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Secondary organic a...
Secondary organic aerosol formation from straw burning using an oxidation flow reactor
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Wang, H. (author)
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Guo, S. (author)
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Wu, Z. (author)
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Qiao, K. (author)
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Tang, R. (author)
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Yu, Y. (author)
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Xu, W. (author)
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Zhu, W. (author)
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Zeng, L. (author)
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Huang, X. (author)
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He, L. (author)
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- Hallquist, Mattias, 1969 (author)
- Gothenburg University,Göteborgs universitet,Institutionen för kemi och molekylärbiologi,Department of Chemistry and Molecular Biology
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(creator_code:org_t)
- Elsevier BV, 2022
- 2022
- English.
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In: Journal of Environmental Sciences (China). - : Elsevier BV. - 1001-0742. ; 114, s. 249-258
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https://gup.ub.gu.se...
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https://doi.org/10.1...
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Abstract
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- Herein, we use an oxidation flow reactor, Gothenburg: Potential Aerosol Mass (Go: PAM) reactor, to investigate the secondary organic aerosol (SOA) formation from wheat straw burning. Biomass burning emissions are exposed to high concentrations of hydroxyl radicals (OH) to simulate processes equivalent to atmospheric oxidation of 0-2.55 days. Primary volatile organic compounds (VOCs) were investigated, and particles were measured before and after the Go: PAM reactor. The influence of water content (i.e. 5% and 11%) in wheat straw was also explored. Two burning stages, the flaming stage, and non-flaming stages, were identified. Primary particle emission factors (EFs) at a water content of 11% (∼3.89 g/kg-fuel) are significantly higher than those at a water content of 5% (∼2.26 g/kg-fuel) during the flaming stage. However, the water content showed no significant influence at the non-flaming stage. EFs of aromatics at a non-flaming stage (321.8±46.2 mg/kg-fuel) are larger than that at a flaming stage (130.9±37.1 mg/kg-fuel). The OA enhancement ratios increased with the increase in OH exposure at first and decreased with the additional increment of OH exposure. The maximum OA enhancement ratio is ∼12 during the non-flaming stages, which is much higher than ∼ 1.7 during the flaming stages. The mass spectrum of the primary wheat burning organic aerosols closely resembles that of resolved biomass burning organic aerosols (BBOA) based on measurements in ambient air. Our results show that large gap (∼60%-90%) still remains to estimate biomass burning SOA if only the oxidation of VOCs were included. © 2021
Subject headings
- NATURVETENSKAP -- Geovetenskap och miljövetenskap -- Meteorologi och atmosfärforskning (hsv//swe)
- NATURAL SCIENCES -- Earth and Related Environmental Sciences -- Meteorology and Atmospheric Sciences (hsv//eng)
- NATURVETENSKAP -- Geovetenskap och miljövetenskap -- Miljövetenskap (hsv//swe)
- NATURAL SCIENCES -- Earth and Related Environmental Sciences -- Environmental Sciences (hsv//eng)
- NATURVETENSKAP -- Kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences (hsv//eng)
- NATURVETENSKAP -- Geovetenskap och miljövetenskap -- Klimatforskning (hsv//swe)
- NATURAL SCIENCES -- Earth and Related Environmental Sciences -- Climate Research (hsv//eng)
Keyword
- Flaming
- Gothenburg: Potential Aerosol Mass (Go: PAM) reactor
- Non-flaming
- Secondary organic aerosol formation
- Wheat straw burning
- Aerosols
- Biomass
- Mass spectrometry
- Oxidation
- Volatile organic compounds
- Aerosol mass
- Flow reactors
- Gothenburg: potential aerosol mass reactor
- Organic aerosol
- Organic aerosol formation
- Wheat straws
- Straw
Publication and Content Type
- ref (subject category)
- art (subject category)
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- By the author/editor
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Wang, H.
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Guo, S.
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Wu, Z.
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Qiao, K.
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Tang, R.
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Yu, Y.
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show more...
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Xu, W.
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Zhu, W.
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Zeng, L.
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Huang, X.
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He, L.
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Hallquist, Matti ...
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show less...
- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Earth and Relate ...
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and Meteorology and ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Earth and Relate ...
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and Environmental Sc ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Chemical Science ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Earth and Relate ...
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and Climate Research
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Journal of Envir ...
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University of Gothenburg