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Stimulated resonant inelastic X-ray scattering in a solid

Higley, Daniel J. (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.;Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA.
Chen, Zhao (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.;Stanford Univ, Dept Phys, Stanford, CA 94305 USA.
Beye, Martin (author)
DESY, Notkestr 85, D-22607 Hamburg, Germany.
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Hantschmann, Markus (author)
Univ Potsdam, Inst Phys & Astron, Karl Liebnecht Str 24-25, D-14476 Potsdam, Germany.;Helmholtz Zentrum Berlin Mat & Energie GmbH, Inst Methods & Instrumentat Synchrotron Radiat Re, Albert Einstein Str 15, D-12489 Berlin, Germany.
Reid, Alex H. (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.
Mehta, Virat (author)
HGST, San Jose Res Ctr, 3403 Yerba Buena Rd, San Jose, CA 95135 USA.
Hellwig, Olav (author)
HGST, San Jose Res Ctr, 3403 Yerba Buena Rd, San Jose, CA 95135 USA.;Tech Univ Chemnitz, Inst Phys, D-09107 Chemnitz, Germany.;Helmholtz Zentrum Dresden Rossendorf, Inst Ion Beam Phys & Mat Res, D-01328 Dresden, Germany.
Dakovski, Georgi L. (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.
Mitra, Ankush (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.;Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England.
Engel, Robin Y. (author)
DESY, Notkestr 85, D-22607 Hamburg, Germany.
Maxwell, Tim (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.
Ding, Yuantao (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.
Bonetti, Stefano (author)
Stockholms universitet,Fysikum,SLAC National Accelerator Laboratory, USA,SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.;Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden.
Bucher, Maximilian (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.
Carron, Sebastian (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.
Chase, Tyler (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.;Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA.
Jal, Emmanuelle (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.;Sorbonne Univ, Lab Chem Phys Matiere & Rayonnement, LCPMR, CNRS, F-75005 Paris, France.
Kukreja, Roopali (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.;Univ Calif Davis, Dept Mat Sci & Engn, Davis, CA 95616 USA.
Liu, Tianmin (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.;Stanford Univ, Dept Phys, Stanford, CA 94305 USA.
Föhlisch, Alexander (author)
Univ Potsdam, Inst Phys & Astron, Karl Liebnecht Str 24-25, D-14476 Potsdam, Germany.;Helmholtz Zentrum Berlin Mat & Energie GmbH, Inst Methods & Instrumentat Synchrotron Radiat Re, Albert Einstein Str 15, D-12489 Berlin, Germany.
Dürr, Hermann (author)
Uppsala universitet,FREIA,SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.
Schlotter, William F. (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.
Stöhr, Joachim (author)
SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.
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SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA;Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.;Stanford Univ, Dept Phys, Stanford, CA 94305 USA. (creator_code:org_t)
2022-04-06
2022
English.
In: Communications Physics. - : Springer Science and Business Media LLC. - 2399-3650. ; 5
  • Journal article (peer-reviewed)
Abstract Subject headings
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  • When materials are exposed to X-ray pulses with sufficiently high intensity, various nonlinear effects can occur. The most fundamental one consists of stimulated electronic decays after resonant absorption of X-rays. Such stimulated decays enhance the number of emitted photons and the emission direction is confined to that of the stimulating incident photons which clone themselves in the process. Here we report the observation of stimulated resonant elastic (REXS) and inelastic (RIXS) X-ray scattering near the cobalt L3 edge in solid Co/Pd multilayer samples. We observe an enhancement of order 106 of the stimulated over the conventional spontaneous RIXS signal into the small acceptance angle of the RIXS spectrometer. We also find that in solids both stimulated REXS and RIXS spectra contain contributions from inelastic electron scattering processes, even for ultrashort 5 fs pulses. Our results reveal the potential and caveats of the development of stimulated RIXS in condensed matter.

Subject headings

NATURVETENSKAP  -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)

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