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  • Kjellsson, LudvigUppsala universitet,Molekyl- och kondenserade materiens fysik,European XFEL GmbH, Holzkoppel 4, 22869 Schenefeld, Germany (author)

Resonant inelastic x-ray scattering at the N2 π*-resonance: Lifetime-vibrational interference, radiative electron rearrangement, and wave-function imaging

  • Article/chapterEnglish2021

Publisher, publication year, extent ...

  • American Physical Society,2021
  • electronicrdacarrier

Numbers

  • LIBRIS-ID:oai:DiVA.org:uu-433870
  • https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-433870URI
  • https://doi.org/10.1103/PhysRevA.103.022812DOI

Supplementary language notes

  • Language:English
  • Summary in:English

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  • Subject category:ref swepub-contenttype
  • Subject category:art swepub-publicationtype

Notes

  • Resonant inelastic x-ray scattering spectra excited at the pi*-resonance of the nitrogen molecule are presented. Well-resolved vibrational excitations in the electronic ground state, and in the 3 sigma g(-1 )1 pi(1)(g) a(1) Pi(g) state are observed. The spectra are analyzed within the Kramers-Heisenberg formalism, and the importance of lifetime-vibrational interference effects is highlighted. In addition, strongly dissociative multiply excited final states populated in radiative electron rearrangement are found in the valence ionization continua. The vibrational wave functions of the core-excited state are imaged on the strongly dissociative final state potentials.

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  • Ekholm, VictorMAX IV Laboratory, Lund University, Box 118, Lund SE-221 00, Sweden (author)
  • Agåker, MarcusUppsala universitet,Molekyl- och kondenserade materiens fysik,MAX IV Laboratory, Lund University, Box 118, Lund SE-221 00, Sweden(Swepub:uu)maaga227 (author)
  • Såthe, ConnyMAX IV Laboratory, Lund University, Box 118, Lund SE-221 00, Sweden (author)
  • Pietzsch, A.Helmholtz Zentrum Berlin, Institute Methods and Instrumentation for Synchrotron Radiation Research, Albert-Einstein-Straße 15, 12489 Berlin, Germany (author)
  • Karlsson, Hans O.,1965-Uppsala universitet,Avdelningen för beräkningsvetenskap(Swepub:uu)hanskarl (author)
  • Jaouen, N.Synchrotron SOLEIL, Saint-Aubin, Boite Postale 48, 91192 Gif-sur-Yvette Cedex, France (author)
  • Nicolau, A.Synchrotron SOLEIL, Saint-Aubin, Boite Postale 48, 91192 Gif-sur-Yvette Cedex, France (author)
  • Guarise, M.Brazilian Center for Research in Energy and Materials (CNPEM), Rua Giuseppe Máximo Scolfaro, 10.000 Polo II de Alta Tecnologia de Campinas, Campinas, São Paulo, Brazil (author)
  • Hague, C.Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, F-75005 Paris, France (author)
  • Lüning, J.Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, F-75005 Paris, France;Helmholtz-Zentrum Berlin für Materialien und Energie, Hahn-Meitner-Platz 1, 14109 Berlin, Germany (author)
  • Chiuzbăian, S.G.Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, F-75005 Paris, France (author)
  • Rubensson, Jan-ErikUppsala universitet,Molekyl- och kondenserade materiens fysik(Swepub:uu)janerube (author)
  • Uppsala universitetMolekyl- och kondenserade materiens fysik (creator_code:org_t)

Related titles

  • In:Physical Review A. Atomic, Molecular, and Optical Physics: American Physical Society1031050-29471094-1622

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