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Evolution of hydrog...
Evolution of hydrogen by few-layered black phosphorus under visible illumination
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- Muduli, Subas Kumar (author)
- Energy Res Inst NTU, Res Techno Plaza,50 Nanyang Dr, Singapore 637553, Singapore.
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- Varrla, Eswaraiah (author)
- Energy Res Inst NTU, Res Techno Plaza,50 Nanyang Dr, Singapore 637553, Singapore.;SRM Univ, Dept Phys & Nanotechnol, SRM Res Inst, Madras 603203, Tamil Nadu, India.
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- Xu, You (author)
- Nanyang Technol Univ, Sch Chem & Biomed Engn, 62 Nanyang Dr, Singapore 637459, Singapore.
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- Kulkarni, Sneha Avinash (author)
- Energy Res Inst NTU, Res Techno Plaza,50 Nanyang Dr, Singapore 637553, Singapore.
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- Katre, Ankita (author)
- CEA Grenoble, LITEN, 17 Rue Martyrs, F-38054 Grenoble 9, France.
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- Chakraborty, Sudip (author)
- Uppsala universitet,Materialteori
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- Chen, Shi (author)
- Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, 21 Nanyang Link, Singapore 637371, Singapore.
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- Sum, Tze Chien (author)
- Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, 21 Nanyang Link, Singapore 637371, Singapore.
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- Xu, Rong (author)
- Nanyang Technol Univ, Sch Chem & Biomed Engn, 62 Nanyang Dr, Singapore 637459, Singapore.
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- Mathews, Nripan (author)
- Energy Res Inst NTU, Res Techno Plaza,50 Nanyang Dr, Singapore 637553, Singapore.;Nanyang Technol Univ, Sch Mat Sci & Engn, Nanyang Ave, Singapore 639798, Singapore.
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Energy Res Inst NTU, Res Techno Plaza,50 Nanyang Dr, Singapore 637553, Singapore Energy Res Inst NTU, Res Techno Plaza,50 Nanyang Dr, Singapore 637553, Singapore.;SRM Univ, Dept Phys & Nanotechnol, SRM Res Inst, Madras 603203, Tamil Nadu, India. (creator_code:org_t)
- 2017
- 2017
- English.
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In: Journal of Materials Chemistry A. - : Royal Society of Chemistry (RSC). - 2050-7488 .- 2050-7496. ; 5:47, s. 24874-24879
- Related links:
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https://dr.ntu.edu.s...
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
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- Recently, a new class of two-dimensional black phosphorus (BP) with a visible direct band gap is predicted as a potential candidate for photo-catalysis applications. Here, we present the first experimental evidence of hydrogen (H-2) evolution from aqueous solution by using BP (nanosheets and nanoparticles) under visible light illumination. Our experimental results describe that liquid phase exfoliated BP nanosheets and BP nanoparticles exhibit suitable energy level alignments for electron transfer and further proton reduction reactions in the solution under visible light illumination. Density functional theory (DFT) calculations predict that the H-2 evolution activity of bilayer BP is independent of edge or center positions, which is unique in BP as compared to those of other 2D materials.
Subject headings
- NATURVETENSKAP -- Kemi -- Materialkemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Materials Chemistry (hsv//eng)
Publication and Content Type
- ref (subject category)
- art (subject category)
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- By the author/editor
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Muduli, Subas Ku ...
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Varrla, Eswaraia ...
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Xu, You
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Kulkarni, Sneha ...
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Katre, Ankita
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Chakraborty, Sud ...
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show more...
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Chen, Shi
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Sum, Tze Chien
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Xu, Rong
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Mathews, Nripan
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- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Chemical Science ...
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and Materials Chemis ...
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Journal of Mater ...
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Uppsala University