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Mesoscale morpholog...
Mesoscale morphology of airborne core-shell nanoparticle clusters : x-ray laser coherent diffraction imaging
- Article/chapterEnglish2013
Publisher, publication year, extent ...
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2013-08-13
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IOP Publishing,2013
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printrdacarrier
Numbers
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LIBRIS-ID:oai:DiVA.org:uu-210260
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https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-210260URI
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https://doi.org/10.1088/0953-4075/46/16/164033DOI
Supplementary language notes
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Language:English
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Summary in:English
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Subject category:ref swepub-contenttype
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Subject category:art swepub-publicationtype
Notes
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Unraveling the complex morphology of functional materials like core-shell nanoparticles and its evolution in different environments is still a challenge. Only recently has the single-particle coherent diffraction imaging (CDI), enabled by the ultrabright femtosecond free-electron laser pulses, provided breakthroughs in understanding mesoscopic morphology of nanoparticulate matter. Here, we report the first CDI results for Co@SiO2 core-shell nanoparticles randomly clustered in large airborne aggregates, obtained using the x-ray free-electron laser at the Linac Coherent Light Source. Our experimental results compare favourably with simulated diffraction patterns for clustered Co@SiO2 nanoparticles with similar to 10 nm core diameter and similar to 30 nm shell outer diameter, which confirms the ability to resolve the mesoscale morphology of complex metastable structures. The findings in this first morphological study of core-shell nanomaterials are a solid base for future time-resolved studies of dynamic phenomena in complex nanoparticulate matter using x-ray lasers.
Subject headings and genre
Added entries (persons, corporate bodies, meetings, titles ...)
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Loh, N. D.
(author)
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Capotondi, F.
(author)
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Hampton, C. Y.
(author)
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Sierra, R. G.
(author)
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Starodub, D.
(author)
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Bostedt, C.
(author)
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Bozek, J.
(author)
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Nelson, A. J.
(author)
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Aslam, M.
(author)
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Li, S.
(author)
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Dravid, V. P.
(author)
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Martin, A. V.
(author)
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Aquila, A.
(author)
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Barty, A.
(author)
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Fleckenstein, H.
(author)
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Gumprecht, L.
(author)
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Liang, M.
(author)
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Nass, K.
(author)
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Schulz, J.
(author)
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White, T. A.
(author)
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Coppola, N.
(author)
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Bajt, S.
(author)
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Barthelmess, M.
(author)
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Graafsma, H.
(author)
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Hirsemann, H.
(author)
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Wunderer, C.
(author)
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Epp, S. W.
(author)
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Erk, B.
(author)
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Rudek, B.
(author)
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Rudenko, A.
(author)
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Foucar, L.
(author)
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Kassemeyer, S.
(author)
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Lomb, L.
(author)
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Rolles, D.
(author)
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Shoeman, R. L.
(author)
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Steinbrener, J.
(author)
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Hartmann, R.
(author)
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Hartmann, A.
(author)
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Hauser, G.
(author)
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Holl, P.
(author)
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Kimmel, N.
(author)
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Reich, C.
(author)
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Soltau, H.
(author)
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Weidenspointner, G.
(author)
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Benner, W. H.
(author)
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Farquar, G. R.
(author)
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Hau-Riege, S. P.
(author)
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Hunter, M. S.
(author)
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Ekeberg, TomasUppsala universitet,Molekylär biofysik(Swepub:uu)tomek611
(author)
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Hantke, MaxUppsala universitet,Molekylär biofysik(Swepub:uu)maxha207
(author)
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Maia, Filipe R. N. C.Uppsala universitet,Molekylär biofysik(Swepub:uu)fimai103
(author)
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Tobias, H. J.
(author)
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Marchesini, S.
(author)
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Frank, M.
(author)
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Strueder, L.
(author)
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Schlichting, I.
(author)
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Ullrich, J.
(author)
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Chapman, H. N.
(author)
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Bucksbaum, P. H.
(author)
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Kiskinova, M.
(author)
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Bogan, M. J.
(author)
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Uppsala universitetMolekylär biofysik
(creator_code:org_t)
Related titles
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In:Journal of Physics B: IOP Publishing46:16 SI, s. 164033-0953-40751361-6455
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Find in a library
To the university's database
- By the author/editor
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Pedersoli, E.
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Loh, N. D.
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Capotondi, F.
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Hampton, C. Y.
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Sierra, R. G.
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Starodub, D.
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show more...
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Bostedt, C.
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Bozek, J.
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Nelson, A. J.
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Aslam, M.
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Li, S.
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Dravid, V. P.
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Martin, A. V.
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Aquila, A.
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Barty, A.
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Fleckenstein, H.
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Gumprecht, L.
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Liang, M.
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Nass, K.
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Schulz, J.
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White, T. A.
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Coppola, N.
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Bajt, S.
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Barthelmess, M.
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Graafsma, H.
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Hirsemann, H.
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Wunderer, C.
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Epp, S. W.
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Erk, B.
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Rudek, B.
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Rudenko, A.
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Foucar, L.
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Kassemeyer, S.
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Lomb, L.
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Rolles, D.
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Shoeman, R. L.
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Steinbrener, J.
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Hartmann, R.
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Hartmann, A.
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Hauser, G.
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Holl, P.
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Kimmel, N.
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Reich, C.
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Soltau, H.
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Weidenspointner, ...
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Benner, W. H.
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Farquar, G. R.
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Hau-Riege, S. P.
-
Hunter, M. S.
-
Ekeberg, Tomas
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Hantke, Max
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Maia, Filipe R. ...
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Tobias, H. J.
-
Marchesini, S.
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Frank, M.
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Strueder, L.
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Schlichting, I.
-
Ullrich, J.
-
Chapman, H. N.
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Bucksbaum, P. H.
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Kiskinova, M.
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Bogan, M. J.
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- NATURAL SCIENCES
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NATURAL SCIENCES
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Journal of Physi ...
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Uppsala University