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The local structure...
The local structure of small water clusters : imprints on the core-level photoelectron spectrum
- Article/chapterEnglish2009
Publisher, publication year, extent ...
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2009-02-23
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IOP Publishing,2009
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printrdacarrier
Numbers
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LIBRIS-ID:oai:DiVA.org:uu-129866
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https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-129866URI
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https://doi.org/10.1088/0953-4075/42/5/055201DOI
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Language:English
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Summary in:English
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Subject category:ref swepub-contenttype
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Subject category:art swepub-publicationtype
Notes
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We report on an O 1s photoelectron-spectroscopy study of small neutral water clusters produced by adiabatic expansion. The photoelectron spectra were acquired under two different experimental conditions. At intermediate resolution, the cluster signal was characterized by a very broad O 1s peak with a flat top. In the second set of measurements, resolution was significantly increased at the cost of lower count rates. The cluster signal was now partly resolved into a bimodal structure. Extensive theoretical calculations were undertaken to facilitate an interpretation of the spectrum. These results suggest that the bimodal feature may be ascribed to ionization of water molecules in different hydrogen-bonding configurations, more specifically, molecules characterized by donation of either one or both hydrogen atoms in H-bonding.
Subject headings and genre
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Borve, K. J.
(author)
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Winkler, M
(author)
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Harnes, J
(author)
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Saethre, L. J.
(author)
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Lindblad, AUppsala universitet,Fysik V(Swepub:uu)anlin087
(author)
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Bergersen, HUppsala universitet,Fysik V
(author)
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Björneholm, OUppsala universitet,Molekyl- och kondenserade materiens fysik(Swepub:uu)ollebjor
(author)
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Svensson, SUppsala universitet,Fysik V(Swepub:uu)svansven
(author)
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Öhrwall, GUppsala universitet,Fysik V
(author)
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Uppsala universitetFysik V
(creator_code:org_t)
Related titles
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In:Journal of Physics B: IOP Publishing42:5, s. 055201-0953-40751361-6455
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- By the author/editor
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Abu-samha, M
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Borve, K. J.
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Winkler, M
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Harnes, J
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Saethre, L. J.
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Lindblad, A
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Bergersen, H
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Björneholm, O
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Svensson, S
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Öhrwall, G
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- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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Journal of Physi ...
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Uppsala University