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Pressure-induced transformation and superhard phase in fullerenes : the effect of solvent intercalation
- Yao, Mingguang (author)
- Cui, Wen (author)
- Xiao, Junping (author)
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- Chen, Shuanglong (author)
- Cui, Jinxing (author)
- Liu, Ran (author)
- Cui, Tian (author)
- Zou, Bo (author)
- Liu, Bingbing (author)
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- (creator_code:org_t)
- AIP Publishing, 2013
- 2013
- English.
- In: Applied Physics Letters. - : AIP Publishing. - 0003-6951 .- 1077-3118. ; 103:7, s. 071913-
- Journal article (peer-reviewed)
Abstract
Subject headings
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- We studied the behavior of solvated and desolvated C-60 crystals under pressure by in situ Raman spectroscopy. The pressure-induced bonding change and structural transformation of C60s are similar in the two samples, both undergoing deformation and amorphization. Nevertheless, the high pressure phases of solvated C-60 can indent diamond anvils while that of desolvated C(60)s cannot. Further experiments suggest that the solvents in the solvated C-60 act as both spacers and bridges by forming covalent bonds with neighbors in 3D network at high pressure, and thus, a fraction of fullerenes may preserve the periodic arrangement in spite of their amorphization.
Subject headings
- NATURVETENSKAP -- Fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences (hsv//eng)
Keyword
- Fullerene
- C60
- intercalation
- solvent
- hydrocarbon
- xylene
- high pressure
- diamond anvil cell
- superhard
- fysik
- Physics
Publication and Content Type
- ref (subject category)
- art (subject category)
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- Zou, Bo
- Liu, Bingbing
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- Umeå University
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