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  • Rath, Asawari D.Uppsala universitet,Molekylär biofysik (author)

Explosion dynamics of sucrose nanospheres monitored by time of flight spectrometry and coherent diffractive imaging at the split-and-delay beam line of the FLASH soft X-ray laser

  • Article/chapterEnglish2014

Publisher, publication year, extent ...

  • 2014
  • printrdacarrier

Numbers

  • LIBRIS-ID:oai:DiVA.org:uu-237616
  • https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-237616URI
  • https://doi.org/10.1364/OE.22.028914DOI

Supplementary language notes

  • Language:English
  • Summary in:English

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  • Subject category:ref swepub-contenttype
  • Subject category:art swepub-publicationtype

Notes

  • We use a Mach-Zehnder type autocorrelator to split and delay XUV pulses from the FLASH soft X-ray laser for triggering and subsequently probing the explosion of aerosolised sugar balls. FLASH was running at 182 eV photon energy with pulses of 70 fs duration. The delay between the pump-probe pulses was varied between zero and 5 ps, and the pulses were focused to reach peak intensities above 1016 W/cm2 with an off-axis parabola. The direct pulse triggered the explosion of single aerosolised sucrose nano-particles, while the delayed pulse probed the exploding structure. The ejected ions were measured by ion time of flight spectrometry, and the particle sizes were measured by coherent diffractive imaging. The results show that sucrose particles of 560-1000 nm diameter retain their size for about 500 fs following the first exposure. Significant sample expansion happens between 500 fs and 1 ps. We present simulations to support these observations.

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  • Timneanu, NicusorUppsala universitet,Molekylär biofysik(Swepub:uu)nti19847 (author)
  • Maia, Filipe R. N. C.Uppsala universitet,Molekylär biofysik(Swepub:uu)fimai103 (author)
  • Bielecki, JohanUppsala universitet,Molekylär biofysik(Swepub:uu)johbi267 (author)
  • Fleckenstein, Holger (author)
  • Iwan, BiancaUppsala universitet,Molekylär biofysik(Swepub:uu)biaiw419 (author)
  • Svenda, MartinUppsala universitet,Molekylär biofysik(Swepub:uu)msv31659 (author)
  • Hasse, DirkUppsala universitet,Molekylär biofysik(Swepub:uu)dirha931 (author)
  • Carlsson, GunillaUppsala universitet,Molekylär biofysik(Swepub:uu)gca29842 (author)
  • Westphal, DanielUppsala universitet,Molekylär biofysik(Swepub:uu)danwe345 (author)
  • Mühlig, KerstinUppsala universitet,Molekylär biofysik(Swepub:uu)kermu539 (author)
  • Hantke, MaxUppsala universitet,Molekylär biofysik(Swepub:uu)maxha207 (author)
  • Ekeberg, TomasUppsala universitet,Molekylär biofysik(Swepub:uu)tomek611 (author)
  • Seibert, M. MarvinUppsala universitet,Molekylär biofysik(Swepub:uu)masei255 (author)
  • Zani, AlessandroUppsala universitet,Molekylär biofysik(Swepub:uu)aleza299 (author)
  • Liang, Mengning (author)
  • Stellato, Francesco (author)
  • Kirian, Richard (author)
  • Bean, Richard (author)
  • Barty, Anton (author)
  • Galli, Lorenzo (author)
  • Nass, Karol (author)
  • Barthelmess, Miriam (author)
  • Aquila, Andrew (author)
  • Toleikis, Sven (author)
  • Treusch, Rolf (author)
  • Roling, Sebastian (author)
  • Wöstmann, Michael (author)
  • Zacharias, Helmut (author)
  • Chapman, Henry N. (author)
  • Bajt, Saša (author)
  • DePonte, Daniel (author)
  • Hajdu, JanosUppsala universitet,Molekylär biofysik(Swepub:uu)janohajd (author)
  • Andreasson, JakobUppsala universitet,Molekylär biofysik(Swepub:uu)jakan998 (author)
  • Uppsala universitetMolekylär biofysik (creator_code:org_t)

Related titles

  • In:Optics Express22:23, s. 28914-289251094-4087

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