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Photoionization in the time and frequency domain
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- Isinger, M. (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Squibb, Richard J. (author)
- University of Gothenburg,Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU)
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- Busto, D. (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Gisselbrecht, M. (author)
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- (creator_code:org_t)
- American Association for the Advancement of Science (AAAS), 2017
- 2017
- English.
- In: Science. - : American Association for the Advancement of Science (AAAS). - 0036-8075 .- 1095-9203. ; 358:6365, s. 893-6
- Journal article (peer-reviewed)
Abstract
Subject headings
Close
- Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration (10−18 s) in the extreme ultraviolet spectral range. The lack of spectral resolution due to the use of short light pulses has raised issues in the interpretation of the experimental results and the comparison with theoretical calculations. We determine photoionization time delays in neon atoms over a 40 eV energy range with an interferometric technique combining high temporal and spectral resolution. We spectrally disentangle direct ionization from ionization with shake-up, in which a second electron is left in an excited state, and obtain excellent agreement with theoretical calculations, thereby solving a puzzle raised by 7-year-old measurements.
Subject headings
- NATURVETENSKAP -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)
- NATURVETENSKAP -- Fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences (hsv//eng)
Keyword
- HIGH HARMONIC-GENERATION; CORRELATION SATELLITES; PHOTOELECTRON-SPECTRA; HIGH-RESOLUTION; FANO RESONANCE; ATTOSECOND; SPECTROSCOPY; SCATTERING; DYNAMICS; STATES
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- ref (subject category)
- art (subject category)
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- Lindroth, Eva
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- L'Huillier, A.
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