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Magic numbers and stabilities of heavy water clusters,(D2O)ND+, N = 3 −48
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- Hansen, Klavs, 1958 (author)
- Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU)
- Ryding, Mauritz Johan, 1981 (author)
- Uggerud, einar (author)
- (creator_code:org_t)
- Elsevier BV, 2019
- 2019
- English.
- In: International Journal of Mass Spectrometry. - : Elsevier BV. - 1387-3806. ; 440, s. 14-19
- Journal article (peer-reviewed)
Abstract
Subject headings
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- The abundance spectrum of deuterated heavy water clusters has been measured, and relative dissociationenergies were extracted from the abundances. The dissociation energies are similar to those of protonatedlight water clusters, except for a slightly reduced excess stability of the N = 21 cluster relative to the N = 22cluster. The difference is interpreted in terms of the special geometry of the N = 21 cluster. The absenceof a similar effect for N = 28/29 suggests that the stability of the N = 28 cluster is not due to a closed shellstructure
Subject headings
- NATURVETENSKAP -- Kemi -- Fysikalisk kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Physical Chemistry (hsv//eng)
- NATURVETENSKAP -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)
Keyword
- Heavy water; Clusters; Unimolecular reactions; Binding energies
Publication and Content Type
- ref (subject category)
- art (subject category)
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