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An effective PtPdAu...
An effective PtPdAuCuFe/C high-entropy-alloy applied to direct ethylene glycol fuel cells
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Wang, Wei (author)
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Li, Xiang (author)
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Cheng, Yangshuai (author)
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- Zhang, Miao, 1990- (author)
- Stockholms universitet,Institutionen för material- och miljökemi (MMK)
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Zhao, Kai (author)
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Liu, Yuheng (author)
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(creator_code:org_t)
- Elsevier BV, 2023
- 2023
- English.
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In: Journal of the Taiwan Institute of Chemical Engineers / Elsevier. - : Elsevier BV. - 1876-1070 .- 1876-1089. ; 143
- Related links:
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
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- Background: As a promising green energy conversion device, direct ethylene glycol fuel cells (DEGFC) have been widely studied. But high-cost of their catalysts has severely limited large-scale commercial application. Developing economic and effective anodic electrocatalyst is an urgent work presently.Methods: Herein, an efficient high entropy alloy catalyst (HEA, penta-element) was prepared. Then, their catalytic performance and properties were authenticated by some electrochemical and physical methods. Importantly, it was also applied to a real DEGFC stack.Significant findings: Notably, the ethylene glycol oxidation current density (0.65 A mg−1PtPdAu) on as-prepared HEA is three times than that of commercial Pt/C (0.22 A mg−1Pt) with good long-term durability. Moreover, the HEA-equipped DEGFC obtains an open circuit potential of 0.58 V, which delivers 2 times larger peak power density (17.63 mW cm−2) than that of commercial Pt/C (7.37 mW cm−2). This work would be a good reference to developing other advanced HEA materials in electrocatalytic fields.
Subject headings
- TEKNIK OCH TEKNOLOGIER -- Kemiteknik -- Kemiska processer (hsv//swe)
- ENGINEERING AND TECHNOLOGY -- Chemical Engineering -- Chemical Process Engineering (hsv//eng)
Keyword
- High entropy alloy
- Electrocatalyst
- Direct ethylene glycol fuel cell
Publication and Content Type
- ref (subject category)
- art (subject category)
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