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Role of the orbital...
Role of the orbital moment in a series of isostructural weak ferromagnets
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- Pincini, D. (author)
- UCL, London Ctr Nanotechnol, Gower St, London WC1E 6BT, England;UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England;Diamond Light Source Ltd, Diamond House,Harwell Sci & Innovat Campus, Didcot OX11 0DE, Oxon, England
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- Fabrizi, F. (author)
- Diamond Light Source Ltd, Diamond House,Harwell Sci & Innovat Campus, Didcot OX11 0DE, Oxon, England
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- Beutier, G. (author)
- Univ Grenoble Alpes, CNRS, Grenoble INP, SIMaP, F-38000 Grenoble, France
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- Nisbet, G. (author)
- Diamond Light Source Ltd, Diamond House,Harwell Sci & Innovat Campus, Didcot OX11 0DE, Oxon, England
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- Elnaggar, H. (author)
- Univ Utrecht, Debye Inst Nanomat Sci, Univ Weg 99, NL-3584 CG Utrecht, Netherlands
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- Dmitrienko, V. E. (author)
- AV Shubnikov Inst Crystallog, FSRC Crystallog & Photon RAS, Moscow 119333, Russia
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Katsnelson, M. , I (author)
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- Kvashnin, Yaroslav (author)
- Uppsala universitet,Materialteori
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Lichtenstein, A. , I (author)
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- Mazurenko, V. V. (author)
- Ural Fed Univ, Dept Theoret Phys & Appl Math, Mira Str 19, Ekaterinburg 620002, Russia
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- Ovchinnikova, E. N. (author)
- Moscow MV Lomonosov State Univ, Fac Phys, Moscow 119991, Russia
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Dimitrova, O. , V (author)
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- Collins, S. P. (author)
- Diamond Light Source Ltd, Diamond House,Harwell Sci & Innovat Campus, Didcot OX11 0DE, Oxon, England
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(creator_code:org_t)
- AMER PHYSICAL SOC, 2018
- 2018
- English.
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In: Physical Review B. - : AMER PHYSICAL SOC. - 2469-9950 .- 2469-9969. ; 98:10
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Abstract
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- The orbital contribution to the magnetic moment of the transition-metal ion in the isostructural weak ferromagnets ACO(3) (A = Mn,Co,Ni) and FeBO3 was investigated by a combination of first-principles calculations, nonresonant x-ray magnetic scattering, and x-ray magnetic circular dichroism. A nontrivial evolution of the orbital moment as a function of the 3d orbitals filling is revealed, with a particularly large value found in the Co member of the family. Here, the coupling between magnetic and lattice degrees of freedom produced by the spin-orbit interaction results in a large single-ion anisotropy and a peculiar magnetic-moment-induced electron cloud distortion, evidenced by the appearance of a subtle scattering amplitude at space-group-forbidden reflections and significant magnetostrictive effects. Our results, which complement a previous investigation on the sign of the Dzyaloshinskii-Moriya interaction across the series, highlight the importance of spin-orbit coupling in the physics of weak ferromagnets and prove the ability of modern first-principles calculations to predict the properties of materials where the Dzyaloshinskii-Moriya interaction is a fundamental ingredient of the magnetic Hamiltonian.
Subject headings
- NATURVETENSKAP -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Condensed Matter Physics (hsv//eng)
Publication and Content Type
- ref (subject category)
- art (subject category)
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- By the author/editor
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Pincini, D.
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Fabrizi, F.
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Beutier, G.
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Nisbet, G.
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Elnaggar, H.
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Dmitrienko, V. E ...
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show more...
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Katsnelson, M. , ...
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Kvashnin, Yarosl ...
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Lichtenstein, A. ...
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Mazurenko, V. V.
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Ovchinnikova, E. ...
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Dimitrova, O. , ...
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Collins, S. P.
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- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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and Condensed Matter ...
- Articles in the publication
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Physical Review ...
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Uppsala University