)
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  • Organic-inorganic halide perovskites have been intensively reinvestigated due to their applications, yet the optoelectronic function of the organic cation remains unclear. Through organic-selective resonant Auger electron spectroscopy measurements on well-defined single-crystal surfaces, we find evidence for electronic coupling in the unoccupied states between the organic and inorganic sublattices of the prototypical hybrid perovskite, which is contrary to the notion based on previous studies that the organic cation is electronically inert. The coupling is relevant for electron dynamics in the material and for understanding optoelectronic functionality.

Subject headings

NATURVETENSKAP  -- Kemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences (hsv//eng)
NATURVETENSKAP  -- Fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences (hsv//eng)
NATURVETENSKAP  -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Condensed Matter Physics (hsv//eng)

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