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  • Andersson, Patrik U,1970Gothenburg University,Göteborgs universitet,Institutionen för kemi och molekylärbiologi,Department of Chemistry and Molecular Biology (author)

Cluster ions DN + ejected from dense and ultra-dense deuterium by Coulomb explosions: Fragment rotation and D+ backscattering from ultra-dense clusters in the surface phase

  • Article/chapterEnglish2012

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  • Elsevier BV,2012

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  • LIBRIS-ID:oai:gup.ub.gu.se/157730
  • https://gup.ub.gu.se/publication/157730URI
  • https://doi.org/10.1016/j.ijms.2011.11.004DOI

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  • Language:English

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  • Subject category:ref swepub-contenttype
  • Subject category:art swepub-publicationtype

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  • The two forms of condensed atomic deuterium, dense deuterium D(1) and ultra-dense deuterium D(−1), can be studied by laser-induced Coulomb explosion time-of-flight mass spectrometry and neutral timeof- flight. In the present study pulsed laser intensity below 1014W cm−2 is used. Cluster ions DN + from D(1) are observed with N = 3, 4, 12 and 17, thus not in close-packed forms. Clusters DN(1) are mainly in the form of chains of D2 and D3 groups, a shape derived from the D(−1) material which D(1) is spontaneously converted to. Only atomic ions D+ with initial kinetic energy of hundreds of eV are observed from D(−1). Half of these ions are ejected from the emitter surface, half of them penetrate into the ultra-dense D(−1) layer on the emitter surface. This second half of the ions is reflected completely from the surface layer formed by ultra-dense D(−1) strongly bonded clusters D3(−1) and D4(−1).

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  • Holmlid, Leif,1942Gothenburg University,Göteborgs universitet,Institutionen för kemi och molekylärbiologi,Department of Chemistry and Molecular Biology(Swepub:gu)xholml (author)
  • Göteborgs universitetInstitutionen för kemi och molekylärbiologi (creator_code:org_t)

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  • In:International Journal of Mass Spectrometry: Elsevier BV310, s. 32-431387-3806

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