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Silica hybrid sol-g...
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Chateau, DenisLaboratoire de Chimie, Université de Lyon, Université Claude Bernard Lyon 1, ENS Lyon, CNRS UMR5182, Lyon 69364, France
(author)
Silica hybrid sol-gel materials with unusually high concentration of Pt-organic molecular guests : Studies of luminescence and nonlinear absorption of light
- Article/chapterEnglish2012
Publisher, publication year, extent ...
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2012-05-04
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Washington :American Chemical Society (ACS),2012
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printrdacarrier
Numbers
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LIBRIS-ID:oai:DiVA.org:umu-54413
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https://urn.kb.se/resolve?urn=urn:nbn:se:umu:diva-54413URI
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https://doi.org/10.1021/am2015537DOI
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Language:English
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Summary in:English
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Subject category:ref swepub-contenttype
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Subject category:art swepub-publicationtype
Notes
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The development of new photonic materials is a key step towards improvement of existing optical devices and for the preparation of a new generation of systems. Therefore synthesis of photonic hybrid materials with a thorough understanding and control of the microstructure-to-properties relationships is crucial. In this perspective, a new preparation method based on fast gelation reactions using simple dispersion of dyes without strong covalent bonding between dye and matrix has been developed. This new sol-gel method is demonstrated through synthesis of monolithic siloxane-based hybrid materials highly doped by various platinum(II) acetylide derivatives. Concentrations of the chromophores as high as 400 mM were obtained and resulted in unprecedented optical power limiting (OPL) performance at 532 nm of the surface-polished solids. Static and time-resolved photoluminescence of the prepared hybrid materials were consistent with both OPL data and previous studies of similar Pt(II) compounds in solution. The impacts of the microstructure and the chemical composition of the matrix on the spectroscopic properties, are discussed.
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Chaput, FredericLaboratoire de Chimie, Université de Lyon, Université Claude Bernard Lyon 1, ENS Lyon, CNRS UMR5182, Lyon 69364, France
(author)
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Lopes, CesarInformation Systems, Swedish Defence Research Agency (FOI), Linköping SE-581 11, Sweden
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Lindgren, MikaelDepartment of Physics, Norwegian University of Science and Technology, Trondheim NO-7491, Norway
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Brännlund, CarlInformation Systems, Swedish Defence Research Agency (FOI), Linköping SE-581 11, Sweden
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Öhgren, JohanInformation Systems, Swedish Defence Research Agency (FOI), Linköping SE-581 11, Sweden
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Djourelov, NikolayInstitut de Physique Nucléaire, Université de Lyon, Université Claude Bernard Lyon 1, CNRS, Villeurbanne, France
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Nedelec, PatrickInstitut de Physique Nucléaire, Université de Lyon, Université Claude Bernard Lyon 1, CNRS, Villeurbanne, France
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Eliasson, Bertil,1954-Umeå universitet,Kemiska institutionen(Swepub:umu)beel0001
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Kindahl, Tomas,1980-Umeå universitet,Kemiska institutionen(Swepub:umu)toskil02
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Lerouge, FredericLaboratoire de Chimie, Université de Lyon, Université Claude Bernard Lyon 1, ENS Lyon, CNRS UMR5182, Lyon 69364, France
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Andraud, ChantalLaboratoire de Chimie, Université de Lyon, Université Claude Bernard Lyon 1, ENS Lyon, CNRS UMR5182, Lyon 69364, France
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Parola, StephaneLaboratoire de Chimie, Université de Lyon, Université Claude Bernard Lyon 1, ENS Lyon, CNRS UMR5182, Lyon 69364, France
(author)
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Laboratoire de Chimie, Université de Lyon, Université Claude Bernard Lyon 1, ENS Lyon, CNRS UMR5182, Lyon 69364, FranceInformation Systems, Swedish Defence Research Agency (FOI), Linköping SE-581 11, Sweden
(creator_code:org_t)
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In:ACS Applied Materials and InterfacesWashington : American Chemical Society (ACS)4:5, s. 2369-23771944-82441944-8252
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Chateau, Denis
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Chaput, Frederic
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Lopes, Cesar
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Lindgren, Mikael
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Brännlund, Carl
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Öhgren, Johan
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Djourelov, Nikol ...
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Nedelec, Patrick
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Lerouge, Frederi ...
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Andraud, Chantal
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Parola, Stephane
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Umeå University