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2D to 3D crossover ...
2D to 3D crossover of the magnetic properties in ordered arrays of iron oxide nanocrystals
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- Faure, B. (author)
- Stockholms universitet,Institutionen för material- och miljökemi (MMK)
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- Wetterskog, Erik, 1983- (author)
- Stockholms universitet,Institutionen för material- och miljökemi (MMK)
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- Gunnarsson, Klas (author)
- Uppsala universitet,Fasta tillståndets fysik
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Josten, E. (author)
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Hermann, R. P. (author)
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Brückel, T. (author)
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Andreasen, J. W. (author)
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Meneau, F. (author)
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Meyer, M. (author)
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- Lyubartsev, Alexander (author)
- Stockholms universitet,Institutionen för material- och miljökemi (MMK)
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- Bergström, Lennart (author)
- Stockholms universitet,Institutionen för material- och miljökemi (MMK)
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- Salazar-Alvarez, German (author)
- Stockholms universitet,Institutionen för material- och miljökemi (MMK)
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- Svedlindh, Peter (author)
- Uppsala universitet,Fasta tillståndets fysik
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(creator_code:org_t)
- 2013
- 2013
- English.
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In: Nanoscale. - : Royal Society of Chemistry (RSC). - 2040-3364 .- 2040-3372. ; 5:3, s. 953-960
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https://pubs.rsc.org...
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https://urn.kb.se/re...
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https://doi.org/10.1...
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https://urn.kb.se/re...
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Abstract
Subject headings
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- The magnetic 2D to 3D crossover behavior of well-ordered arrays of monodomain γ-Fe2O3 spherical nanoparticles with different thicknesses has been investigated by magnetometry and Monte Carlo (MC) simulations. Using the structural information of the arrays obtained from grazing incidence small-angle X-ray scattering and scanning electron microscopy together with the experimentally determined values for the saturation magnetization and magnetic anisotropy of the nanoparticles, we show that MC simulations can reproduce the thickness-dependent magnetic behavior. The magnetic dipolar particle interactions induce a ferromagnetic coupling that increases in strength with decreasing thickness of the array. The 2D to 3D transition in the magnetic properties is mainly driven by a change in the orientation of the magnetic vortex states with increasing thickness, becoming more isotropic as the thickness of the array increases. Magnetic anisotropy prevents long-range ferromagnetic order from being established at low temperature and the nanoparticle magnetic moments instead freeze along directions defined by the distribution of easy magnetization directions.
Subject headings
- NATURVETENSKAP -- Kemi -- Materialkemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Materials Chemistry (hsv//eng)
Keyword
- Teknisk fysik med inriktning mot fasta tillståndets fysik
- Engineering Science with specialization in Solid State Physics
- Materials Chemistry
Publication and Content Type
- ref (subject category)
- art (subject category)
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Nanoscale
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To the university's database
- By the author/editor
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Faure, B.
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Wetterskog, Erik ...
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Gunnarsson, Klas
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Josten, E.
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Hermann, R. P.
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Brückel, T.
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show more...
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Andreasen, J. W.
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Meneau, F.
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Meyer, M.
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Lyubartsev, Alex ...
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Bergström, Lenna ...
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Salazar-Alvarez, ...
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Svedlindh, Peter
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show less...
- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Chemical Science ...
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and Materials Chemis ...
- Articles in the publication
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Nanoscale
- By the university
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Uppsala University
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Stockholm University