Electronic Light-Matter Strong Coupling in Nanofluidic Fabry-Pérot Cavities

Electronic light-matter strong coupling has been limited to solid molecular films due to the challenge of preparing optical cavities with nanoscale dimensions. Here we report a technique to fabricate such Fabry-Pérot nanocavities in which solutions can be introduced such that light-molecule interactions can be studied at will in the liquid phase. We illustrate the versatility of these cavities by studying the emission properties of Chlorin e6 solutions in both the weak and strong coupling regimes as a function of cavity detuning. Liquid nanocavities will broaden the investigation of strong coupling to many solution-based molecular processes. © 2017 American Chemical Society.

TEKNIK OCH TEKNOLOGIER Elektroteknik och elektronik Telekommunikation hsv//swe
ENGINEERING AND TECHNOLOGY Electrical Engineering, Electronic Engineering, Information Engineering Telecommunications hsv//eng
Chlorin e6
fluorescence lifetime decay
quantum yield
Rabi splitting
radiative and nonradiative decay rates
Emission properties
Fluorescence lifetimes
Nanoscale dimensions
Nonradiative decay rate
Solid molecular films
Strong-coupling regime

Chervy, T. (author)
Thomas, A. (author)
Börjesson, Karl,1982Gothenburg University,Göteborgs universitet,Institutionen för kemi och molekylärbiologi,Department of Chemistry and Molecular Biology(Swepub:gu)xbokar (author)
Hertzog, M. (author)
George, J. (author)
Devaux, E. (author)
Genet, C. (author)
Hutchison, J. A. (author)
Ebbesen, T. W. (author)
Göteborgs universitetInstitutionen för kemi och molekylärbiologi (creator_code:org_t)

By the author/editor: Bahsoun, H.; Chervy, T.; Thomas, A.; Börjesson, Karl, ...; Hertzog, M.; George, J.; show more...; Devaux, E.; Genet, C.; Hutchison, J. A.; Ebbesen, T. W.; show less...

About the subject

ENGINEERING AND TECHNOLOGY: ENGINEERING AND ...; and Electrical Engin ...; and Telecommunicatio ...

Kungliga biblioteket hanterar dina personuppgifter i enlighet med EU:s dataskyddsförordning (2018), GDPR. Läs mer om hur det funkar här.
Så här hanterar KB dina uppgifter vid användning av denna tjänst.