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Observation of the ...
Observation of the fastest chemical processes in the radiolysis of water
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- Loh, Z-H (author)
- Nanyang Technol Univ, Sch Phys & Math Sci, Div Chem & Biol Chem, Singapore, Singapore
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- Doumy, G. (author)
- Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA
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- Arnold, C. (author)
- DESY, Ctr Free Electron Laser Sci, Hamburg, Germany;Univ Hamburg, Dept Phys, Hamburg, Germany;Hamburg Ctr Ultrafast Imaging, Hamburg, Germany
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- Kjellsson, Ludvig (author)
- Uppsala universitet,Molekyl- och kondenserade materiens fysik,European XFEL GmbH, Schenefeld, Germany
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- Southworth, S. H. (author)
- Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA
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- Al Haddad, A. (author)
- Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA
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- Kumagai, Y. (author)
- Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA
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- Tu, M-F (author)
- Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA
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- Ho, P. J. (author)
- Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA
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- March, A. M. (author)
- Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA
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- Schaller, R. D. (author)
- Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL USA;Northwestern Univ, Dept Chem, Evanston, IL USA
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- Yusof, M. S. Bin Mohd (author)
- Nanyang Technol Univ, Sch Phys & Math Sci, Div Chem & Biol Chem, Singapore, Singapore
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- Debnath, T. (author)
- Nanyang Technol Univ, Sch Phys & Math Sci, Div Chem & Biol Chem, Singapore, Singapore
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- Simon, M. (author)
- Sorbonne Univ, F-750005 Paris, France;CNRS, LCPMR, F-750005 Paris, France
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- Welsch, R. (author)
- DESY, Ctr Free Electron Laser Sci, Hamburg, Germany;Hamburg Ctr Ultrafast Imaging, Hamburg, Germany
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- Inhester, L. (author)
- DESY, Ctr Free Electron Laser Sci, Hamburg, Germany
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- Khalili, K. (author)
- Tech Univ Denmark, Dept Energy Convers & Storage, Roskilde, Denmark
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- Nanda, K. (author)
- Univ Southern Calif, Dept Chem, Los Angeles, CA 90007 USA
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Krylov, A. , I (author)
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- Moeller, S. (author)
- SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA USA
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- Coslovich, G. (author)
- SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA USA
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- Koralek, J. (author)
- SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA USA
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- Minitti, M. P. (author)
- SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA USA
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- Schlotter, W. F. (author)
- SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA USA
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- Rubensson, Jan-Erik (author)
- Uppsala universitet,Molekyl- och kondenserade materiens fysik
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- Santra, R. (author)
- DESY, Ctr Free Electron Laser Sci, Hamburg, Germany;Univ Hamburg, Dept Phys, Hamburg, Germany;Hamburg Ctr Ultrafast Imaging, Hamburg, Germany
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- Young, L. (author)
- Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA;Univ Chicago, Dept Phys, Chicago, IL 60637 USA;Univ Chicago, James Franck Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA
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(creator_code:org_t)
- AMER ASSOC ADVANCEMENT SCIENCE, 2020
- 2020
- English.
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In: Science. - : AMER ASSOC ADVANCEMENT SCIENCE. - 0036-8075 .- 1095-9203. ; 367:6474, s. 179-182
- Related links:
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https://bib-pubdb1.d...
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
Subject headings
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- Elementary processes associated with ionization of liquid water provide a framework for understanding radiation-matter interactions in chemistry and biology. Although numerous studies have been conducted on the dynamics of the hydrated electron, its partner arising from ionization of liquid water, H2O+, remains elusive. We used tunable femtosecond soft x-ray pulses from an x-ray free electron laser to reveal the dynamics of the valence hole created by strong-field ionization and to track the primary proton transfer reaction giving rise to the formation of OH. The isolated resonance associated with the valence hole (H2O+/OH) enabled straightforward detection. Molecular dynamics simulations revealed that the x-ray spectra are sensitive to structural dynamics at the ionization site. We found signatures of hydrated-electron dynamics in the x-ray spectrum.
Subject headings
- NATURVETENSKAP -- Kemi -- Materialkemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Materials Chemistry (hsv//eng)
Publication and Content Type
- ref (subject category)
- art (subject category)
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To the university's database
- By the author/editor
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Loh, Z-H
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Doumy, G.
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Arnold, C.
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Kjellsson, Ludvi ...
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Southworth, S. H ...
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Al Haddad, A.
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show more...
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Kumagai, Y.
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Tu, M-F
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Ho, P. J.
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March, A. M.
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Schaller, R. D.
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Yusof, M. S. Bin ...
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Debnath, T.
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Simon, M.
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Welsch, R.
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Inhester, L.
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Khalili, K.
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Nanda, K.
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Krylov, A. , I
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Moeller, S.
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Coslovich, G.
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Koralek, J.
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Minitti, M. P.
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Schlotter, W. F.
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Rubensson, Jan-E ...
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Santra, R.
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Young, L.
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- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Chemical Science ...
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and Materials Chemis ...
- Articles in the publication
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Science
- By the university
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Uppsala University