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Photoexcitation-Bas...
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Yue, BingbingUniv Shanghai Sci & Technol, Sch Mat & Chem, Shanghai 200093, Peoples R China.;Fudan Univ, Dept Macromol Sci, State Key Lab Mol Engn Polymers, Shanghai 200438, Peoples R China.
(author)
Photoexcitation-Based Supramolecular Access to Full-Scale Phase-Diagram Structures through in situ Phase-Volume Ratio Phototuning
- Article/chapterEnglish2022
Publisher, publication year, extent ...
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2022-09-20
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John Wiley & Sons,2022
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printrdacarrier
Numbers
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LIBRIS-ID:oai:DiVA.org:uu-495165
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https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-495165URI
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https://doi.org/10.1002/anie.202209777DOI
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https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-189086URI
Supplementary language notes
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Language:English
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Summary in:English
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Subject category:ref swepub-contenttype
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Subject category:art swepub-publicationtype
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Funding Agencies|Shanghai Sailing Program [20YF1432400]; National Natural Science Foundation of China (NSFC) [22105128]; National Key Research and Development Program of China [2017YFA0207700]; Swedish Research Council [2020-04600, SNIC 2020-3-29, 2018-05973]
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Controlling phase separation and transition plays a core role in establishing and maintaining the function of diverse self-assembled systems. However, it remains challenging to achieve wide-range continuous phase transition for dynamically producing a variety of assembled structures. Here, we developed a far-from-equilibrium system, upon the integration of photoexcitation-induced aggregation molecules and block copolymers, to establish an in situ phase-volume ratio photocontrol strategy. Thus, full-scale phase-diagram structures, from lamellar structure to gyroidal, cylindrical, and finally to a spherical one, can be accessed under different irradiation periods. Moreover, the phase transition was accompanied by considerable aggregation-induced phosphorescence and hydrophilicity/hydrophobicity change for building a functional surface. This strategy allows for a conceptual advance of accessing a wide range of distinct self-assembled structures and functions in real time.
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Jia, XiaoyongFudan Univ, Dept Macromol Sci, State Key Lab Mol Engn Polymers, Shanghai 200438, Peoples R China.;Henan Univ, Coll Chem & Chem Engn, Henan Ctr Outstanding Overseas Scientists, Kaifeng 475004, Henan, Peoples R China.
(author)
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Baryshnikov, GlibLinköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten(Swepub:liu)gliba58
(author)
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Jin, XinWenzhou Med Univ, Sch Biomed Engn, Inst Lasers & Biophoton, Wenzhou 325035, Zhejiang, Peoples R China.
(author)
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Feng, XichengUniv Shanghai Sci & Technol, Sch Mat & Chem, Shanghai 200093, Peoples R China.
(author)
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Lu, YunleUniv Shanghai Sci & Technol, Sch Mat & Chem, Shanghai 200093, Peoples R China.;Fudan Univ, Dept Macromol Sci, State Key Lab Mol Engn Polymers, Shanghai 200438, Peoples R China.
(author)
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Luo, MengkaiFudan Univ, Dept Macromol Sci, State Key Lab Mol Engn Polymers, Shanghai 200438, Peoples R China.
(author)
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Zhang, ManFudan Univ, Dept Macromol Sci, State Key Lab Mol Engn Polymers, Shanghai 200438, Peoples R China.
(author)
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Shen, ShenFudan Univ, Dept Macromol Sci, State Key Lab Mol Engn Polymers, Shanghai 200438, Peoples R China.
(author)
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Ågren, HansUppsala universitet,Kemisk och biomolekylär fysik,Henan Univ, Coll Chem & Chem Engn, Henan Ctr Outstanding Overseas Scientists, Kaifeng 475004, Henan, Peoples R China.,Henan Univ, Peoples R China; Uppsala Univ, Sweden(Swepub:uu)hanag788
(author)
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Zhu, LiangliangFudan Univ, Dept Macromol Sci, State Key Lab Mol Engn Polymers, Shanghai 200438, Peoples R China.
(author)
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Univ Shanghai Sci & Technol, Sch Mat & Chem, Shanghai 200093, Peoples R China.;Fudan Univ, Dept Macromol Sci, State Key Lab Mol Engn Polymers, Shanghai 200438, Peoples R China.Fudan Univ, Dept Macromol Sci, State Key Lab Mol Engn Polymers, Shanghai 200438, Peoples R China.;Henan Univ, Coll Chem & Chem Engn, Henan Ctr Outstanding Overseas Scientists, Kaifeng 475004, Henan, Peoples R China.
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In:Angewandte Chemie International Edition: John Wiley & Sons61:431433-78511521-3773
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Yue, Bingbing
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Jia, Xiaoyong
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Baryshnikov, Gli ...
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Jin, Xin
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Feng, Xicheng
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Lu, Yunle
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Luo, Mengkai
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Zhang, Man
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Shen, Shen
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Ågren, Hans
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Zhu, Liangliang
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